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Understanding the three-dimensional multiscale porous microstructures by applying deep neural networks

Research Project

Project/Area Number 21K14090
Research Category

Grant-in-Aid for Early-Career Scientists

Allocation TypeMulti-year Fund
Review Section Basic Section 19020:Thermal engineering-related
Research InstitutionThe University of Tokyo

Principal Investigator

SCIAZKO Anna  東京大学, 生産技術研究所, 特任助教 (30898945)

Project Period (FY) 2021-04-01 – 2023-03-31
Project Status Completed (Fiscal Year 2022)
Budget Amount *help
¥4,680,000 (Direct Cost: ¥3,600,000、Indirect Cost: ¥1,080,000)
Fiscal Year 2022: ¥1,690,000 (Direct Cost: ¥1,300,000、Indirect Cost: ¥390,000)
Fiscal Year 2021: ¥2,990,000 (Direct Cost: ¥2,300,000、Indirect Cost: ¥690,000)
Keywordssolid oxide fuel cell / machine learning / 3D microstructure / FIB-SEM / GAN network / semantic segmentation / super-resolution / artificial structure / porous material / porous electrode
Outline of Research at the Start

The multiscale porous media found interest in many fields of engineering. In particular, the porous electrode microstructure determines the performances of fuel cells and batteries. The multi-sized pore design is beneficial as large pores enhance the gas transport and nano-pores increase active reaction area. Here, the characterization methods of multi-sized porous media based on deep neural networks will be proposed. The focus is to provide high resolution large volume 3D characterization, fabricate synthetic 3D structure from single 2D image and correlate microstructure with performance.


Outline of Final Research Achievements

An automated microstructure analysis framework using machine learning was developed. The framework was built to improve three-dimensional (3D) microscopy analysis by super resolution and semantic segmentation algorithms. The developed framework can contribute in shortening actual measurement time up to 8 times and data post-processing time by two orders of magnitude. Furthermore, a novel method with generative network was proposed to create an artificial 3D microstructure model from a single two-dimensional image. Additionally, the generative network trained with microstructure datasets, can fabricate realistic microstructure models with predefined properties and gradients. The automated segmentation framework was used to characterize gadolinium doped ceria ceria-based solid oxide fuel (SOFC) anodes with the controlled properties (porosity, material composition, and particle size) and it enables to reconstruct SOFC anode with carbon deposition.

Academic Significance and Societal Importance of the Research Achievements

The porous media found interest in many fields of engineering. Particularly, the porous electrode microstructure determines the performances of fuel cells and batteries. This study proposed comprehensive framework for analyzing porous media microstructures based on machine learning methods.

Report

(3 results)
  • 2022 Annual Research Report   Final Research Report ( PDF )
  • 2021 Research-status Report
  • Research Products

    (14 results)

All 2023 2022 2021

All Journal Article (3 results) (of which Int'l Joint Research: 3 results,  Peer Reviewed: 3 results) Presentation (11 results) (of which Int'l Joint Research: 7 results,  Invited: 2 results)

  • [Journal Article] 3D microstructures of solid oxide fuel cell Ni-YSZ anodes with carbon deposition2023

    • Author(s)
      Sciazko Anna、Komatsu Yosuke、Nakamura Akiko、Ouyang Zhufeng、Hara Toru、Shikazono Naoki
    • Journal Title

      Chemical Engineering Journal

      Volume: 460 Pages: 141680-141680

    • DOI

      10.1016/j.cej.2023.141680

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Effects of mass fraction of La0.9Sr0.1Cr0.5Mn0.5O3-δ and Gd0.1Ce0.9O2-δ composite anodes for nickel free solid oxide fuel cells2022

    • Author(s)
      Sciazko Anna、Komatsu Yosuke、Yokoi Ryosuke、Shimura Takaaki、Shikazono Naoki
    • Journal Title

      Journal of the European Ceramic Society

      Volume: 42 Issue: 4 Pages: 1556-1567

    • DOI

      10.1016/j.jeurceramsoc.2021.11.039

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Operando observations of active three phase boundary of patterned nickel - yttria stabilized zirconia electrode in solid oxide cell2022

    • Author(s)
      Ouyang, Z., Komatsu, Y., Sciazko, A., Onishi, J., Nishimura, K. and Shikazono, N.
    • Journal Title

      J. Power Sources

      Volume: 529 Pages: 231228-231228

    • DOI

      10.1016/j.jpowsour.2022.231228

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Presentation] Machine Learning Methods for Predicting Microstructural Changes in Solid Oxide Cell Electrodes2022

    • Author(s)
      Sciazko, A., Yamagishi, R., Komatsu, Y., Ouyang, Z., Onishi, J., Nishimura, K., Shikazono, N.
    • Organizer
      Materials Science and Technology 2022 (MS&T22), Pittsburgh, Pennsylvania, USA
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 機械学習による SOFC微細構造変化の予測2022

    • Author(s)
      シチョンシコ アンナ,小松 洋介,山岸 鈴奈,鹿園 直毅
    • Organizer
      第26回動力・エネルギー技術シンポジウム講演論文集,佐賀
    • Related Report
      2022 Annual Research Report
    • Invited
  • [Presentation] Microstructures of Ni-GDC electrodes with carbon deposition2022

    • Author(s)
      Sciazko, A., Komatsu, Y., Nakamura, A., Sunada, Y., Ouyang, Z., Hara, T. and Shikazono, N.
    • Organizer
      15th European SOFC & SOE Forum, B1104, Lucerne, Switzerland
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Synthesizing Electrode Microstructures with Predefined Spatial Gradients By Conditional Generative Adversarial Networks2022

    • Author(s)
      Yamagishi, R., Sciazko, A., Komatsu, Y., and Shikazono, N.
    • Organizer
      Proc. 241th ECS meeting, I06-1083, Vancouver, Canada
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 析出還元法によるナノNi-GDCアノードの発電特性と微細構造2022

    • Author(s)
      Sciazko A., 砂田祐輔,小松洋介,鹿園直毅
    • Organizer
      第31回SOFC研究発表会講演要旨集
    • Related Report
      2022 Annual Research Report
  • [Presentation] Prediction of Microstructure Evolutions in Solid Oxide Cell Electrodes with Unsupervised Image-to-Image Translation Networks2022

    • Author(s)
      Sciazko, A., Komatsu, Y. and Shikazono, N.
    • Organizer
      46th International Conference and Expo on Advanced Ceramics and Composites (ICACC2022)
    • Related Report
      2021 Research-status Report
    • Int'l Joint Research
  • [Presentation] NiO Reduction Prediction with Unsupervised Image-to-Image Translation Network2021

    • Author(s)
      Sciazko A., Komatsu, Y., Shikazono, N.
    • Organizer
      第30回SOFC研究発表会
    • Related Report
      2021 Research-status Report
  • [Presentation] 3-D microstructures of Ni-YSZ anodes with carbon deposition2021

    • Author(s)
      Sciazko, A, Komatsu, Y., Ouyang, Z. and Shikazono, N.
    • Organizer
      6th Asian SOFC Symposium and Exhibition
    • Related Report
      2021 Research-status Report
    • Int'l Joint Research
  • [Presentation] Degradation predictions of solid oxide cells through Electrochemical Impedance Spectra with Long Short-Term Memory Neural Network2021

    • Author(s)
      Yamagishi, R., Sciazko, A., Komatsu, Y., Nishimura, K. and Shikazono, N.
    • Organizer
      6th Asian SOFC Symposium and Exhibition
    • Related Report
      2021 Research-status Report
    • Int'l Joint Research
  • [Presentation] Unsupervised Generative Adversarial Network for 3-D Microstructure Synthesis from 2-D Image2021

    • Author(s)
      Sciazko, A., Komatsu, Y. and Shikazono, N.
    • Organizer
      ECS Transactions, Volume 103, Number 1
    • Related Report
      2021 Research-status Report
    • Int'l Joint Research
  • [Presentation] 非等方な解像度を有するFIB-SEMデータセットからの電極構造再構築2021

    • Author(s)
      SCIAZKO ANNA, 小松洋介, 志村敬彬, 鹿園直毅
    • Organizer
      第25回 動力・エネルギー技術シンポジウム
    • Related Report
      2021 Research-status Report

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Published: 2021-04-28   Modified: 2024-01-30  

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