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Decomposition of odor trace images into elemental profiles with odor image sensor

Research Project

Project/Area Number 18H03782
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Review Section Medium-sized Section 21:Electrical and electronic engineering and related fields
Research InstitutionKyushu University

Principal Investigator

HAYASHI Kenshi  九州大学, システム情報科学研究院, 教授 (50202263)

Co-Investigator(Kenkyū-buntansha) 中野 幸二  九州大学, 工学研究院, 准教授 (10180324)
冨浦 洋一  九州大学, システム情報科学研究院, 教授 (10217523)
Project Period (FY) 2018-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2020)
Budget Amount *help
¥44,330,000 (Direct Cost: ¥34,100,000、Indirect Cost: ¥10,230,000)
Fiscal Year 2020: ¥9,490,000 (Direct Cost: ¥7,300,000、Indirect Cost: ¥2,190,000)
Fiscal Year 2019: ¥15,470,000 (Direct Cost: ¥11,900,000、Indirect Cost: ¥3,570,000)
Fiscal Year 2018: ¥19,370,000 (Direct Cost: ¥14,900,000、Indirect Cost: ¥4,470,000)
Keywords匂いイメージセンサ / 2次元化学センサ / 化学空間情報 / ビッグデータ / 機械学習 / プラズモニックガスセンサ / 蛍光色素 / 匂い分子ホスト分子 / プロファイル分解 / センサアレイ / ピクセル化匂いセンサ / 匂いセンサロボット / 可視化 / 匂いセンサ / 分子認識
Outline of Final Research Achievements

We have developed an odor image sensor that visualizes the flow and traces of odors. The odor image sensor is composed of a two-dimensional gas sensor device, and uses a localized plasmon resonance (LSPR) that converts chemical substance information into optical information. In addition, the sub-pixel structure was realized by maskless exposure fabrication methods, and an odor image sensor capable of odor identification was realized. In addition, we have developed a sensor that has a fluorescent dye-LSPR coupling as a response mechanism and can generate image big data by hyperspectral imaging, gas identification by machine learning, high-speed 2D calibration technology, and odor visualization image decomposition into element odor profiles have also been realized.

Academic Significance and Societal Importance of the Research Achievements

要素臭プロファイルへ分解することを匂いセンシングの定義として明確にした。匂いなどの化学物質空間の可視化技術は、新しい価値を持つ情報を生成が可能で、災害現場などでの人の発見、危険物などの漏洩ガス源の発見などに繋がる技術である。また、2次元ガスセンサは化学センサの実用化を阻む根本的な問題を解決できる。すわなち、高速なセンサ特性のキャリブレーション、ビッグデータの取得を通じたデータ駆動型科学の導入を可能とし、化学センサによるサイバーフィジカルシステムを実現できる。

Report

(4 results)
  • 2020 Annual Research Report   Final Research Report ( PDF )
  • 2019 Annual Research Report
  • 2018 Annual Research Report
  • Research Products

    (47 results)

All 2021 2020 2019 2018 Other

All Int'l Joint Research (2 results) Journal Article (14 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 13 results,  Open Access: 4 results) Presentation (28 results) (of which Int'l Joint Research: 3 results) Remarks (3 results)

  • [Int'l Joint Research] Southwest University(中国)

    • Related Report
      2020 Annual Research Report
  • [Int'l Joint Research] Southwest University(中国)

    • Related Report
      2019 Annual Research Report
  • [Journal Article] Direct Electron Transfer Reaction of Cytochrome c Immobilized on a Bare ITO Electrode2021

    • Author(s)
      Matsuda Naoki、Okabe Hirotaka、Nagamura Toshihiko、Nakano Koji
    • Journal Title

      Bulletin of the Chemical Society of Japan

      Volume: 94 Issue: 2 Pages: 433-439

    • DOI

      10.1246/bcsj.20200192

    • NAID

      130007995392

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] 2D LSPR gas sensor with Au/Ag core-shell structure coated by fluorescent dyes2020

    • Author(s)
      Kohei Semasa, Fumihiro Sassa, Kenshi Hayashi
    • Journal Title

      Proceedings of IEEE Sensors

      Volume: 2020-October Pages: 1-4

    • DOI

      10.1109/sensors47125.2020.9278828

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Covalent Hyperbranched Polymer Self-Assemblies of Three-Way Junction DNA for Single-Molecule Devices22020

    • Author(s)
      Koji Nakano, Takafumi Sawada, Yoshifumi Mori, Kohei Morita, Ryoichi Ishimatsu
    • Journal Title

      Langmuir

      Volume: 91 Issue: 34 Pages: 10166-10174

    • DOI

      10.1021/acs.langmuir.0c01621

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Enzyme-linked immunosorbent assay based on light absorption of enzymatically generated aniline oligomer: Flow injection analysis for 3-phenoxybenzoic acid with anti-3-phenoxybenzoic acid monoclonal antibody2020

    • Author(s)
      Ryoichi Ishimatsu, Shinichi Shimizu, Surat Hongsibsong, Koji Nakano, Chacriya Malasuk, Yuji Oki, Kinichi Morita
    • Journal Title

      Talanta

      Volume: 218 Pages: 121102-121102

    • DOI

      10.1016/j.talanta.2020.121102

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] 高校生を工学に惹きつけるための工学教育コンテンツ2020

    • Author(s)
      高松 洋,野口博司,安福規之,田中將己,中野幸二,柁川一弘,津守不二夫,田井 明
    • Journal Title

      工学教育

      Volume: 65 Pages: 64-67

    • NAID

      130007922444

    • Related Report
      2020 Annual Research Report
  • [Journal Article] Electrogenerated Chemiluminescence of Tris(dibenzoylmethane)phenanthroline Europium(III) as a Light Source: An Application for the Detection of PO<sub>4</sub><sup>3−</sup> Based on the Ion Associate Formation of Phosphomolybdic Acid and Malachite Green2019

    • Author(s)
      Eri KUNISAWA, Ryoichi ISHIMATSU, Koji NAKANO, and Toshihiko IMATO
    • Journal Title

      Analytical Sciences

      Volume: 35 Issue: 7 Pages: 799-802

    • DOI

      10.2116/analsci.19N003

    • NAID

      130007676957

    • ISSN
      0910-6340, 1348-2246
    • Year and Date
      2019-07-10
    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Probe gas sensing system based on reflected light detection from localized surface plasmon resonance2019

    • Author(s)
      Hao Guo, Takaaki Soeda, Zhongyuan Yang, Fumihiro Sassa, Kenshi Hayashi
    • Journal Title

      ISOEN 2019 - 18th International Symposium on Olfaction and Electronic Nose, Proceedings

      Volume: 19025031 Pages: 65-68

    • DOI

      10.1109/isoen.2019.8823157

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Invisible Odor Trace Tracking with LSPR based High Speed Gas Sensor Robot System2019

    • Author(s)
      Yasuhiro Kusuda, Zhongyuan Yang, Takaaki Soeda, Fumihiro Sassa, Kenshi Hayashi
    • Journal Title

      Proceedings of IEEE Sensors

      Volume: 2019-October Pages: 1-4

    • DOI

      10.1109/sensors43011.2019.8956599

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] 2D LSPR multi gas sensor array with 4-segmented subpixel using Au/Ag core shell structure2019

    • Author(s)
      Takaaki Soeda, Zhongyuan Yang, Fumihiro Sassa, Yoichi Tomiura, Kenshi Hayashi
    • Journal Title

      Proceedings of IEEE Sensors

      Volume: 2019-October Pages: 1-4

    • DOI

      10.1109/sensors43011.2019.8956635

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Efficient Electrogenerated Chemiluminescence of Pyrrolopyrrole Aza-BODIPYs in the Near-Infrared Region with Tripropylamine: Involving Formation of S2 and T2 StatesEfficient Electrogenerated Chemiluminescence of Pyrrolopyrrole Aza-BODIPYs in the Near-Infrared Region with Tripropylamine: Involving Formation of S2 and T2 States2019

    • Author(s)
      R. Ishimatsu, H. Shintaku, Y. Kage, M. Misaki, S. Shimizu, K. Nakano, H. Furuta, T. Imato
    • Journal Title

      J. Am. Chem. Soc.

      Volume: 141 Issue: 30 Pages: 11791-11795

    • DOI

      10.1021/jacs.9b05245

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Folding and Assembly of Vanilloid Receptor Secondary-Structure Peptide with Hexahistidine Linker at Nickel?Nitrilotriacetic Acid Monolayer for Capsaicin Recognition2019

    • Author(s)
      Nakano Koji、Horiuchi Jun、Hirata Shingo、Yamanaka Makoto、Himeno Toshiki、Ishimatsu Ryoichi
    • Journal Title

      Langmuir

      Volume: 35 Issue: 6 Pages: 2047-2054

    • DOI

      10.1021/acs.langmuir.8b03202

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Electrogenerated Chemiluminescence and Electronic States of Several Organometallic Eu(III) and Tb(III) Complexes: Effects of the Ligands2019

    • Author(s)
      R. Ishimatsu, E. Kunisawa, K. Nakano, C. Adachi, T. Imato
    • Journal Title

      ChemistrySelect

      Volume: 4 Issue: 9 Pages: 2815-2831

    • DOI

      10.1002/slct.201900595

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Totally synthetic microperoxidase-112018

    • Author(s)
      Tanabe Junichi、Nakano Koji、Hirata Ryutaro、Himeno Toshiki、Ishimatsu Ryoichi、Imato Toshihiko、Okabe Hirotaka、Matsuda Naoki
    • Journal Title

      Royal Society Open Science

      Volume: 5 Issue: 5 Pages: 172311-172311

    • DOI

      10.1098/rsos.172311

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Carbon Quantum Dots as Fluorescent Component in Peroxyoxalate Chemiluminescence for Hydrogen Peroxide Determination2018

    • Author(s)
      Nakano Koji、Honda Takayuki、Yamasaki Kanako、Tanaka Yoshiki、Taniguchi Keiichi、Ishimatsu Ryoichi、Imato Toshihiko
    • Journal Title

      Bulletin of the Chemical Society of Japan

      Volume: 91 Issue: 7 Pages: 1128-1130

    • DOI

      10.1246/bcsj.20180095

    • NAID

      130007404790

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Presentation] LSPR2次元センサの応答特性分布を利用した複数種のガス濃度分布の推定2021

    • Author(s)
      澤田 新,佐々 文洋,林 健司
    • Organizer
      令和3年電気学会全国大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 応答特性分布を持つ2次元センサによるガス濃度分布の推定2020

    • Author(s)
      澤田 新,佐々 文洋,林 健司
    • Organizer
      令和2年度応用物理学会九州支部学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 人探索に向けた色素修飾LSPRガスセンサロボットシステム2020

    • Author(s)
      楠田康弘、楊中元、佐々文洋、林健司
    • Organizer
      令和2年度応用物理学会九州支部学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 2D LSPR gas sensor with Au/Ag core-shell structure coated by fluorescent dyes2020

    • Author(s)
      Kohei Semasa, Fumihiro Sassa, Kenshi Hayashi
    • Organizer
      IEEE SENSORS 2020
    • Related Report
      2020 Annual Research Report
  • [Presentation] ペルオキシダーゼ活性を持つペプチド核酸モノリスハイブリッドーPNAzymeの合成と遺伝子センシング応用2020

    • Author(s)
      中野幸二,田邊潤壱,石松亮一
    • Organizer
      日本分析化学会第70年会
    • Related Report
      2020 Annual Research Report
  • [Presentation] ピレスロイド系殺虫剤の体内代謝物である3-phenoxybenzoic acid検出に向けたフローインジェクションELISA法の開発2020

    • Author(s)
      石松亮一,清水慎一,中野幸二
    • Organizer
      日本分析化学会第70年会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 分子鋳型ゾルゲルフィルタを用いたマルチLSPRガスセンサの開発2020

    • Author(s)
      清水晶太, 河野寛貴, 楠田康弘, 佐々文洋, 林 健司
    • Organizer
      MBE MICT
    • Related Report
      2019 Annual Research Report
  • [Presentation] Probe gas sensing system based on reflected light detection from localized surface plasmon resonance2019

    • Author(s)
      Hao Guo, Takaaki Soeda, Zhongyuan Yang, Fumihiro Sassa, Kenshi Hayashi
    • Organizer
      ISOEN2019
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Invisible Odor Trace Tracking with LSPR based High Speed Gas Sensor Robot System2019

    • Author(s)
      Yasuhiro Kusuda, Zhongyuan Yang, Takaaki Soeda, Fumihiro Sassa, Kenshi Hayashi
    • Organizer
      18th IEEE Sensors, SENSORS 2019
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 2D LSPR multi gas sensor array with 4-segmented subpixel using Au/Ag core shell structure2019

    • Author(s)
      Takaaki Soeda, Zhongyuan Yang, Fumihiro Sassa, Yoichi Tomiura, Kenshi Hayashi
    • Organizer
      18th IEEE Sensors, SENSORS 2019
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] ガス拡散を用いた二次元化学センサ応答の較正2019

    • Author(s)
      瀬政 康平, 佐々 文洋, 林 健司
    • Organizer
      第36回「センサ・マイクロマシンと応用システム」シンポジウム
    • Related Report
      2019 Annual Research Report
  • [Presentation] 人工バニロイドレセプターペプチドのHelix-Turn-Helixフォールディングを伴う自己組織化膜形成とカプサイシンセンシング2019

    • Author(s)
      中野幸二、堀内 潤、平田真吾、山中 真、姫野俊基、石松亮一
    • Organizer
      第79回分析化学討論会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 電極反応で生成する有機ラジカルイオンのミリ秒時間分解スペクトルの取得による均一電子移動速度反応の評価2019

    • Author(s)
      石松亮一、山口雄輝、中野幸二
    • Organizer
      第79回分析化学討論会
    • Related Report
      2019 Annual Research Report
  • [Presentation] バニロイドレセプターペプチドのメトキシクマリン修飾アラニン組込みおよびポリエチレングリコール化による新規ペプチドホスト分子の合成とバイオ分析応用2019

    • Author(s)
      中野幸二、堀内 潤、石松亮一
    • Organizer
      日本分析化学会第68年会
    • Related Report
      2019 Annual Research Report
  • [Presentation] ポリアニリン生成に基づくフロー吸光 ELISA 法の開発2019

    • Author(s)
      石松亮一、清水慎一、森田金市、中野幸二
    • Organizer
      日本分析化学会第68年会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 有機ラジカルイオンの吸収スペクトル測定に基づく高速検出法を用いた均一電子移動反応速度の解析2019

    • Author(s)
      山口雄輝、石松亮一、中野幸二
    • Organizer
      日本分析化学会第68年会
    • Related Report
      2019 Annual Research Report
  • [Presentation] ペプチド核酸とタンパク質酵素のワンポット合成化合物-PNAzymeの研究と核酸分析への応用2019

    • Author(s)
      瀬崎佑介、中野幸二、石松亮一
    • Organizer
      日本分析化学会第68年会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 多チャンネル匂いセンサの出力の匂い要素へのプロファイル分解2018

    • Author(s)
      鄭 暁帆,冨浦 洋一,林 健司
    • Organizer
      情報処理学会九州支部「若手の会セミナー」
    • Related Report
      2018 Annual Research Report
  • [Presentation] LSPR散乱光を利用したガス可視化撮像光学系2018

    • Author(s)
      副田 貴明,楊 中元,佐々 文洋,林 健司
    • Organizer
      平成30年度E部門総合研究会
    • Related Report
      2018 Annual Research Report
  • [Presentation] フォトパターニングコアシェル構造を持つ ピクセル化マルチガスセンサによる匂い撮像素子2018

    • Author(s)
      副田 貴明,楊 中元,佐々 文洋,林 健司
    • Organizer
      第35回「センサ・マイクロマシンと応用システム」シンポジウム
    • Related Report
      2018 Annual Research Report
  • [Presentation] イメージプロジェクタによる光誘起Au/Ag コアシェル構造LSPRマルチガスセンサの作製2018

    • Author(s)
      副田 貴明,楊 中元,佐々 文洋,林 健司
    • Organizer
      平成31年電気学会全国大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 高速LSPRガスセンサを搭載した匂い痕跡可視化ロボット2018

    • Author(s)
      楊 中元,佐々 文洋,林 健司
    • Organizer
      平成30年度E部門総合研究会
    • Related Report
      2018 Annual Research Report
  • [Presentation] バニロイド受容性電位チャネルタンパク質の分子認識ドメインの固相ペプチド合成とカプサイシンのバイオセンシング2018

    • Author(s)
      中野幸二、堀内潤、姫野俊基、石松亮一、今任稔彦
    • Organizer
      日本分析化学会 第78回分析化学討論会
    • Related Report
      2018 Annual Research Report
  • [Presentation] カーボン量子ドットの過シュウ酸エステル化学発光反応における蛍光体としての組み込みと過酸化水素分析への応用2018

    • Author(s)
      中野幸二、本田敬之、山﨑香菜子、田仲慶紀、谷口渓一、勝尾祐太、石松亮一、今任稔彦
    • Organizer
      日本分析化学会第67年会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 電極反応で生成する有機ラジカルイオンのミリ秒時間分解スペクトル2018

    • Author(s)
      石松亮一、古川佳栄、中野幸二、今任稔彦
    • Organizer
      日本分析化学会第67年会
    • Related Report
      2018 Annual Research Report
  • [Presentation] フロー電気化学発光デバイスの開発に向けたアルキルピレンの電気化学発光特性2018

    • Author(s)
      岡田拓也、石松亮一、中野幸二
    • Organizer
      日本分析化学会第67年会
    • Related Report
      2018 Annual Research Report
  • [Presentation] ジフェニルエーテル系除草剤の代謝物の定量分析を目的としたポリアニリン生成に基づくフロー吸光 ELISA 法の開発2018

    • Author(s)
      清水慎一、石松亮一、森田金市、中野幸二
    • Organizer
      日本分析化学会第67年会
    • Related Report
      2018 Annual Research Report
  • [Presentation] PNAzyme-ペプチド核酸とタンパク質触媒のワンポット固相合成による新規核酸分析試薬の研究2018

    • Author(s)
      瀬崎佑介、田邉潤壱、石松亮一、中野幸二
    • Organizer
      日本分析化学会第67年会
    • Related Report
      2018 Annual Research Report
  • [Remarks] 九州大学システム情報科学研究院有機電子デバイス研究室

    • URL

      https://o.ed.kyushu-u.ac.jp/

    • Related Report
      2020 Annual Research Report
  • [Remarks] 九州大学システム情報科学研究院有機デバイス研究室

    • URL

      https://o.ed.kyushu-u.ac.jp/

    • Related Report
      2019 Annual Research Report
  • [Remarks] 九州大学システム情報科学研究院有機デバイス研究室

    • URL

      http://o.ed.kyushu-u.ac.jp/

    • Related Report
      2018 Annual Research Report

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Published: 2018-04-23   Modified: 2022-01-27  

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