Mixed-conductive membrane reactor as energy-saving catalysis process

• Project/Area Number: 19206084
• Research Category: Grant-in-Aid for Scientific Research (A)
• Allocation Type: Single-year Grants
• Section: 一般
• Research Field: Catalyst/Resource chemical process
• Research Institution: Kyushu University
• Principal Investigator: TERAOKA Yasutake Kyushu University, 大学院・総合理工学研究院, 教授 (70163904)
• Project Period (FY): 2007 – 2009
• Project Status: Completed (Fiscal Year 2009)
• Budget Amount: ¥48,100,000 (Direct Cost: ¥37,000,000、Indirect Cost: ¥11,100,000); Fiscal Year 2009: ¥4,810,000 (Direct Cost: ¥3,700,000、Indirect Cost: ¥1,110,000); Fiscal Year 2008: ¥23,010,000 (Direct Cost: ¥17,700,000、Indirect Cost: ¥5,310,000); Fiscal Year 2007: ¥20,280,000 (Direct Cost: ¥15,600,000、Indirect Cost: ¥4,680,000)
• Keywords: 触媒・化学プロセス / 混合導電体 / メンブレンリアクター / セラミックス

Research Abstract

Mixed-conductive membrane reactors (MBR) which can separate molecules have high potential as an energy-saving catalytic process. Main purpose of this study is to establish scientific technology for development of mixed-conductive MBR. Reaction mechanism has been proposed regarding methane partial oxidation MBR using oxygen permeable membrane. New type proton-electron mixed-conductive membranes which have the hetero structure with proton conductive and electron conductive phases have been proposed and the possible electrochemical permeation of hydrogen has been confirmed..

Research Products

• [Journal Article] Oxygen Separation by Mixed-Conductive Ceramics at Elevated Temperatures (2008)
  • Author(s): H. Kusaba, Y. Teraoka
  • Journal Title: Journal of the Technical Association of Refractories, Japan 28 Pages: 20-27
  • NAID: 10018634339
• [Presentation] Fe系ペロブスカイト型酸化物の酸素透過特性とメタン部分酸化用メンブレンリアクターへの応用 (2011)
  • Author(s): 草場一、穴井太郎、姜天龍、永長久寛、寺岡靖剛
  • Organizer: 第48回セラミックス基礎科学討論会
  • Place of Presentation: 沖縄
  • Year and Date: 2011-01-12
• [Presentation] Ba-Sr-Fe-Ga系ペロブスカイト型酸化物を用いたメタン部分酸化用メンブレンリアクターのメタン部分酸化特性 (2009)
  • Author(s): 穴井太郎、草場一、永長久寛、寺岡靖剛
  • Organizer: 石油学会九州・沖縄支部30周年記念沖縄大会
  • Place of Presentation: 沖縄
  • Year and Date: 2009-12-18
• [Presentation] Ba-Sr-Fe-Ga系ペロブスカイト型酸化物を用いたメタン部分酸化用メンブレンリアクターのメタン部分酸化特性 (2009)
  • Author(s): 穴井太郎、草場一、永長久寛、寺岡靖剛
  • Organizer: 石油学会 九州・沖縄支部30周年記念沖縄大会
  • Place of Presentation: 沖縄
  • Year and Date: 2009-12-18
• [Presentation] ペロブスカイト系酸素分離膜を用いたメタン部分酸化用メンブレンリアクター (2009)
  • Author(s): 草場一、穴井太郎、永長久寛、寺岡靖剛
  • Organizer: 第16回九州夏期セラミックス研究会
  • Place of Presentation: 宮崎
  • Year and Date: 2009-08-27
• [Presentation] Ba-Sr-Fe-Ga系ペロブスカイト型酸化物を用いたメタン部分酸化用メンブレンリアクター (2009)
  • Author(s): 穴井太郎、草場一、永長久寛、寺岡靖剛
  • Organizer: 第46回化学関連支部合同九州大会
  • Place of Presentation: 福岡
  • Year and Date: 2009-07-11
• [Presentation] Ba-Sr-Fe-Ga系ペロブスカイト型酸化物を用いたメタン部分酸化用メンブレンリアクター (2009)
  • Author(s): 穴井太郎、草場一、永長久寛、寺岡靖剛
  • Organizer: 第46回化学関連支部合同九州大会
  • Place of Presentation: 北九州
  • Year and Date: 2009-07-11
• [Presentation] Synthesis and Characterization of dual-phase proton-electron mixed conductors (2007)
  • Author(s): Y. Matsunaga, H. Kusaba, H. Einaga, Y. Teraoka
  • Organizer: 9th Cross Straits Symposium on Materials, Energy and Environmental Sciences
  • Place of Presentation: Korea
  • Year and Date: 2007-11-22
• [Presentation] Synthesis and Characterization of dual-phase proton-electron mixed conductors (2007)
  • Author(s): Y.Matsunaga, H.Kusaba, H.Einaga, Y.Teraoka
  • Organizer: 9th Cross Straits Symposium on Materials, Energy and Enviromental Sciences
  • Place of Presentation: Pohang(Korea)
  • Year and Date: 2007-11-22
• [Presentation] Catalytic research on partial oxidation of methane to synthesis gas (2007)
  • Author(s): E.S. Kim, CH.Y. Kang, H. Kusaba, H. Einaga, Y. Teraoka
  • Organizer: 9th Cross Straits Symposium on Materials, Energy and Environmental Sciences
  • Place of Presentation: Korea
  • Year and Date: 2007-11-21
• [Presentation] Catalytic research on partial oxidation of methane to synthesis gas (2007)
  • Author(s): E.S.Kim, CH.Y.Kang, H.Kusaba, H.Einaga, Y.Teraoka
  • Organizer: 9th Cross Straits Symposium on Materials, Energy and Enviromental Sciences
  • Place of Presentation: Pohang(Korea)
  • Year and Date: 2007-11-21
• [Presentation] Ba-Sr-Fe系ペロブスカイト型酸化物を用いたメタン部分酸化用メンブレンリアクター (2007)
  • Author(s): 姜天龍、草場一、永長久寛、寺岡靖剛
  • Organizer: 第100回触媒討論会
  • Place of Presentation: 札幌
  • Year and Date: 2007-09-19
• [Remarks] ホームページ
  • URL: http://www.mm.kyushu-u.ac.jp/lab_04/index.html