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Development of novel carbon dioxide separation membrane using nanosheets

Research Project

Project/Area Number 18H01835
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Review Section Basic Section 28030:Nanomaterials-related
Research InstitutionKumamoto University (2020)
National Institute of Advanced Industrial Science and Technology (2018-2019)

Principal Investigator

Hatakeyama Kazuto  熊本大学, 産業ナノマテリアル研究所, 助教 (30773965)

Co-Investigator(Kenkyū-buntansha) 木田 徹也  熊本大学, 大学院先端科学研究部(工), 教授 (70363421)
伊田 進太郎  熊本大学, 大学院先端科学研究部(工), 教授 (70404324)
伯田 幸也  国立研究開発法人産業技術総合研究所, 材料・化学領域, ラボチーム長 (30250707)
Project Period (FY) 2018-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2020)
Budget Amount *help
¥17,550,000 (Direct Cost: ¥13,500,000、Indirect Cost: ¥4,050,000)
Fiscal Year 2020: ¥3,640,000 (Direct Cost: ¥2,800,000、Indirect Cost: ¥840,000)
Fiscal Year 2019: ¥4,290,000 (Direct Cost: ¥3,300,000、Indirect Cost: ¥990,000)
Fiscal Year 2018: ¥9,620,000 (Direct Cost: ¥7,400,000、Indirect Cost: ¥2,220,000)
Keywordsナノシート / 二酸化炭素分離 / 二酸化炭素 / 酸化グラフェン / 膜分離 / 気体選択膜 / 二酸化炭素分離膜 / ガス分離膜
Outline of Final Research Achievements

Nanosheets have been introduced into various application fields due to their extreme two-dimensional structure and specific properties. In this study, we tried to develop a carbon dioxide selective membrane via a new separation mechanism by our techniques for controlling the nanosheet property and interlayer space. As a result, we succeeded in obtaining the selectivity of carbon dioxide opposite to the molecular size. It was suggested that the gas permeation through nanosheet film is driven by a anomalous mechanism different from the common-sense one because the selectivity didn’t depend on the surface state and layer spacing of the nanosheet thin film.

Academic Significance and Societal Importance of the Research Achievements

本研究により、ナノシートを用いた二酸化炭素分離膜の開発が進展した。ナノシートは極限に薄い「紙」であり、ナノシートから作製された分離膜は、従来の分離膜の性能を突破できる可能性を持つ。例えば本研究で得られた、分子のサイズに逆行した分離性のもその1つとみることができる。このように、本研究で得られた成果は、地球上の二酸化炭素削減に寄与し、自足可能な社会の発展に貢献できるものである。

Report

(4 results)
  • 2020 Annual Research Report   Final Research Report ( PDF )
  • 2019 Annual Research Report
  • 2018 Annual Research Report
  • Research Products

    (28 results)

All 2021 2020 2019 2018

All Journal Article (12 results) (of which Int'l Joint Research: 4 results,  Peer Reviewed: 12 results,  Open Access: 1 results) Presentation (11 results) (of which Int'l Joint Research: 6 results,  Invited: 1 results) Patent(Industrial Property Rights) (5 results)

  • [Journal Article] Oxygen reduction reaction activity of an iron phthalocyanine/graphene oxide nanocomposite2021

    • Author(s)
      Irisa Kenichiro、Hatakeyama Kazuto、Yoshimoto Soichiro、Koinuma Michio、Ida Shintaro
    • Journal Title

      RSC Advances

      Volume: 11 Issue: 26 Pages: 15927-15932

    • DOI

      10.1039/d1ra01001h

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Reversible hydrogenation and irreversible epoxidation induced by graphene oxide electrolysis2021

    • Author(s)
      Taniguchi Takaaki、Wong Kar Chun、Nurdiwijayanto Leanddas、Hatakeyama Kazuto、Awaya Keisuke、Ida Shintaro、Koinuma Michio、Ueda Shigenori、Osada Minoru、Yokoi Hiroyuki
    • Journal Title

      Carbon

      Volume: 177 Pages: 26-34

    • DOI

      10.1016/j.carbon.2021.02.057

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Electrochemical hydrogen production from humid air using cation-modified graphene oxide membranes2021

    • Author(s)
      Hamidah Nur Laila、Shintani Masataka、Ahmad Fauzi Aynul Sakinah、Kitamura Shota、Mission Elaine G.、Hatakeyama Kazuto、Sasaki Mitsuru、Quitain Armando T.、Kida Tetsuya
    • Journal Title

      Pure and Applied Chemistry

      Volume: 93 Issue: 1 Pages: 1-11

    • DOI

      10.1515/pac-2019-0807

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Slide-Ring Material/Highly Dispersed Graphene Oxide Composite with Mechanical Strength and Tunable Electrical Conduction as a Stretchable-Base Substrate2020

    • Author(s)
      Hatakeyama Kazuto、Ishikawa Yoshie、Kirihara Kazuhiro、Ito Tsuyohito、Mayumi Koichi、Ito Kohzo、Terashima Kazuo、Hakuta Yukiya、Shimizu Yoshiki
    • Journal Title

      ACS Applied Materials & Interfaces

      Volume: 12 Issue: 42 Pages: 47911-47920

    • DOI

      10.1021/acsami.0c12687

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Carbon-based potentiometric hydrogen sensor using a proton conducting graphene oxide membrane coupled with a WO3 sensing electrode2020

    • Author(s)
      Ahmad Fauzi Aynul Sakinah、Hamidah Nur Laila、Sato Shinya、Shintani Masataka、Putri Ghina Kifayah、Kitamura Shota、Hatakeyama Kazuto、Quitain Armando T.、Kida Tetsuya
    • Journal Title

      Sensors and Actuators B: Chemical

      Volume: 323 Pages: 128678-128678

    • DOI

      10.1016/j.snb.2020.128678

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Fabrication of layer-by-layer graphene oxide thin film on copper substrate by electrophoretic deposition2020

    • Author(s)
      Ye Nan、Ohnishi Satoka、Okada Mitsuhiro、Hatakeyama Kazuto、Seki Kazuhiko、Kubo Toshitaka、Shimizu Tetsuo
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 59 Issue: 12 Pages: 125001-125001

    • DOI

      10.35848/1347-4065/abc3a2

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Graphene Oxide Membranes with Cerium-Enhanced Proton Conductivity for Water Vapor Electrolysis2020

    • Author(s)
      Hamidah Nur Laila、Shintani Masataka、Ahmad Fauzi Aynul Sakinah、Putri Ghina Kifayah、Kitamura Shota、Hatakeyama Kazuto、Sasaki Mitsuru、Quitain Armando T.、Kida Tetsuya
    • Journal Title

      ACS Applied Nano Materials

      Volume: 3 Issue: 5 Pages: 4292-4304

    • DOI

      10.1021/acsanm.0c00439

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Movable cross-linked elastomer with aligned carbon nanotube/nanofiber as high thermally conductive tough flexible composite2020

    • Author(s)
      Goto Taku、Ito Tsuyohito、Mayumi Koichi、Maeda Rina、Shimizu Yoshiki、Hatakeyama Kazuto、Ito Kohzo、Hakuta Yukiya、Terashima Kazuo
    • Journal Title

      Composites Science and Technology

      Volume: 190 Pages: 108009-108009

    • DOI

      10.1016/j.compscitech.2020.108009

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] A simple ozone bubbling procedure for the preparation of graphene oxide2019

    • Author(s)
      Hatakeyama Kazuto、Hakuta Yukiya、Sugiyama Jun-ichi、Shimizu Yoshiki
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 58 Issue: SI Pages: SIIA05-SIIA05

    • DOI

      10.7567/1347-4065/ab1e3f

    • NAID

      210000156441

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] A Two-Step Method for Stable and Impurity-Free Graphene Oxide Dispersion in Various Organic Solvents without a Stabilizer or Chemical Modification2019

    • Author(s)
      Hatakeyama Kazuto、Koinuma Michio、Shimizu Yoshiki、Hakuta Yukiya
    • Journal Title

      Bulletin of the Chemical Society of Japan

      Volume: 92 Issue: 3 Pages: 511-520

    • DOI

      10.1246/bcsj.20180309

    • NAID

      130007613747

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Development of High Thermally Conductive Flexible Elastomer as a Composite Material of Slide-Ring Material and Plasma-Surface-Modified Boron Nitride Particles: Effect of Plasma-Surface Modification of Boron Nitride Particles2018

    • Author(s)
      Goto Taku、Iida Masaki、Tan Helen、Liu Chang、Mayumi Koichi、Maeda Rina、Kitahara Koichi、Hatakeyama Kazuto、Ito Tsuyohito、Shimizu Yoshiki、Yokoyama Hideaki、Kimura Kaoru、Ito Kohzo、Hakuta Yukiya、Terashima Kazuo
    • Journal Title

      Journal of the Japan Institute of Metals and Materials

      Volume: 82 Issue: 10 Pages: 403-407

    • DOI

      10.2320/jinstmet.JAW201809

    • NAID

      130007487536

    • ISSN
      0021-4876, 1880-6880, 2433-7501
    • Year and Date
      2018-10-01
    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Water Vapor Electrolysis with Proton-Conducting Graphene Oxide Nanosheets2018

    • Author(s)
      Tetsuya Kida, Yuta Kuwaki, Azumi Miyamoto, Nur Laila Hamidah, Kazuto Hatakeyama, Armando T. Quitain, Mitsuru Sasaki, and Atsushi Urakawa
    • Journal Title

      ACS Sustainable Chem. Eng.

      Volume: 6 Issue: 9 Pages: 11753-11758

    • DOI

      10.1021/acssuschemeng.8b01998

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Presentation] A Simple Ozone Treatment for Oxidizing Carbon Materials using Barrier Discharge2019

    • Author(s)
      畠山 一翔、伯田 幸也、 杉山 順一、清水 禎樹
    • Organizer
      10th International Workshop of Microplasma
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] オゾンバブリングによる酸化グラフェン作製技術の検討2019

    • Author(s)
      畠山 一翔、伯田 幸也、杉山 順一、清水 禎樹
    • Organizer
      第12回酸 化グラフェンシンポジウム
    • Related Report
      2019 Annual Research Report
  • [Presentation] 有機溶媒に対する高分散性酸化グラフェンの開発2019

    • Author(s)
      畠山 一翔、鯉沼陸央、清水 禎樹、伯田 幸也
    • Organizer
      第 46回炭素材料学会年会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 靭性、電気伝導性にすぐれた環動高分子/酸化グラフェン複合体の作製2019

    • Author(s)
      畠山 一翔、伯田 幸也、清水 禎樹、伊藤 剛仁、寺嶋和夫、伊藤耕三
    • Organizer
      グラフェン・酸化グラフェン合同シンポジウム
    • Related Report
      2019 Annual Research Report
  • [Presentation] Decoration of ZnO film with gold nanoparticles in open air by atmospheric-pressure micro-plasma jet and the photocatalytic properties of the decorated film2019

    • Author(s)
      清水 禎樹、畠山 一翔、伯田 幸也
    • Organizer
      10th International Workshop of Microplasma
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Surface-modifications of graphene nano-plates via plasma in liquid2019

    • Author(s)
      飯田 雅樹、後藤 拓、畠山 一翔、伊 藤 剛仁、清水 禎樹、伯田 幸也、寺嶋 和夫
    • Organizer
      XXXIV ICPIG & ICRP-10
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Direct deposition of plasmonic nanoparticles via sputtering performed in open air for easy manufacturing of plasmonic nanocomposite film2019

    • Author(s)
      清水 禎樹、畠山 一翔、伯田 幸也
    • Organizer
      2019 MRS Fall Meeting
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Preparation of Stable and Impurity-Free Graphene Oxide Dispersion in Various Organic Solvents2019

    • Author(s)
      Hatakeyama Kazuto、Koinuma Michio、Shimizu Yoshiki、Hakuta Yukiya
    • Organizer
      1 & 2D Materials International Conference and Exhibition
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 酸化グラフェンの特徴と実用化への取り組み2019

    • Author(s)
      畠山一翔
    • Organizer
      第1回 2D材料研究会
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] New Preparation Method for Graphene-like Carbon Material2018

    • Author(s)
      Hatakeyama Kazuto、Shimizu Yoshiki
    • Organizer
      ACSIN14 & ICSPM26
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 高安定な酸化グラフェン有機溶媒分散液の開発2018

    • Author(s)
      畠山一翔、鯉沼陸央、清水禎樹、伯田幸也
    • Organizer
      第11回酸化グラフェンシンポジウム
    • Related Report
      2018 Annual Research Report
  • [Patent(Industrial Property Rights)] コネクタ及びコネクタ対2020

    • Inventor(s)
      関和、久保、岡田、古賀、清水、畠山、葉、川合
    • Industrial Property Rights Holder
      国立研究開発法人産業技術総合研究所
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      2020-001060
    • Filing Date
      2020
    • Related Report
      2020 Annual Research Report
  • [Patent(Industrial Property Rights)] 導電性被覆が形成された金属材料2020

    • Inventor(s)
      関和彦、久保利隆、岡田光博、畠山一翔、古賀健司、清水哲夫、葉楠
    • Industrial Property Rights Holder
      国立研究開発法人産業技術総合研究所
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      2020-010602
    • Filing Date
      2020
    • Related Report
      2019 Annual Research Report
  • [Patent(Industrial Property Rights)] 強柔軟・高誘電性エラストマーとその製造方法2019

    • Inventor(s)
      伯田幸也、寺嶋和夫、後藤拓、清水禎樹、畠山一 翔、他4名
    • Industrial Property Rights Holder
      国立研究開発法人産業技術総合研究所
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      2019-165646
    • Filing Date
      2019
    • Related Report
      2019 Annual Research Report
  • [Patent(Industrial Property Rights)] 高放熱・高柔軟・高靭性ナノコンポジットとその製造方法2019

    • Inventor(s)
      伯田幸也、寺嶋和夫、清水禎樹、畠山一翔、他4名
    • Industrial Property Rights Holder
      国立研究開発法人産業技術総合研究所
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      2019-121160
    • Filing Date
      2019
    • Related Report
      2019 Annual Research Report
  • [Patent(Industrial Property Rights)] 様々な溶媒に対して高安定性を有する酸化グラフェン分散液とその製造技術2018

    • Inventor(s)
      畠山一翔、清水禎樹、伯田幸也
    • Industrial Property Rights Holder
      産業技術総合研究所
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      2018-177559
    • Filing Date
      2018
    • Related Report
      2018 Annual Research Report

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Published: 2018-04-23   Modified: 2022-01-27  

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