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Measurement of surface tension change at the liquid interface in contact with plasma

Research Project

Project/Area Number 18K03596
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Review Section Basic Section 14030:Applied plasma science-related
Research InstitutionHokkaido University

Principal Investigator

Shirai Naoki  北海道大学, 工学研究院, 准教授 (80552281)

Project Period (FY) 2018-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2020)
Budget Amount *help
¥4,160,000 (Direct Cost: ¥3,200,000、Indirect Cost: ¥960,000)
Fiscal Year 2020: ¥1,300,000 (Direct Cost: ¥1,000,000、Indirect Cost: ¥300,000)
Fiscal Year 2019: ¥1,300,000 (Direct Cost: ¥1,000,000、Indirect Cost: ¥300,000)
Fiscal Year 2018: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Keywords大気圧プラズマ / 表面張力 / 気液界面プラズマ / ラジカル
Outline of Final Research Achievements

The plasma-liquid interface is highly chemically reactive, however, the reactive species and radicals that contribute to the reaction are short-lived, and their measurement has not progressed much. In this study, we focused on the surface tension of the liquid and investigated how it is changed by plasma. Since the surface tension is determined by van der Waals forces and hydrogen bonds between molecules, reactive species and radicals transported by atmospheric pressure plasma may affect the change in surface tension. We first established a means of measuring the surface tension of water interacting with plasma and confirmed that the surface tension value of water increased when it was irradiated with plasma. It was confirmed that the surface tension value of water increased when it was irradiated with plasma. It was clarified that the cause of the increase may be the substances produced by OH radicals.

Academic Significance and Societal Importance of the Research Achievements

プラズマが液体と接した際に生じる界面現象について、表面張力というパラメータに着目したことは世界に先駆けた取り組みである。また実際にプラズマが接すると表面張力が増加するという予想に反した結果が得られたが、これはプラズマによるラジカル等の影響で分子の配向等が変化した可能性があり、今後この成果を発展させることでこれまで原理は十分に理解されずに応用事例が先行していたプラズマ液体界面の相互作用において、学術的理解を得ることが可能になる。

Report

(4 results)
  • 2020 Annual Research Report   Final Research Report ( PDF )
  • 2019 Research-status Report
  • 2018 Research-status Report
  • Research Products

    (19 results)

All 2021 2020 2019 2018

All Journal Article (3 results) (of which Peer Reviewed: 3 results) Presentation (16 results) (of which Int'l Joint Research: 3 results,  Invited: 5 results)

  • [Journal Article] Synthesis mechanism of cuprous oxide nanoparticles by atmospheric-pressure plasma electrolysis2021

    • Author(s)
      J. Liu, N. Shirai and K. Sasaki
    • Journal Title

      J. Phys. D: Appl. Phys.

      Volume: 54 Issue: 10 Pages: 105201-105201

    • DOI

      10.1088/1361-6463/abca2a

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Mechanism of droplet generation and optical emission of metal atoms in atmospheric-pressure dc glow discharge employing liquid cathode2020

    • Author(s)
      Shirai Naoki、Suga Goju、Sasaki Koichi
    • Journal Title

      Plasma Sources Science and Technology

      Volume: 29 Issue: 2 Pages: 025007-025007

    • DOI

      10.1088/1361-6595/ab6abc

    • NAID

      120006957266

    • Related Report
      2019 Research-status Report
    • Peer Reviewed
  • [Journal Article] Correlation between gas-phase OH density and intensity of luminol chemiluminescence in liquid interacting with atmospheric-pressure plasma2019

    • Author(s)
      Shirai Naoki、Suga Goju、Sasaki Koichi
    • Journal Title

      Journal of Physics D: Applied Physics

      Volume: 52 Issue: 39 Pages: 39LT02-39LT02

    • DOI

      10.1088/1361-6463/ab2ff2

    • NAID

      120006886031

    • Related Report
      2019 Research-status Report
    • Peer Reviewed
  • [Presentation] 誘導結合ヘリウムプラズマと相互作用する液体ガリウムからの液滴放出特性:液体温度の重要性2021

    • Author(s)
      濱名 優輝, 白井 直機, 佐々木 浩一
    • Organizer
      第38回プラズマプロセシング研究会
    • Related Report
      2020 Annual Research Report
  • [Presentation] プラズマ・液体相互作用における液相側現象理解のための実験技術の開発2021

    • Author(s)
      佐々木浩一、白井直機
    • Organizer
      第38回プラズマプロセシング研究会
    • Related Report
      2020 Annual Research Report
    • Invited
  • [Presentation] 大気圧気液界面プラズマによって誘起される気相ラジカルと液中化学ルミネッセンスの相関2021

    • Author(s)
      宮崎 俊明,白井 直機, 佐々木 浩一
    • Organizer
      プラズマ・核融合学会 北海道地区研究連絡会 第24回研究会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 誘導結合プラズマと相互作用する液体ガリウムからの液滴放出現象:ガスの溶存が与える液滴放出への影響2021

    • Author(s)
      濱名 優輝, 白井 直機, 佐々木 浩一
    • Organizer
      第68回応用物理学会春季学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 交差ガス流を用いた直流駆動大気圧プラズマにおけるOHラジカルの生成の最適化2020

    • Author(s)
      大和田 裕樹, 白井 直機, 佐々木 浩一
    • Organizer
      第67回応用物理学会春季学術講演会第81回応用物理学会秋季学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] レーザー誘起ブレイクダウン分光法及び液体電極直流グロー放電による乳製品に含まれるミネラル成分の簡易分析2020

    • Author(s)
      丸山 一沙, 白井 直機, 佐々木 浩一
    • Organizer
      第81回応用物理学会秋季学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 大気圧プラズマの空間アフターグローにより誘起される水の表面張力変化とOH密度分布との関連性2020

    • Author(s)
      金子 拓真, 白井 直機, 佐々木 浩一
    • Organizer
      第67回応用物理学会春季学術講演会
    • Related Report
      2019 Research-status Report
  • [Presentation] Measurement of surface tension at interface between water and spatial afterglow of an atmospheric-pressure helium plasma2019

    • Author(s)
      T. Kaneko, N. Shirai and K. Sasaki
    • Organizer
      XXXIV International Conference on Phenomena in Ionized Gases (XXXIV ICPIG) and the 10th International Conference on Reactive Plasmas (ICRP-10)
    • Related Report
      2019 Research-status Report
  • [Presentation] Visualization of OH radial in liquid induced by atmospheric pressure plasma by luminol chemiluminescence2019

    • Author(s)
      N. Shirai, G. Suga and K. Sasaki
    • Organizer
      XXXIV International Conference on Phenomena in Ionized Gases (XXXIV ICPIG) and the 10th International Conference on Reactive Plasmas (ICRP-10)
    • Related Report
      2019 Research-status Report
  • [Presentation] Correlation between OH density in gas and intensity of luminol chemiluminescence in liquid interacting with atmospheric-pressure DC glow discharge2019

    • Author(s)
      N. Shirai
    • Organizer
      72nd Annual Gaseous Electronics Conference
    • Related Report
      2019 Research-status Report
    • Invited
  • [Presentation] 大気圧プラズマの空間アフターグローにより励起される気液界面の表面張力の時間変化2019

    • Author(s)
      金子 拓真,白井 直機,佐々木 浩一
    • Organizer
      第80回応用物理学会秋季学術講演会
    • Related Report
      2019 Research-status Report
  • [Presentation] 大気圧プラズマの空間アフターグローと相互作用する気液界面における表面張力の計測2019

    • Author(s)
      金子拓真、白井直機、佐々木浩一
    • Organizer
      応用物理学会春季学術講演会
    • Related Report
      2018 Research-status Report
  • [Presentation] Plasma liquid interaction induced by atmospheric pressure glow discharge2019

    • Author(s)
      Naoki Shirai
    • Organizer
      11th EU-Joint Symposium on Plasma Processing
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] 大気圧プラズマの空間アフターグローと相互作用する 気液界面における表面張力の測定2019

    • Author(s)
      金子拓真、白井直機、佐々木浩一
    • Organizer
      プラズマ・核融合学会 北海道地区研究連絡会 第22回研究発表会
    • Related Report
      2018 Research-status Report
  • [Presentation] Investigation of plasma-liquid interaction of atmospheric pressure plasmas using a liquid electrode2018

    • Author(s)
      Naoki Shirai
    • Organizer
      Gordon Research Conference
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Luminol chemiluminescence for visualization of short-lived reactive species induced in atmospheric pressure DC glow discharge2018

    • Author(s)
      Naoki Shirai, Yutaka Matsuda, Koichi Sasaki
    • Organizer
      第28回日本MRS年次大会
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research / Invited

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Published: 2018-04-23   Modified: 2022-01-27  

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