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Ambient time-resolved x-ray spectroscopy to directly prove quantum effects on biological reactions

Research Project

Project/Area Number 18K19011
Research Category

Grant-in-Aid for Challenging Research (Exploratory)

Allocation TypeMulti-year Fund
Review Section Medium-sized Section 29:Applied condensed matter physics and related fields
Research InstitutionTohoku University

Principal Investigator

Fukidome Hirokazu  東北大学, 電気通信研究所, 准教授 (10342841)

Co-Investigator(Kenkyū-buntansha) 松田 巌  東京大学, 物性研究所, 准教授 (00343103)
Project Period (FY) 2018-06-29 – 2020-03-31
Project Status Completed (Fiscal Year 2019)
Budget Amount *help
¥6,240,000 (Direct Cost: ¥4,800,000、Indirect Cost: ¥1,440,000)
Fiscal Year 2019: ¥3,250,000 (Direct Cost: ¥2,500,000、Indirect Cost: ¥750,000)
Fiscal Year 2018: ¥2,990,000 (Direct Cost: ¥2,300,000、Indirect Cost: ¥690,000)
Keywordsグラフェン / 軟X線分光 / 時間分解 / 積層 / ねじれ / 光励起 / キャリア・ダイナミクス / 分子 / 軟X線 / X線分光 / 生体分子 / 量子ダイナミクス
Outline of Final Research Achievements

For the purpose of exploiting new field of molecular biology based on quantum theory, it is necessary to devlelop an ultrathin window material, graphene, for time-resolved soft x-ray spectroscopy under ambient pressure. During the research, we fortunately exploited a research deployment on carrier dynamics, such as an observation that photoexcited carrier density is modulated, depending on the layer of graphene.

Academic Significance and Societal Importance of the Research Achievements

本研究では、僅かにグラフェンの積層が摂動を受けただけで、層毎にグラフェン中の光励起キャリアの密度が大きく変調されるという初めての研究成果が得られた。このことは、グラフェンの窓材としての量子生物学への応用だけでなく、光デバイス応用においても重要な研究成果になると考えられる。

Report

(3 results)
  • 2019 Annual Research Report   Final Research Report ( PDF )
  • 2018 Research-status Report
  • Research Products

    (29 results)

All 2020 2019 2018 Other

All Int'l Joint Research (2 results) Journal Article (7 results) (of which Int'l Joint Research: 3 results,  Peer Reviewed: 7 results,  Open Access: 4 results) Presentation (16 results) (of which Int'l Joint Research: 6 results,  Invited: 13 results) Book (1 results) Remarks (3 results)

  • [Int'l Joint Research] Sungkyunkwan University(韓国)

    • Related Report
      2019 Annual Research Report
  • [Int'l Joint Research] Sungkyunkwan University(韓国)

    • Related Report
      2018 Research-status Report
  • [Journal Article] Direct Formation of Solution-based Al2O3 on Epitaxial Graphene Surface for Sensor Applications2019

    • Author(s)
      K.S. Kim, H. Fukidome, and M. Suemitsu
    • Journal Title

      Sensors and Materials

      Volume: 31 Issue: 7 Pages: 2291

    • DOI

      10.18494/SAM.2019.2317

    • ISSN
      0914-4935, 2435-0869
    • Year and Date
      2019-07-19
    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Modulation of Electronic States near Electrodes in Graphene Transistors Observed by Operando Photoelectron Nanospectroscopy2019

    • Author(s)
      H. Fukidome, K. Funakubo, N. Nagamura, K. Horiba, Y. Tateno, M. Oshima, and M. Suemitsu
    • Journal Title

      Sensors and Materials

      Volume: 31 Issue: 7 Pages: 2303

    • DOI

      10.18494/SAM.2019.2327

    • ISSN
      0914-4935, 2435-0869
    • Year and Date
      2019-07-19
    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Ultrafast Unbalanced Electron Distributions in Quasicrystalline 30° Twisted Bilayer Graphene2019

    • Author(s)
      Takeshi Suzuki*, Takushi Iimori, Sung Joon Ahn, Yuhao Zhao, Mari Watanabe, Jiadi Xu, Masami Fujisawa, Teruto Kanai, Nobuhisa Ishii, Jiro Itatani, Kento Suwa, Hirokazu Fukidome, Satoru Tanaka, Joung Real Ahn, Kozo Okazaki, Shik Shin, Fumio Komori*, Iwao Matsuda*
    • Journal Title

      ACS Nano

      Volume: 13 Issue: 10 Pages: 11981-11987

    • DOI

      10.1021/acsnano.9b06091

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Influence of interface dipole layers on the performance of graphene field effect transistors2019

    • Author(s)
      Nagamura Naoka、Fukidome Hirokazu、Nagashio Kosuke、Horiba Koji、Ide Takayuki、Funakubo Kazutoshi、Tashima Keiichiro、Toriumi Akira、Suemitsu Maki、Horn Karsten、Oshima Masaharu
    • Journal Title

      Carbon

      Volume: 152 Pages: 680-687

    • DOI

      10.1016/j.carbon.2019.06.038

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Interfacial carrier dynamics of graphene on SiC, traced by the full-range time-resolved core-level photoemission spectroscopy2018

    • Author(s)
      Someya T.、Fukidome H.、Endo N.、Takahashi K.、Yamamoto S.、Matsuda I.
    • Journal Title

      Applied Physics Letters

      Volume: 113 Issue: 5 Pages: 051601-051601

    • DOI

      10.1063/1.5043223

    • Related Report
      2018 Research-status Report
    • Peer Reviewed
  • [Journal Article] Enhancement of CO2 adsorption on oxygen-functionalized epitaxial graphene surface under near-ambient conditions2018

    • Author(s)
      Yamamoto Susumu、Takeuchi Kaori、Hamamoto Yuji、Liu Ro-Ya、Shiozawa Yuichiro、Koitaya Takanori、Someya Takashi、Tashima Keiichiro、Fukidome Hirokazu、Mukai Kozo、Yoshimoto Shinya、Suemitsu Maki、Morikawa Yoshitada、Yoshinobu Jun、Matsuda Iwao
    • Journal Title

      Physical Chemistry Chemical Physics

      Volume: 20 Issue: 29 Pages: 19532-19538

    • DOI

      10.1039/c8cp03251c

    • Related Report
      2018 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Operation Mechanism of GaN-based Transistors Elucidated by Element-Specific X-ray Nanospectroscopy2018

    • Author(s)
      Omika Keiichi、Tateno Yasunori、Kouchi Tsuyoshi、Komatani Tsutomu、Yaegassi Seiji、Yui Keiichi、Nakata Ken、Nagamura Naoka、Kotsugi Masato、Horiba Koji、Oshima Masaharu、Suemitsu Maki、Fukidome Hirokazu
    • Journal Title

      Scientific Reports

      Volume: 8 Issue: 1 Pages: 13268-13268

    • DOI

      10.1038/s41598-018-31485-4

    • Related Report
      2018 Research-status Report
    • Peer Reviewed / Open Access
  • [Presentation] Segmented soft X-ray undulator for on-demand polarization controls with the fastest switching2020

    • Author(s)
      松田巌
    • Organizer
      IMR+MAX IV
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 低温水素前処理されたC終端SiC基板上に成長させたグラフェンを用いたトランジスタの高速キャリア輸送特性の評価2020

    • Author(s)
      鴨川 貴優、佐々木 文憲、小濱 路生、渡邉 一世、吹留 博一
    • Organizer
      第67回応用物理学会春季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 軟X線分光法の基礎から学ぶ次世代放射光利用2019

    • Author(s)
      松田巌
    • Organizer
      日産アーク 技術セミナー 第5回放射光利用セミナー
    • Related Report
      2019 Annual Research Report
    • Invited
  • [Presentation] Chronology of photoexcited carriers in atomic layers2019

    • Author(s)
      松田巌
    • Organizer
      韓国真空学会 真空学会合同国際シンポジウム
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 先端軟X線レーザーで視る 原子層のダイナミクス2019

    • Author(s)
      松田巌
    • Organizer
      原子衝突学会 年会
    • Related Report
      2019 Annual Research Report
    • Invited
  • [Presentation] 表面超構造で制御する原子層の電子物性2019

    • Author(s)
      松田巌
    • Organizer
      日本物理学会 2019年秋季大会 シンポジウム「表面と原子層を融合した新しい2次元物質科学に向けて」
    • Related Report
      2019 Annual Research Report
    • Invited
  • [Presentation] Evolutions of the Dirac Fermions in Monatomic Layers2019

    • Author(s)
      松田巌
    • Organizer
      The 11th annual Recent Progress in Graphene and Two-dimensional Materials Research Conference (RPGR2019)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Upshifts in operando soft X-ray spectroscopies2019

    • Author(s)
      松田巌
    • Organizer
      Next Generation Synchrotron Radiation Workshop
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 集光軟 X 線で期待する 物質科学の展開2019

    • Author(s)
      松田巌
    • Organizer
      X線ナノ集光技術研究会
    • Related Report
      2019 Annual Research Report
    • Invited
  • [Presentation] Evolutions of the Dirac fermions in monatomic layers2019

    • Author(s)
      松田巌
    • Organizer
      Graphene Flagship EU-Japan 201
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] X-ray Optospintronics at SACLA2019

    • Author(s)
      松田巌
    • Organizer
      IRCCS The 3rd Joint International Symposium
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 酸化イットリウムを用いた高周波エピタキシャルグラフェン・トランジスタの高速キャリア輸送特性2019

    • Author(s)
      鴨川貴優、小濱路生、佐々木文憲、渡邊一世、吹留博一
    • Organizer
      第80回応用物理学会秋季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 酸化イットリウムを用いた高周波エピタキシャルグラフェン・トランジスタの高速キャリア輸送特性2019

    • Author(s)
      吹留博一、鴨川貴優、小濱路生、佐々木文憲、渡邊一世
    • Organizer
      2019年度日本表面真空学会学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 実デバイスの産学連携オペランド顕微軟X線分光分光と埋もれた界面の観察に向けて2019

    • Author(s)
      吹留博一
    • Organizer
      表面科学会 放射光表面科学研究部会・表面科学会 プローブ顕微鏡研究部会合同研究会
    • Related Report
      2018 Research-status Report
    • Invited
  • [Presentation] 動作しているデバイスの表面準位の時空間ダイナミクスの局所電界による制御2018

    • Author(s)
      吹留博一
    • Organizer
      第36回表面科学会講演大会
    • Related Report
      2018 Research-status Report
    • Invited
  • [Presentation] オペランドナノX線分光の利用を特徴とする産官学連携次世代デバイス研究開発2018

    • Author(s)
      吹留博一
    • Organizer
      東北大学多元物質科学研究所放射光産学連携準備室第1回ワークショップ
    • Related Report
      2018 Research-status Report
    • Invited
  • [Book] Monoatomic Two-dimensional Layers2018

    • Author(s)
      Hriokaz Fukidome(共著)
    • Total Pages
      232
    • Publisher
      Elsevier
    • ISBN
      9780128141618
    • Related Report
      2018 Research-status Report
  • [Remarks] 吹留研究室 研究紹介

    • URL

      http://www.fukidome.riec.tohoku.ac.jp/%e7%a0%94%e7%a9%b6%e7%b4%b9%e4%bb%8b/

    • Related Report
      2019 Annual Research Report
  • [Remarks] 松田巌研究室 研究

    • Related Report
      2019 Annual Research Report
  • [Remarks] https://imatsuda.issp.u-tokyo.ac.jp/research.html

    • Related Report
      2019 Annual Research Report

URL: 

Published: 2018-07-25   Modified: 2021-02-19  

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