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Manifestation of nonlinear anomalous Hall effect by controlling charge-ordered domains in organic conductors

Research Project

Project/Area Number 21K18594
Research Category

Grant-in-Aid for Challenging Research (Exploratory)

Allocation TypeMulti-year Fund
Review Section Medium-sized Section 13:Condensed matter physics and related fields
Research InstitutionThe University of Tokyo

Principal Investigator

Osada Toshihito  東京大学, 物性研究所, 教授 (00192526)

Project Period (FY) 2021-07-09 – 2024-03-31
Project Status Completed (Fiscal Year 2023)
Budget Amount *help
¥6,240,000 (Direct Cost: ¥4,800,000、Indirect Cost: ¥1,440,000)
Fiscal Year 2022: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Fiscal Year 2021: ¥4,810,000 (Direct Cost: ¥3,700,000、Indirect Cost: ¥1,110,000)
Keywords非線形異常ホール効果 / 有機導体 / ディラック電子系 / 電荷秩序 / ドメイン / 非線形異常エッチングスハウゼン効果 / ドメイン制御
Outline of Research at the Start

有機導体α-(BEDT-TTF)2I3の弱い電荷秩序状態はギャップの開いたDirac電子系で、有限のBerry曲率双極子によりゼロ磁場下で電流誘起の異常Hall効果や軌道磁化が期待される。しかし現実の結晶では2種の電荷秩序ドメインが存在し、これらの効果を打ち消してしまう。本研究の目的は、片方の電荷秩序ドメインのみを選択的に形成させる手法を確立し、隠れた非線形異常Hall効果を顕在化させることである。そのために磁場中で電流を流して試料を徐冷しドメイン核を電流誘起軌道磁化を用いて配向させる。このドメイン制御手法の確立と有機導体初のトポロジカル輸送現象の観測が本研究の意義である。

Outline of Final Research Achievements

The weak charge ordering state of an organic conductor α-(BEDT-TTF)2I3 is a gapped tilted Dirac electron system breaking inversion symmetry, which is expected to exhibit the nonlinear anomalous Hall effect. However, its observation is expected to be difficult due to the cancellation between the two types of domains. Therefore, we have attempted to observe the nonlinear anomalous Hall effect by selective forming of one domain by the current field cooling method. (1) We were able to observe the nonlinear anomalous Hall effect even with normal cooling. This implies an imbalance in the domain ratio. (2) No significant effect on selective domain forming was observed by the current field cooling. (3) We discovered the nonlinear anomalous Ettingshausen effect, which is a thermoelectric analogue of the nonlinear anomalous Hall effect.

Academic Significance and Societal Importance of the Research Achievements

トポロジカル伝導現象は基礎・応用の観点から現代物性物理学の重要なトピックスの1つである。一方、有機分子性結晶は単純な電子構造を持ち、物質設計や物性制御の舞台を提供してきた。本研究は、有機分子性結晶においてトポロジカル伝導を初めて発現させたという意義を持つ。電流磁場中冷却法の有効性は確認できなかったが、観測を困難にするドメイン問題も大きな障害にはならないことが明らかとなった。さらに対応するトポロジカル熱電効果である非線形異常Ettingshausen効果の発見を通じ、トポロジカル物性物理の発展にも貢献できた。

Report

(4 results)
  • 2023 Annual Research Report   Final Research Report ( PDF )
  • 2022 Research-status Report
  • 2021 Research-status Report
  • Research Products

    (30 results)

All 2024 2023 2022 2021 Other

All Journal Article (11 results) (of which Peer Reviewed: 11 results,  Open Access: 7 results) Presentation (18 results) (of which Invited: 1 results) Remarks (1 results)

  • [Journal Article] Hofstadter Butterfly and Broken-Symmetry Quantum Hall States in α-Type Organic Dirac Fermion Systems2024

    • Author(s)
      Osada Toshihito
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 93 Issue: 3

    • DOI

      10.7566/jpsj.93.034711

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Quantized thermoelectric Hall plateau in the quantum limit of graphite as a nodal-line semimetal2023

    • Author(s)
      Kiswandhi Andhika、Ochi Tomotaka、Taen Toshihiro、Sato Mitsuyuki、Uchida Kazuhito、Osada Toshihito
    • Journal Title

      Physical Review B

      Volume: 107 Issue: 19

    • DOI

      10.1103/physrevb.107.195106

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Magnetic-field periodic quantum Sondheimer oscillations in thin-film graphite2023

    • Author(s)
      Taen Toshihiro、Kiswandhi Andhika、Osada Toshihito
    • Journal Title

      Physical Review B

      Volume: 108 Issue: 23 Pages: 235411-235411

    • DOI

      10.1103/physrevb.108.235411

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Broken-Symmetry Quantum Hall State in an Organic Dirac Fermion System2023

    • Author(s)
      Osada Toshihito
    • Journal Title

      JPSJ News and Comments

      Volume: 20 Pages: 06-06

    • DOI

      10.7566/jpsjnc.20.06

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Nonlinear Topological Transport in Organic Dirac Fermion System2022

    • Author(s)
      長田 俊人、アンディカ・ キスワンディ
    • Journal Title

      Butsuri

      Volume: 77 Issue: 4 Pages: 233-238

    • DOI

      10.11316/butsuri.77.4_233

    • ISSN
      0029-0181, 2423-8872
    • Year and Date
      2022-04-05
    • Related Report
      2022 Research-status Report
    • Peer Reviewed
  • [Journal Article] Observation of possible nonlinear anomalous Hall effect in organic two-dimensional Dirac fermion system2022

    • Author(s)
      Kiswandhi Andhika、Osada Toshihito
    • Journal Title

      Journal of Physics: Condensed Matter

      Volume: 34 Issue: 10 Pages: 105602-105602

    • DOI

      10.1088/1361-648x/ac3fd5

    • Related Report
      2022 Research-status Report 2021 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] 有機ディラック電子系におけるトポロジカル輸送現象2022

    • Author(s)
      長田俊人
    • Journal Title

      固体物理

      Volume: 57 Pages: 227-240

    • Related Report
      2022 Research-status Report 2021 Research-status Report
    • Peer Reviewed
  • [Journal Article] Thermoelectric Hall Effect at High-Magnetic-Field Quantum Limit in Graphite as a Nodal-Line Semimetal2022

    • Author(s)
      Osada Toshihito、Ochi Tomotaka、Taen Toshihiro
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 91 Issue: 6

    • DOI

      10.7566/jpsj.91.063701

    • Related Report
      2022 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] Weak localization on moire superlattice in twisted double bilayer graphene2022

    • Author(s)
      Kashiwagi Masaki、Taen Toshihiro、Uchida Kazuhito、Watanabe Kenji、Taniguchi Takashi、Osada Toshihito
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 61 Issue: 10 Pages: 100907-100907

    • DOI

      10.35848/1347-4065/ac934a

    • Related Report
      2022 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] Possible Nonlinear Anomalous Thermoelectric Effect in Organic Massive Dirac Fermion System2021

    • Author(s)
      Osada Toshihito、Kiswandhi Andhika
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 90 Issue: 5 Pages: 053704-053704

    • DOI

      10.7566/jpsj.90.053704

    • NAID

      40022563499

    • Related Report
      2021 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] Thermoelectric Effect at Quantum Limit in Two-Dimensional Organic Dirac Fermion System with Zeeman Splitting2021

    • Author(s)
      Osada Toshihito
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 90 Issue: 11 Pages: 113703-113703

    • DOI

      10.7566/jpsj.90.113703

    • NAID

      210000159372

    • Related Report
      2021 Research-status Report
    • Peer Reviewed / Open Access
  • [Presentation] α型層状有機結晶における3次元ディラック点2024

    • Author(s)
      長田俊人
    • Organizer
      日本物理学会2024年春季大会
    • Related Report
      2023 Annual Research Report
  • [Presentation] 薄膜グラファイトにおける磁場に周期的な量子Sondheimer振動の温度依存性2024

    • Author(s)
      田縁俊光,Andhika Kiswandhi,長田俊人
    • Organizer
      日本物理学会2024年春季大会
    • Related Report
      2023 Annual Research Report
  • [Presentation] 有Dirac電子系における対称性の破れた量子Hall状態と角度依存エッジ伝導2023

    • Author(s)
      長田俊人, 佐藤光幸
    • Organizer
      日本物理学会第78回年次大会
    • Related Report
      2023 Annual Research Report
  • [Presentation] Thermoelectric Hall conductivity of topological nodal line semimetal ZrSiS2023

    • Author(s)
      Andhika Kiswandhi,Toshihito Osada
    • Organizer
      日本物理学会第78回年次大会
    • Related Report
      2023 Annual Research Report
  • [Presentation] 捩れ積層グラフェンにおけるモアレ超格子中弱局在効果II2023

    • Author(s)
      柏木聖生, 内田和人, 渡邊賢司, 谷口尚, 長田俊人
    • Organizer
      日本物理学会第78回年次大会
    • Related Report
      2023 Annual Research Report
  • [Presentation] Quantized thermoelectric Hall conductivity in straight nodal line semimetal: the case of graphite2023

    • Author(s)
      Andhika Kiswandhi,Tomotaka Ochi,Toshihiro Taen,Mitsuyuki Sato,Kazuhito Uchida, Toshihito Osada
    • Organizer
      日本物理学会2023年春季大会
    • Related Report
      2022 Research-status Report
  • [Presentation] 強磁場領域における半金属薄膜の量子Sondheimer効果2023

    • Author(s)
      長田俊人,足立洋駿,田縁俊光,Andhika Kiswandhi
    • Organizer
      日本物理学会2023年春季大会
    • Related Report
      2022 Research-status Report
  • [Presentation] 強磁場下において薄膜グラファイトが示す磁場に周期的な抵抗振動と膜厚依存性2023

    • Author(s)
      田縁俊光,Andhika Kiswandhi,長田俊人
    • Organizer
      日本物理学会2023年春季大会
    • Related Report
      2022 Research-status Report
  • [Presentation] 質量のある有機ディラック電子系における非線形伝導2022

    • Author(s)
      長田俊人,柏木 聖生,アンディカ ・キスワンディ
    • Organizer
      日本物理学会2022年秋季大会
    • Related Report
      2022 Research-status Report
  • [Presentation] 多層ディラック電子系での低温強磁場下熱電測定2022

    • Author(s)
      佐藤光幸,長田俊人
    • Organizer
      日本物理学会2022年秋季大会
    • Related Report
      2022 Research-status Report
  • [Presentation] Quantum thermoelectric Hall effect study on bulk graphite under magnetic field up to 10 T2022

    • Author(s)
      Andhika Kiswandhi,Toshihito Osada
    • Organizer
      日本物理学会2022年秋季大会
    • Related Report
      2022 Research-status Report
  • [Presentation] 薄膜グラファイトにおける磁場に周期的な抵抗振動と膜厚に対する依存性2022

    • Author(s)
      田縁俊光,長田俊人
    • Organizer
      日本物理学会2022年秋季大会
    • Related Report
      2022 Research-status Report
  • [Presentation] 強磁場量子極限下のノーダルライン半金属における量子熱電効果2022

    • Author(s)
      長田俊人, 越智友崇
    • Organizer
      日本物理学会(第77回年次大会)
    • Related Report
      2021 Research-status Report
  • [Presentation] Nonlinear Anomalous Transport in the Weak Charge Order Phase of α-(BEDT-TTF)2I32022

    • Author(s)
      Andhika Kiswandhi,Toshihito Osada
    • Organizer
      日本物理学会(第77回年次大会)
    • Related Report
      2021 Research-status Report
  • [Presentation] 有機ディラック電子系におけるトポロジカル輸送2022

    • Author(s)
      長田俊人
    • Organizer
      日本物理学会(第77回年次大会)
    • Related Report
      2021 Research-status Report
    • Invited
  • [Presentation] 強磁場量子極限下のグラファイト薄膜における量子熱電効果の探索2022

    • Author(s)
      越智友崇, 長田俊人
    • Organizer
      日本物理学会(第77回年次大会)
    • Related Report
      2021 Research-status Report
  • [Presentation] 量子極限下の有機Dirac電子系α-(BEDT-TTF)2I3における量子熱電効果2021

    • Author(s)
      長田俊人
    • Organizer
      日本物理学会(2021年秋季大会)
    • Related Report
      2021 Research-status Report
  • [Presentation] Nonlinear Anomalous Hall Effect in α-(BEDT-TTF)2I3 under High Pressure2021

    • Author(s)
      Andhika Kiswandhi,Toshihito Osada
    • Organizer
      日本物理学会(2021年秋季大会)
    • Related Report
      2021 Research-status Report
  • [Remarks] 長田研究室

    • URL

      https://osada.issp.u-tokyo.ac.jp/

    • Related Report
      2023 Annual Research Report 2022 Research-status Report 2021 Research-status Report

URL: 

Published: 2021-07-13   Modified: 2025-01-30  

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