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Many-body interactions on two-dimensional electronic states formed in transition-metal oxides

Research Project

Project/Area Number 17K14325
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeMulti-year Fund
Research Field Condensed matter physics I
Research InstitutionHigh Energy Accelerator Research Organization

Principal Investigator

Yukawa Ryu  大学共同利用機関法人高エネルギー加速器研究機構, 物質構造科学研究所, 特任助教 (40759479)

Project Period (FY) 2017-04-01 – 2019-03-31
Project Status Completed (Fiscal Year 2018)
Budget Amount *help
¥4,030,000 (Direct Cost: ¥3,100,000、Indirect Cost: ¥930,000)
Fiscal Year 2018: ¥780,000 (Direct Cost: ¥600,000、Indirect Cost: ¥180,000)
Fiscal Year 2017: ¥3,250,000 (Direct Cost: ¥2,500,000、Indirect Cost: ¥750,000)
Keywords角度分解光電子分光 / 酸化物 / バンド構造 / 電子状態 / 多体間相互作用 / 表面 / 量子化 / 電子輸送
Outline of Final Research Achievements

In this study, stable electron doping method on transition-metal oxide surfaces has been established, and many-body interactions in two-dimensional electronic states (2DES) formed in a transition-metal oxide have been elucidated both by angle-resolved photoemission spectroscopy and by electronic conductivity. The main results are as follows.
(1) We have developed an alkali-metal deposition system which enables a precise control of the electron doping on transition metal oxide surfaces. (2) The origin of many-body interactions in 2DES formed at an anatase TiO2 surface has been clarified. (3) We found the difference in electron-phonon interactions between at the anatase TiO2 surface and in the bulk.

Academic Significance and Societal Importance of the Research Achievements

遷移金属酸化物においては電子輸送特性に対する多体間相互作用の寄与が大きいため、酸化物物質設計・物性制御においてキャリア密度に応じた詳細な多体間相互作用の解明が必要不可欠である。特に電子デバイスの微細化に伴う低次元系の研究において、表面・極薄膜での電子的振る舞いを理解する事が必要不可欠である。そのため、低次元系での電子の多体間相互作用を明らかにした本成果は高い重要性と発展性を持つものと考えられる。

Report

(3 results)
  • 2018 Annual Research Report   Final Research Report ( PDF )
  • 2017 Research-status Report
  • Research Products

    (12 results)

All 2019 2018 2017 Other

All Int'l Joint Research (1 results) Journal Article (6 results) (of which Int'l Joint Research: 3 results,  Peer Reviewed: 6 results,  Open Access: 2 results) Presentation (5 results) (of which Int'l Joint Research: 2 results)

  • [Int'l Joint Research] Synchrotron SOLEIL/Paris-Sud University(フランス)

    • Related Report
      2018 Annual Research Report
  • [Journal Article] Emergence of metallic monoclinic states of VO2 films induced by K deposition2019

    • Author(s)
      Shiga D.、Minohara M.、Kitamura M.、Yukawa R.、Horiba K.、Kumigashira H.
    • Journal Title

      Physical Review B

      Volume: 99 Issue: 12 Pages: 125120-125120

    • DOI

      10.1103/physrevb.99.125120

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Control of two-dimensional electronic states at anatase TiO2(001) surface by K adsorption2018

    • Author(s)
      Yukawa R.、Minohara M.、Shiga D.、Kitamura M.、Mitsuhashi T.、Kobayashi M.、Horiba K.、Kumigashira H.
    • Journal Title

      Physical Review B

      Volume: 97 Issue: 16 Pages: 165428-165428

    • DOI

      10.1103/physrevb.97.165428

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] High-density two-dimensional electron system induced by oxygen vacancies in ZnO2018

    • Author(s)
      Rodel T. C.、Dai J.、Fortuna F.、Frantzeskakis E.、Le Fevre P.、Bertran F.、Kobayashi M.、Yukawa R.、Mitsuhashi T.、Kitamura M.、Horiba K.、Kumigashira H.、Santander-Syro A. F.
    • Journal Title

      Physical Review Materials

      Volume: 2 Issue: 5

    • DOI

      10.1103/physrevmaterials.2.051601

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Converting topological insulators into topological metals within the tetradymite family2018

    • Author(s)
      Chen K.-W.、Aryal N.、Dai J.、Graf D.、Zhang S.、Das S.、Le F?vre P.、Bertran F.、Yukawa R.、Horiba K.、Kumigashira H.、Frantzeskakis E.、Fortuna F.、Balicas L.、Santander-Syro A. F.、Manousakis E.、Baumbach R. E.
    • Journal Title

      Physical Review B

      Volume: 97 Issue: 16 Pages: 165112-165112

    • DOI

      10.1103/physrevb.97.165112

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Surface electronic structure of SmB 6 (111)2018

    • Author(s)
      Y. Ohtsubo, K. Hagiwara, C. Wang, R. Yukawa, K. Horiba, H. Kumigashira, W. Hirano, F. Iga, S. Kimura
    • Journal Title

      Physica B: Condensed Matter

      Volume: 536 Pages: 75-77

    • DOI

      10.1016/j.physb.2017.09.033

    • Related Report
      2017 Research-status Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Emergence of Quantum Critical Behavior in Metallic Quantum-Well States of Strongly Correlated Oxides2017

    • Author(s)
      Kobayashi Masaki、Yoshimatsu Kohei、Mitsuhashi Taichi、Kitamura Miho、Sakai Enju、Yukawa Ryu、Minohara Makoto、Fujimori Atsushi、Horiba Koji、Kumigashira Hiroshi
    • Journal Title

      Scientific Reports

      Volume: 7 Issue: 1 Pages: 16621-16621

    • DOI

      10.1038/s41598-017-16666-x

    • Related Report
      2017 Research-status Report
    • Peer Reviewed / Open Access
  • [Presentation] In-situ Angle-Resolved Photoemission Studies of the Quasi-Two-Dimensional Electron Liquid States Formed at Anatase TiO2 (001) Surface by K Adsorption2018

    • Author(s)
      R. Yukawa, M. Minohara, D. Shiga, M. Kitamura, T. Mitsuhashi, M. Kobayashi, K. Horiba, and H. Kumigashira
    • Organizer
      ACSIN-14 & ICSPM26
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] K吸着によるAnatase TiO2 (001)表面の2次元電子状態制御2018

    • Author(s)
      湯川龍、 簔原誠人、 志賀大亮、 北村未歩、 三橋太一、小林正起、 堀場弘司、 組頭広志
    • Organizer
      表面・界面スペクトロスコピー2018
    • Related Report
      2018 Annual Research Report
  • [Presentation] K吸着によるAnatase TiO2 (001)表面の2次元電子状態制御2018

    • Author(s)
      湯川龍、 簔原誠人、 志賀大亮、 北村未歩、 三橋太一、小林正起、 堀場弘司、 組頭広志
    • Organizer
      2017年度量子ビームサイエンスフェスタ
    • Related Report
      2017 Research-status Report
  • [Presentation] 光触媒作用をもつアナターゼ型TiO2表面に誘起される機能解析:電子状態と表面構造2018

    • Author(s)
      湯川龍, 簔原誠人, 志賀大亮, 北村未歩, 堀場弘司, 望月出海, 兵頭俊夫, 組頭広志
    • Organizer
      第3回 元素戦略<研究拠点形成型>・大型研究施設携シンポジウム
    • Related Report
      2017 Research-status Report
  • [Presentation] Two-dimensional electron liquid states at the K-adsorbed anatase-TiO2 (001) surface2017

    • Author(s)
      R. Yukawa, M. Minohara, D. Shiga, M. Kitamura, T. Mitsuhashi, M. Kobayashi, K. Horiba, and H. Kumigashira
    • Organizer
      International Workshop on Oxide Electronics (iWOE-24)
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research

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Published: 2017-04-28   Modified: 2020-03-30  

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