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Creation of 2D flat band materials through concerted experimental and theoretical studies

Research Project

Project/Area Number 20H00328
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Review Section Medium-sized Section 28:Nano/micro science and related fields
Research InstitutionJapan Advanced Institute of Science and Technology

Principal Investigator

Yamada-Takamura Yukiko  北陸先端科学技術大学院大学, 先端科学技術研究科, 教授 (90344720)

Co-Investigator(Kenkyū-buntansha) 吉田 靖雄  金沢大学, 数物科学系, 准教授 (10589790)
深谷 有喜  国立研究開発法人日本原子力研究開発機構, 原子力科学研究部門 原子力科学研究所 先端基礎研究センター, 研究主幹 (40370465)
尾崎 泰助  東京大学, 物性研究所, 教授 (70356723)
Project Period (FY) 2020-04-01 – 2024-03-31
Project Status Completed (Fiscal Year 2023)
Budget Amount *help
¥44,330,000 (Direct Cost: ¥34,100,000、Indirect Cost: ¥10,230,000)
Fiscal Year 2023: ¥11,440,000 (Direct Cost: ¥8,800,000、Indirect Cost: ¥2,640,000)
Fiscal Year 2022: ¥11,440,000 (Direct Cost: ¥8,800,000、Indirect Cost: ¥2,640,000)
Fiscal Year 2021: ¥11,440,000 (Direct Cost: ¥8,800,000、Indirect Cost: ¥2,640,000)
Fiscal Year 2020: ¥10,010,000 (Direct Cost: ¥7,700,000、Indirect Cost: ¥2,310,000)
Keywords二次元材料 / フラットバンド / 走査プローブ顕微鏡 / 全反射高速陽電子回折 / 第一原理電子状態計算 / 角度分解光電子分光 / 薄膜 / エピタキシー / 超薄膜
Outline of Research at the Start

電子が材料中で質量ゼロの相対論的粒子の様に振る舞うとみなせる電子状態を有するグラフェンやトポロジカル絶縁体が注目される一方で,その対極にある平坦(フラット)な電子状態をもつ材料「フラットバンドマテリアル」の探索が始まった.本研究課題では,新しいフラットバンド材料として期待される二次元格子群の微細構造制御と,それに付随する電子状態変化の解析に実験と理論計算の両面から協奏的に取り組む.

Outline of Final Research Achievements

Graphene, a honeycomb lattice of carbon atoms, which have linearly dispersing electronic bands resulting in high-mobility carriers mimicking massless relativistic particles attracts huge interests since its discovery in 2004. On the other hand, materials having dispersionless flat bands are also attracting interests since flat band can contribute to ferromagnetism or superconductivity. Hypothetical, two-dimensional (2D) kagome lattice is long known to have both linearly dispersing electronic bands and a flat band through theoretical studies, but experimental studies are scarce since it is difficult to find a kagome lattice in a real crystal. In this work, one of the new 2D flat band materials which has biatomic thickness suggested by our theoretical study was realized, and its electronic structure was experimentally characterized. Our work expands the crystal structures candidates to be considered, which will contribute to the exploration of new flat band materials.

Academic Significance and Societal Importance of the Research Achievements

仮想的で厚みのない二次元格子のバンド構造にフラットバンドが現れることは、従来の理論研究の結果から知られていた。本研究では、新しく提案された二原子分に相当する厚みのあるフラットバンドが発現する二次元結晶構造を実現し、その構造と電子状態の関係、低温における構造変化などを明らかにした。この研究を通じて、二次元フラットバンドマテリアルの候補となる結晶構造が増加した上に、それらには、厚み方向の原子間距離などにより電子状態制御が可能となるなど従来の仮想的二次元格子にはない性質があるため、今後の発展が期待できる。

Report

(6 results)
  • 2023 Annual Research Report   Final Research Report ( PDF )
  • 2022 Annual Research Report
  • 2021 Annual Research Report
  • 2020 Comments on the Screening Results   Annual Research Report
  • Research Products

    (33 results)

All 2024 2023 2022 2021 2020 Other

All Int'l Joint Research (4 results) Journal Article (3 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 2 results,  Open Access: 3 results) Presentation (25 results) (of which Int'l Joint Research: 13 results,  Invited: 21 results) Remarks (1 results)

  • [Int'l Joint Research] Tamkang University, Taiwan(その他の国・地域)

    • Related Report
      2023 Annual Research Report
  • [Int'l Joint Research] Tamkang University, Taiwan(その他の国・地域)

    • Related Report
      2022 Annual Research Report
  • [Int'l Joint Research] Tamkang University, Taiwan(その他の国・地域)

    • Related Report
      2021 Annual Research Report
  • [Int'l Joint Research] Tamkang University, Taiwan(その他の国・地域)

    • Related Report
      2020 Annual Research Report
  • [Journal Article] Methods for constructing parameter-dependent flat-band lattices2021

    • Author(s)
      Toshitaka Ogata, Mitsuaki Kawamura, and Taisuke Ozaki
    • Journal Title

      Physical Review B

      Volume: 103 Issue: 20

    • DOI

      10.1103/physrevb.103.205119

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] ZrB2(0001)薄膜表面上の二次元Ge二重三角格子2021

    • Author(s)
      深谷有喜, 吉信淳, アントワーヌ・フロランス, 高村(山田)由起子
    • Journal Title

      PHOTON FACTORY NEWS

      Volume: 39 Pages: 24-27

    • Related Report
      2021 Annual Research Report
    • Open Access
  • [Journal Article] Emergence of nearly flat bands through a kagome lattice embedded in an epitaxial two-dimensional Ge layer with a bitriangular structure2020

    • Author(s)
      A. Fleurence, C.-C. Lee, R. Friedlein, Y. Fukaya, S. Yoshimoto, K. Mukai, H. Yamane, N. Kosugi, J. Yoshinobu, T. Ozaki, and Y. Yamada-Takamura
    • Journal Title

      Physical Review B

      Volume: 102 Issue: 20

    • DOI

      10.1103/physrevb.102.201102

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Presentation] 表面科学的手法によるエピタキシャル二次元材料の構造・電子状態評価2024

    • Author(s)
      高村(山田) 由起子
    • Organizer
      応用物理学会薄膜・表面物理分科会Controlled growth and characterization研究会
    • Related Report
      2023 Annual Research Report
    • Invited
  • [Presentation] Surface Structure Analysis with Electrons and Positrons2024

    • Author(s)
      Y. Fukaya
    • Organizer
      日本物理学会2024年春季大会
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Ge二重三角格子の電荷密度波相2024

    • Author(s)
      高村(山田) 由起子
    • Organizer
      金沢物性科学研究会 Condmat Kanazawa 2024
    • Related Report
      2023 Annual Research Report
    • Invited
  • [Presentation] Absolute binding energies of electrons in condensed matters2024

    • Author(s)
      T. Ozaki
    • Organizer
      Second Workshop on Fundamentals in density functional theory (DFT2024)
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Novel 2D Materials Beyond Graphene Stabilized on Substrates2024

    • Author(s)
      Yukiko Yamada-Takamura
    • Organizer
      JAIST International Symposium on Nano-Materials for Novel Devices 2023 (JAIST-NMND2023)
    • Related Report
      2023 Annual Research Report
    • Invited
  • [Presentation] Research on Ultrathin Sn Films Grown on InSb(111)A for the Growth of Stanene2024

    • Author(s)
      Takato Yokoo, Yuki Nishita, Antoine Fleurence, Yukiko Yamada-Takamura
    • Organizer
      JAIST International Symposium on Nano-Materials for Novel Devices 2023 (JAIST-NMND2023)
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Structure determination of novel 2D materials2023

    • Author(s)
      Yukiko Yamada-Takamura
    • Organizer
      Symposia of the 30th Anniversary of the Advanced Science Research Center, Japan Atomic Energy Agency
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Structure determination of 2D materials using positron beam2023

    • Author(s)
      Y. Fukaya
    • Organizer
      Annual Meeting of the Japan Society of Vacuum and Surface Science 2023 (JVSS 2023)
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Closest Wannier functions to a given set of localized orbitals2023

    • Author(s)
      T. Ozaki
    • Organizer
      The IOP-FHI workshop on the frontiers of electronic-structure theory and materials genomics
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 全反射高速陽電子回折による最表面構造研究2023

    • Author(s)
      深谷有喜
    • Organizer
      第84回応用物理学会秋季学術講演会
    • Related Report
      2023 Annual Research Report
    • Invited
  • [Presentation] Search for Stanene: Ultrathin Sn Films Grown on InSb(111)A2023

    • Author(s)
      Takato Yokoo, Yuki Nishita, Antoine Fleurence, Yukiko Yamada-Takamura
    • Organizer
      31st International Colloquium on Scanning Probe Microscopy (ICSPM31)
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 陽電子ビームを用いた表面・二次元物質の構造決定2023

    • Author(s)
      深谷有喜
    • Organizer
      日本物理学会2023年春季大会
    • Related Report
      2022 Annual Research Report
    • Invited
  • [Presentation] 表面構造研究における実験と計算の協奏2023

    • Author(s)
      尾崎泰助
    • Organizer
      Kyutech物性グループセミナー, 九州工業大学戸畑キャンパス
    • Related Report
      2022 Annual Research Report
    • Invited
  • [Presentation] Emergence of charge density waves in a germanium two-dimensional flatband material2022

    • Author(s)
      Antoine Fleurence, Chi-Cheng Lee, Rainer Friedlein, Yuki Fukaya, Howon Kim, Yukio Hasegawa, Hiroyuki Yamane, Nobuhiro Kosugi, Taisuke Ozaki, and Yukiko Yamada-Takamura
    • Organizer
      The 22nd International Vacuum Congress (IVC-22)
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Structure analysis of 2D materials by total-reflection high-energy positron diffraction (TRHEPD)2022

    • Author(s)
      Y. Fukaya
    • Organizer
      14th International Symposium on Atomic Level Characterizations for New Materials and Devices '22 (ALC '22)
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Novel two-dimensional materials stabilized on substrates2022

    • Author(s)
      Yukiko Yamada-Takamura
    • Organizer
      9th International Workshop on 2D Materials, A3 Foresight Program
    • Related Report
      2021 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Towards experimental realization of a new 2D flat band material2021

    • Author(s)
      Yukiko Yamada-Takamura
    • Organizer
      E-Workshop for Skill Development on Energetic Beam Technology: From Materials Engineering to Diagnostics
    • Related Report
      2021 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 実験と計算の協奏による新奇二次元材料の創成2021

    • Author(s)
      高村(山田) 由起子
    • Organizer
      ISSP WOMEN'S WEEK 2021
    • Related Report
      2021 Annual Research Report
    • Invited
  • [Presentation] Novel two-dimensional materials stabilized on substrates2021

    • Author(s)
      Yukiko Yamada-Takamura
    • Organizer
      第61回 フラーレン・ナノチューブ・グラフェン総合シンポジウム
    • Related Report
      2021 Annual Research Report
    • Invited
  • [Presentation] Theory of core-level photoelectron spectroscopy2021

    • Author(s)
      Taisuke Ozaki
    • Organizer
      The 10th Workshop on Advanced Spectroscopy of Organic Materials for Electronic Applications (ASOMEA-X)
    • Related Report
      2021 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 基板上二次元材料の原子レベル構造制御2021

    • Author(s)
      高村(山田) 由起子
    • Organizer
      (公社)日本表面真空学会 東日本合同セミナー 表面・薄膜分析シリーズ Vol.7 先端的試料作製技術-原子層物質-
    • Related Report
      2021 Annual Research Report
    • Invited
  • [Presentation] 全反射高速陽電子回折による二次元フラットバンドマテリアルの構造特定2021

    • Author(s)
      高村(山田) 由起子, アントワーヌ・フロランス
    • Organizer
      低速陽電子実験施設研究会
    • Related Report
      2020 Annual Research Report
    • Invited
  • [Presentation] 放射光による IV 族二次元材料の構造・電子状態解析2021

    • Author(s)
      高村(山田) 由起子
    • Organizer
      NANOSPEC 2021 SPring-8ユーザー協同体顕微ナノ材料科学研究会日本表面真空学会放射光表面科学研究部会プローブ顕微鏡研究部会合同シンポジウム
    • Related Report
      2020 Annual Research Report
    • Invited
  • [Presentation] 内殻光電子分光(XPS)における絶対束縛エネルギーの第一原理計算2021

    • Author(s)
      尾崎泰助
    • Organizer
      NANOSPEC 2021 SPring-8ユーザー協同体顕微ナノ材料科学研究会 日本表面真空学会放射光表面科学研究部会プローブ顕微鏡研究部会合同シンポジウム
    • Related Report
      2020 Annual Research Report
    • Invited
  • [Presentation] Atomic configuration of two-dimensional Ge bitriangular structure2021

    • Author(s)
      Y. Fukaya, C.-C. Lee, A. Fleurence, Y. Hasegawa, T. Ozaki, and Y. Yamada-Takamura
    • Organizer
      The 9th International Symposium on Surface Science (ISSS-9)
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Remarks] 研究内容の英文プレスリリース

    • URL

      https://www.eurekalert.org/news-releases/781149

    • Related Report
      2020 Annual Research Report

URL: 

Published: 2020-04-28   Modified: 2025-01-30  

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