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Elucidation of actual process of radiocesium ageing in soil by isotope ratio analysis

Research Project

Project/Area Number 18K18211
Research Category

Grant-in-Aid for Early-Career Scientists

Allocation TypeMulti-year Fund
Review Section Basic Section 64010:Environmental load and risk assessment-related
Research InstitutionNational Agriculture and Food Research Organization

Principal Investigator

Wakabayashi Shokichi  国立研究開発法人農業・食品産業技術総合研究機構, 東北農業研究センター, 主任研究員 (80707654)

Project Period (FY) 2018-04-01 – 2022-03-31
Project Status Completed (Fiscal Year 2021)
Budget Amount *help
¥4,160,000 (Direct Cost: ¥3,200,000、Indirect Cost: ¥960,000)
Fiscal Year 2021: ¥780,000 (Direct Cost: ¥600,000、Indirect Cost: ¥180,000)
Fiscal Year 2020: ¥780,000 (Direct Cost: ¥600,000、Indirect Cost: ¥180,000)
Fiscal Year 2019: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Fiscal Year 2018: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Keywords農地土壌 / 放射性セシウム / エイジング / 同位体比 / 交換性画分 / 土壌放射性セシウム / 粘土鉱物組成 / 水田と畑
Outline of Final Research Achievements

Radioactive cesium (137Cs) deposited in soil becomes fixed to the interlayer of micaceous minerals over time and becomes less leachable. This phenomenon is called as the "ageing" of soil 137Cs. This study investigated the process of the ageing after the accident at the Tokyo Electric Power Company's Fukushima Daiichi Nuclear Power Plant using a new analytical index (137Cs/133Cs ratio in exchangeable fraction). Analyzing the dynamics of the index in many farmlands, the progression rate of long-term ageing (the decline rate of 137Cs/133Cs ratio in exchangeable fraction) was evaluated as 0.04 /y on average and 0.07 /y at the maximum. Additionally, some analytical results indicated that there were differences in the ageing progress between upland fields and paddy fields, and that soil potassium fertility affected the behavior of 137Cs.

Academic Significance and Societal Importance of the Research Achievements

土壌中における放射性セシウムのエイジングは、農作物の汚染リスクが時間経過とともにどの程度低減するかを見積もる上で重要である。本研究で評価したエイジングの進行速度に、土壌中の放射性セシウム濃度の減少速度(放射性壊変や土壌からの溶脱による)を評価し加算することで、農作物の汚染リスク(ある条件下で栽培された農作物の放射性セシウム濃度)の経年変化を見積もることができる。農作物の放射性セシウム濃度が基準値を超過することを中長期にわたり防ぐ上で、汚染リスクが過去に比べてどの程度低下したかを見積もることは、今後の対策や調査の必要性・規模について議論するための判断材料となる。

Report

(5 results)
  • 2021 Annual Research Report   Final Research Report ( PDF )
  • 2020 Research-status Report
  • 2019 Research-status Report
  • 2018 Research-status Report
  • Research Products

    (4 results)

All 2020 2019 Other

All Journal Article (1 results) (of which Peer Reviewed: 1 results) Presentation (2 results) Remarks (1 results)

  • [Journal Article] Evaluation of 137Cs ageing by dynamics of 137Cs/133Cs ratio in Andosol paddy fields with/without potassium fertilizer application2020

    • Author(s)
      Shokichi Wakabayashi, Shigeru Takahashi, Hisaya Matsunami, Shioka Hamamatsu, Mayumi Hachinohe, Nobuharu Kihou, Noriko Yamaguchi
    • Journal Title

      Journal of Environemntal Radioactivity

      Volume: 218 Pages: 106252-106252

    • DOI

      10.1016/j.jenvrad.2020.106252

    • Related Report
      2019 Research-status Report
    • Peer Reviewed
  • [Presentation] 福島県内農地土壌における交換性137Csの経時変化とその要因2020

    • Author(s)
      若林正吉・藤村恵人・矢ヶ崎泰海
    • Organizer
      日本土壌肥料学会東北支部
    • Related Report
      2020 Research-status Report
  • [Presentation] 137Cs/133Cs比を用いた黒ボク土水田における放射性セシウムのエイジングの評価2019

    • Author(s)
      若林正吉、伊藤純雄、高橋 茂、松波寿弥、濱松潮香、八戸真弓、木方展治、山口紀子
    • Organizer
      日本ペドロジー学会
    • Related Report
      2019 Research-status Report
  • [Remarks] 同位体比分析により土壌中における137Csのエイジングの進行速度を評価できる

    • URL

      https://www.naro.go.jp/project/results/4th_laboratory/tarc/2020/tarc20_s18.html

    • Related Report
      2021 Annual Research Report

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Published: 2018-04-23   Modified: 2023-01-30  

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