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Feedstock recycling of organic and inorganic materials from plastic-metal composites

Research Project

Project/Area Number 21241018
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field Environmental technology/Environmental materials
Research InstitutionTohoku University

Principal Investigator

YOSHIOKA Toshiaki  東北大学, 大学院・環境科学研究科, 教授 (30241532)

Co-Investigator(Kenkyū-buntansha) KAMEDA Tomohito  東北大学, 大学院工学研究科, 准教授 (60333895)
GRAUSE Guido  東北大学, 大学院環境科学研究科, 助教 (60570017)
Project Period (FY) 2009 – 2012
Project Status Completed (Fiscal Year 2012)
Budget Amount *help
¥45,890,000 (Direct Cost: ¥35,300,000、Indirect Cost: ¥10,590,000)
Fiscal Year 2012: ¥9,490,000 (Direct Cost: ¥7,300,000、Indirect Cost: ¥2,190,000)
Fiscal Year 2011: ¥12,350,000 (Direct Cost: ¥9,500,000、Indirect Cost: ¥2,850,000)
Fiscal Year 2010: ¥12,610,000 (Direct Cost: ¥9,700,000、Indirect Cost: ¥2,910,000)
Fiscal Year 2009: ¥11,440,000 (Direct Cost: ¥8,800,000、Indirect Cost: ¥2,640,000)
Keywordsリサイクル / フィードストック / 複合材料 / 無機 / 有機原料 / ポリエチレンテレフタレート / 無機・有機原料
Research Abstract

Plastics such as PET, PC and plastic-metal composites were thermally decomposed using fixed-bed and fluidized-bed reactors, which showed that it is possible to recover organic and inorganic materials simultaneously.

Report

(5 results)
  • 2012 Annual Research Report   Final Research Report ( PDF )
  • 2011 Annual Research Report
  • 2010 Annual Research Report
  • 2009 Annual Research Report
  • Research Products

    (50 results)

All 2013 2012 2011 2010 2009 Other

All Journal Article (14 results) (of which Peer Reviewed: 14 results) Presentation (28 results) Book (3 results) Remarks (5 results)

  • [Journal Article] Novel Approach for Determining the Proportions of Pyrolysis and Hydrolysis in the Degradation of Poly(ethylene terephthalate) in 18O-Labeled Steam2013

    • Author(s)
      Shogo Kumagai, Yuto Morohoshi, Guido Grause, Tomohito Kameda, Toshiaki Yoshioka
    • Journal Title

      Chemistry Letters

      Volume: 42 Pages: 212-214

    • NAID

      10031155755

    • Related Report
      2012 Annual Research Report 2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Recovery of glass fibers from glass fiber reinforced plastics by pyrolysis2013

    • Author(s)
      Guido Grause, Tomoyuki Mochizuki, Tomohito Kameda, Toshiaki Yoshioka
    • Journal Title

      Journal of Material Cycles and Waste Management

      Volume: 15 Issue: 2 Pages: 122-128

    • DOI

      10.1007/s10163-012-0101-x

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Feedstock recycling of waste polymeric material2011

    • Author(s)
      Guido Grause, Alfons Buekens, Yusaku Sakata, Akitsugu Okuwaki, Toshiaki Yoshioka
    • Journal Title

      Journal of Material Cycles and Waste Management

      Volume: 13 Pages: 265-282

    • Related Report
      2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Pyrolysis of Mixed Plastics in the Fluidized Bed of Hard Burnt Lime2011

    • Author(s)
      Guido Grause, Shotaro Matsumoto, Tomohito Kameda, Toshiaki Yoshioka
    • Journal Title

      Industrial & Engineering Chemistry Research

      Volume: 50 Pages: 5459-5466

    • Related Report
      2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Hydrolytic Degradation of Poly(ethylene terephthalate) in a Pyrolytic Two Step Process in Order to Obtain Benzene Rich Oil2011

    • Author(s)
      Guido Grause, Tomohiko Handa, Tomohito Kameda, Tadaaki Mizoguchi, Toshiaki Yoshioka
    • Journal Title

      Journal of Applied Polymer Science

      Volume: 120 Pages: 3687-3694

    • Related Report
      2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Effect of Temperature Management on the Hydrolytic Degradation of PET in a Calcium Oxide filled tube reactor2011

    • Author(s)
      Guido Grause, Tomohiko Handa, Tomohito Kameda, Tadaaki Mizoguchi, Toshiaki Yoshioka
    • Journal Title

      Chemical Engineering Journal

      Volume: 166 Pages: 523-528

    • Related Report
      2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Improvement of the Benzene Yield During Pyrolysis of Terephthalic Acid Using a CaO Fixed-bed Reactor2011

    • Author(s)
      Shogo Kumagai, Guido Grause, Tomohito Kameda, Tatsuo Takano, Hideki Horiuchi, Toshiaki Yoshioka
    • Journal Title

      Industrial & Engineering Chemistry Research

      Volume: 50 Pages: 6594-6600

    • Related Report
      2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Improvement of the Benzene Yield During Pyrolysis of Terephthalic Acid Using a CaO Fised-Bed Reactor2011

    • Author(s)
      Shogo Kumagai, Guido Grause, Tomohito Kameda, Tatsuo Takano, Hideki Horiuchi, Toshiaki Yoshioka
    • Journal Title

      Industrial & Engineering Chemistry Research

      Volume: 50 Pages: 6594-6600

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Decomposition of Gaseous Terephthalic Acid in the Presence of CaO2011

    • Author(s)
      Shogo Kumagai, Guido Grause, Tomohito Kameda, Tatsuo Takano, Hideki Horiuchi, Toshiaki Yoshioka
    • Journal Title

      Industrial & Engineering Chemistry Research

      Volume: 50 Pages: 1831-1836

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] High Value Products from the Catalytic Hydrolysis of Polycarbonate Waste2010

    • Author(s)
      Guido Grause, Norihiro Tsukada, William J. Hall, Tomohito Kameda, Paul T. Williams, Toshiaki Yoshioka
    • Journal Title

      Polymer Journal

      Volume: 42 Pages: 438-442

    • NAID

      10026365517

    • Related Report
      2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] High Value Products from the Catalytic Hydrolysis of Polycarbonate Waste2010

    • Author(s)
      Guido Grause, Norihiro Tsukada, William J.Hall, Tomohito Kameda, Paul T.Williams, Toshiaki Yoshioka
    • Journal Title

      Polymer Journal (印刷中)

    • NAID

      10026365517

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Pyrolytic hydrolysis of polycarbonate in the presence of earth-alkali oxides and hydroxides2009

    • Author(s)
      Guido Grause, Katsuya Sugawara, Tadaaki Mizoguchi, Toshiaki Yoshioka
    • Journal Title

      Polymer Degradation and Stability

      Volume: 94 Pages: 1119-1124

    • Related Report
      2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Pyrolytic hydrolysis of polycarbonate in the presence of earth-alkali oxides and hydroxides2009

    • Author(s)
      Guido Grouse, Katsuya Sugawara, Tadaaki Mizoguchi, Toshiaki Yoshioka
    • Journal Title

      Polymer Degradation and Stability 94

      Pages: 1104-1108

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Pyrolysis of mixed plastics in the fluidized bed using hard burnt lime as bed material2009

    • Author(s)
      Shotaro Matsumoto, Guido Grause, Tomohito Kameda, Toshiaki Yoshioka
    • Journal Title

      Proc.The 5th International Symposium on Feedstock and Mechanical Recycling of Polymeric Materials(ISFR2009)

      Pages: 47-51

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Presentation] Feedstock Recycling of Organic and Inorganic Materials by Thermal Decomposition of Metal-Containing Plastics2013

    • Author(s)
      Shogo Kumagai, Guido Grause, Tomohito Kameda, Toshiaki Yoshioka
    • Organizer
      The 12th Expert Meeting on Solid Waste Management in Asia and Pacific Islands (12th SWAPI)
    • Place of Presentation
      Tokyo, Japan
    • Year and Date
      2013-02-27
    • Related Report
      2012 Final Research Report
  • [Presentation] Recovery of Organic and Inorganic Materials by Thermal Decomposition of Metal-Containing Poly(ethylene terephthalate)2012

    • Author(s)
      Shogo Kumagai, Guido Grause, Tomohito Kameda, Toshiaki Yoshioka
    • Organizer
      3rd & 4th International Symposium of Environmental Leader
    • Place of Presentation
      Xi'an and Shanghai, China
    • Year and Date
      2012-11-12
    • Related Report
      2012 Final Research Report
  • [Presentation] Kinetic Investigation of Pyrolysis and Hydrolysis of Poly(ethylene terephthalate)2012

    • Author(s)
      Guido Grause, Yuto Morohoshi, Shogo Kumagai, Tomohito Kameda, Toshiaki Yoshioka
    • Organizer
      19th International Symposium on Analytical and Applied Pyrolysis
    • Place of Presentation
      Linz, Austria
    • Year and Date
      2012-05-24
    • Related Report
      2012 Final Research Report
  • [Presentation] 生石灰を用いたテレフタル酸の熱分解によるベンゼン生成機構の検討2012

    • Author(s)
      熊谷将吾, Grause Guido, 亀田知人, 吉岡敏明
    • Organizer
      日本化学会第92春季年会
    • Place of Presentation
      慶應義塾大学(神奈川県)
    • Year and Date
      2012-03-28
    • Related Report
      2011 Annual Research Report
  • [Presentation] Recovery of Organic and Inorganic Materials by Thermal Decomposition of Metal-Containing Poly(ethylene terephthalate)2012

    • Author(s)
      Shogo Kumagai, Guido Grause, Tomohito Kameda, Toshiaki Yoshioka
    • Organizer
      3rd & 4th International Symposium of Environmental Leader
    • Place of Presentation
      Xi' an, Shanghai (China)
    • Related Report
      2012 Annual Research Report
  • [Presentation] Feedstock Recycling of Organic and Inorganic Materials from Solid Waste2011

    • Author(s)
      Shogo Kumagai, Guido Grause, Tomohito Kameda, Toshiaki Yoshioka
    • Organizer
      The 2nd International Symposium of Environmental Leader
    • Place of Presentation
      Ho Chi Minh, Viet Nam
    • Year and Date
      2011-12-15
    • Related Report
      2012 Final Research Report
  • [Presentation] Feedstock Recycling of Organic and Inorganic Materials from Solid Waste2011

    • Author(s)
      Shogo Kumagai, Grause Guido, Tomohito Kameda, Toshiaki Yoshioka
    • Organizer
      2^<nd> International Symposium of Environmental Leader
    • Place of Presentation
      Ho Chi Minh (Viet Nam)
    • Year and Date
      2011-12-15
    • Related Report
      2011 Annual Research Report
  • [Presentation] Simultaneous silver and benzene recovery from X-ray film2011

    • Author(s)
      Shogo Kumagai, Guido Grause, Tomohito Kameda, Toshiaki Yoshioka
    • Organizer
      6th International Symposium on Feedstock Recycling of Polymeric Materials (ISFR2011)
    • Place of Presentation
      Toledo, Spain
    • Year and Date
      2011-10-06
    • Related Report
      2012 Final Research Report
  • [Presentation] Simultaneous Silver and Benzene Recovery from X-ray Film2011

    • Author(s)
      Shogo Kumagai, Grause Guido, Tomohito Kameda, Toshiaki Yoshioka
    • Organizer
      6^<th> International Symposium on Feedstock Recycling of Polymeric Materials (ISFR2011)
    • Place of Presentation
      Toledo (Spain)
    • Year and Date
      2011-10-06
    • Related Report
      2011 Annual Research Report
  • [Presentation] X線フィルムの熱分解油化と銀の回収2011

    • Author(s)
      熊谷将吾, Grause Guido, 亀田知人, 吉岡敏明
    • Organizer
      日本化学会第91春季年会
    • Place of Presentation
      神奈川大学(神奈川県)
    • Year and Date
      2011-03-28
    • Related Report
      2010 Annual Research Report
  • [Presentation] Improvement of the benzene yield from the pyrolysis of terephthalic acid using CaO2010

    • Author(s)
      Shogo Kumagai, Guido Grause, Tomohito Kameda, Toshiaki Yoshioka
    • Organizer
      2010 International Chemical Congress of Pacific Basin Societies (PACIFICHEM 2010)
    • Place of Presentation
      Hawaii, USA
    • Year and Date
      2010-12-18
    • Related Report
      2012 Final Research Report
  • [Presentation] Improvement of the benzene yield from the pyrolysis of terephthalic acid using CaO2010

    • Author(s)
      Shogo Kuraagai, Guido Grause, Tomohito Kameda, Toshiaki Yoshioka
    • Organizer
      2010 International Chemical Congress of Pacific Basin Societies (PACIFICHEM 2010)
    • Place of Presentation
      Hawaii (USA)
    • Year and Date
      2010-12-18
    • Related Report
      2010 Annual Research Report
  • [Presentation] New Application for the Use of Calcium Oxide in the Chemical Eecycling of Polymers2010

    • Author(s)
      Grause Guido, 松本翔太朗, 熊谷将吾, 亀田知人, 吉岡敏明, 高野達夫, 堀内英樹
    • Organizer
      無機マテリアル学会第121回学術講演会
    • Place of Presentation
      東北大学(宮城県)
    • Year and Date
      2010-11-05
    • Related Report
      2010 Annual Research Report
  • [Presentation] 生石灰を用いたテレフタル酸の熱分解によるベンゼン転化率の向上及び残渣の抑制2010

    • Author(s)
      熊谷将吾, Grause Guido, 亀田知人, 吉岡敏明
    • Organizer
      プラスチックリサイクル化学研究会第13回討論会
    • Place of Presentation
      千葉大学(千葉県)
    • Year and Date
      2010-09-21
    • Related Report
      2010 Annual Research Report
  • [Presentation] Decomposition of Gaseous Terephthalic Acid Using CaO Fixed-bed Reactor2010

    • Author(s)
      Shogo Kumagai
    • Organizer
      5^<th> International Symposium on Chemical-Environmental-Biomedical Technology for Young Researchers (isCEBT)
    • Place of Presentation
      Sendai (Japan)
    • Year and Date
      2010-09-06
    • Related Report
      2010 Annual Research Report
  • [Presentation] 固定床反応器を用いたPETの熱分解によるベンゼン回収率の向上2010

    • Author(s)
      熊谷将吾, Guido Grause, 亀田知人, 吉岡敏明
    • Organizer
      日本化学会第90春季年会
    • Place of Presentation
      近畿大学(東大阪市)
    • Year and Date
      2010-03-28
    • Related Report
      2009 Annual Research Report
  • [Presentation] 流動媒体に硬焼生石灰を用いたPET含有混合プラスチックの熱分解油化2009

    • Author(s)
      熊谷将吾, 松本翔太朗, Guido Grause, 亀田知人, 吉岡敏明
    • Organizer
      廃棄物資源循環学会東北支部第2回研究発表会
    • Place of Presentation
      夢メッセみやぎ(仙台市)
    • Year and Date
      2009-10-16
    • Related Report
      2009 Annual Research Report
  • [Presentation] Pyrolysis of mixed plastics in the fluidized bed using hard burnt lime as bed material2009

    • Author(s)
      Shotaro Matsumoto, Guido Grause, Tomohito Kameda, Toshiaki Yoshioka
    • Organizer
      The 5th International Symposium on Feedstock and Mechanical Recycling of Polymeric Materials (ISFR2009)
    • Place of Presentation
      Chengdu, China
    • Year and Date
      2009-10-12
    • Related Report
      2012 Final Research Report
  • [Presentation] プラスチックのフィードストックリサイクルとトランスファーテクノロジー2009

    • Author(s)
      吉岡敏明
    • Organizer
      第23回環境工学連合会講演会
    • Place of Presentation
      日本学術会議講堂(東京都)
    • Year and Date
      2009-04-17
    • Related Report
      2009 Annual Research Report
  • [Presentation] KINETIC INVESTIGATION OF PYROLYSIS AND HYDROLYSIS OF POLY(ETHYLENE TEREPHTHALATE)

    • Author(s)
      Guido Grause, Yuto Morohoshi, Shogo Kumagai, Tomohito Kameda, Toshiaki Yoshioka
    • Organizer
      19th International Symposium on Analytical and Applied Pyrolysis
    • Place of Presentation
      Linz (Austria)
    • Related Report
      2012 Annual Research Report
  • [Presentation] ポリエチレンテレフタレートの水蒸気分解速度解析

    • Author(s)
      諸星勇翔, 熊谷将吾, Grause Guido, 亀田知人, 吉岡敏明
    • Organizer
      平成24年度化学系学協会東北大会
    • Place of Presentation
      秋田
    • Related Report
      2012 Annual Research Report
  • [Presentation] 生石灰を用いた金属含有ポリエチレンテレフタレートの熱分解油化および金属回収

    • Author(s)
      熊谷将吾,Grause Guido,亀田知人,吉岡敏明
    • Organizer
      プラスチックリサイクル化学研究会第15回研究討論会
    • Place of Presentation
      米沢
    • Related Report
      2012 Annual Research Report
  • [Presentation] 18O同位体標識水を用いたポリエチレンテレフタレートの熱分解及び加水分解速度の解析

    • Author(s)
      諸星勇翔, 熊谷将吾, Grause Guido, 亀田知人, 吉岡敏明
    • Organizer
      プラスチックリサイクル化学研究会第15回研究討論会
    • Place of Presentation
      米沢
    • Related Report
      2012 Annual Research Report
  • [Presentation] Recovery of phenols from bisphenol A polycarbonate in the presence of MgO

    • Author(s)
      Rikard K rrbrant, Guido Grause, Tomohito Kameda, Toshiaki Yoshioka
    • Organizer
      第23回廃棄物資源循環学会研究発表会
    • Place of Presentation
      仙台
    • Related Report
      2012 Annual Research Report
  • [Presentation] Feedstock Recycling of Organic and Inorganic Materials by Thermal Decomposition of Metal-Containing Plastics

    • Author(s)
      Shogo Kumagai, Guido Grause, Tomohito Kameda, Toshiaki Yoshioka
    • Organizer
      The 12th Expert Meeting on Solid Waste Management in Asia and Pacific Islands (12th SWAPI)
    • Place of Presentation
      Tokyo (Japan)
    • Related Report
      2012 Annual Research Report
  • [Presentation] 熱硬化性樹脂プリント基板の熱分解挙動

    • Author(s)
      熊谷将吾, Grause Guido, 亀田知人, 吉岡敏明
    • Organizer
      日本化学会第93春季年会
    • Place of Presentation
      草津
    • Related Report
      2012 Annual Research Report
  • [Presentation] MgOの存在下におけるビスフェノールAポリカーボネートの水蒸気加水分解

    • Author(s)
      Kaerrbrant Rikard, Grause Guido, 亀田知人, 吉岡敏明
    • Organizer
      日本化学会第93春季年会
    • Place of Presentation
      草津
    • Related Report
      2012 Annual Research Report
  • [Presentation] ポリエチレンテレフタレートの水蒸気熱分解における加水分解の解析

    • Author(s)
      諸星勇翔、熊谷将吾, Grause Guido, 亀田知人, 吉岡敏明
    • Organizer
      日本化学会第93春季年会
    • Place of Presentation
      草津
    • Related Report
      2012 Annual Research Report
  • [Book] 産業調査会事典出版センター2012

    • Author(s)
      熊谷将吾,吉岡敏明
    • Publisher
      2編の3.プラスチック系材料の処理技術,リサイクル・廃棄物事典
    • Related Report
      2012 Final Research Report
  • [Book] 産業調査会事典出版センター2012

    • Author(s)
      熊谷将吾,吉岡敏明
    • Publisher
      3編の2.プラスチック分解のための科学リサイクル・廃棄物事典
    • Related Report
      2012 Final Research Report
  • [Book] リサイクル・廃棄物事典2012

    • Author(s)
      熊谷将吾, 吉岡敏明, 2編3、3編2
    • Publisher
      産業調査会辞典出版センター
    • Related Report
      2011 Annual Research Report
  • [Remarks] 東北大学大学院環境科学研究科 吉岡研究室ホームページ

    • URL

      http://www.che.tohoku.ac.jp/~env/index.html

    • Related Report
      2012 Final Research Report
  • [Remarks] 東北大学大学院環境科学研究科 吉岡研究室 研究業績

    • URL

      http://www.che.tohoku.ac.jp/~env/gyouseki.html

    • Related Report
      2012 Annual Research Report
  • [Remarks]

    • URL

      http://www.che.tohoku.ac.jp/~env/gyouseki.html

    • Related Report
      2011 Annual Research Report
  • [Remarks]

    • URL

      http://www.che.tohoku.ac.jp/~env/gyouseki.html

    • Related Report
      2010 Annual Research Report
  • [Remarks]

    • URL

      http://www.che.tohoku.ac.jp/~env/gyouseki.html

    • Related Report
      2009 Annual Research Report

URL: 

Published: 2009-04-01   Modified: 2019-07-29  

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