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Measurements of nanosale lithium diffusion coefficient using radioactive 8Li tracer

Research Project

Project/Area Number 22510118
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Nanomaterials/Nanobioscience
Research InstitutionHigh Energy Accelerator Research Organization

Principal Investigator

ISHIYAMA Hironobu  大学共同利用機関法人高エネルギー加速器研究機構, 素粒子原子核研究所, 研究機関講師 (50321534)

Co-Investigator(Renkei-kenkyūsha) JEONG Sunchan  大学共同利用機関法人高エネルギー加速器研究機構, 素粒子原子核研究所, 教授 (00262105)
HIRAYAMA Yoshikazu  大学共同利用機関法人高エネルギー加速器研究機構, 素粒子原子核研究所, 助教 (30391733)
SUGAI Hiroyuki  独立行政法人日本原子力研究開発機構, 原子力科学研究所, 研究副主幹 (80391291)
OSA Akihiko  独立行政法人日本原子力研究開発機構, 原子力科学研究所, 研究主幹 (80343929)
SATAKA Masao  独立行政法人日本原子力研究開発機構, 原子力科学研究所, 研究主幹 (70354826)
Project Period (FY) 2010 – 2012
Project Status Completed (Fiscal Year 2012)
Budget Amount *help
¥4,680,000 (Direct Cost: ¥3,600,000、Indirect Cost: ¥1,080,000)
Fiscal Year 2012: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2011: ¥650,000 (Direct Cost: ¥500,000、Indirect Cost: ¥150,000)
Fiscal Year 2010: ¥3,120,000 (Direct Cost: ¥2,400,000、Indirect Cost: ¥720,000)
Keywordsナノ計測
Research Abstract

We have developed a new in-situ nanoscale diffusion measurement method in solids for secondary lithium-ion batteries using a radioactive 8Li tracer. We have found the detection limit of the lithium diffusion coefficient can be improved to the order of 10^<-12>cm^2/s by detecting α particles emitted at a small angle relative to a sample surface that is irradiated with a low-energy 8Li of about 8 keV.

Report

(4 results)
  • 2012 Annual Research Report   Final Research Report ( PDF )
  • 2011 Annual Research Report
  • 2010 Annual Research Report
  • Research Products

    (22 results)

All 2013 2012 2011 2010 Other

All Journal Article (9 results) (of which Peer Reviewed: 5 results) Presentation (9 results) (of which Invited: 1 results) Remarks (4 results)

  • [Journal Article] Toward Online Nanoscale Diffusion Measurements Using Radioactive 8Li Tracer2013

    • Author(s)
      H. Ishiyama, S.C. Jeong, Y.X. Watanabe, Y. Hirayama, N. Imai, H. Miyatake, M. Oyaizu, I. Katayama, M. Sataka, A. Osa, Y. Otokawa, M. Matsuda, H. Makii
    • Journal Title

      Jpn. J. Appl. Phys

      Volume: 52 Pages: 10205-10205

    • Related Report
      2012 Final Research Report
  • [Journal Article] Toward Online Nanoscale Diffusion Measurements Using Radioactive 8Li Tracer2013

    • Author(s)
      H. Ishiyama
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 52 Issue: 1R Pages: 010205-010205

    • DOI

      10.7567/jjap.52.010205

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] GEM-MSTPC : An active-target type detector in low-pressure He/CO2 mixed gas2012

    • Author(s)
      H.Ishiyama, et al
    • Journal Title

      JINST

      Volume: 7 Issue: 03 Pages: 138-142

    • DOI

      10.1088/1748-0221/7/03/c03036

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Wall-loss distribution of charge breeding in an electron resonance ion source2012

    • Author(s)
      S.C.Jeong, H.Ishiyama, 5番目,計12名
    • Journal Title

      Review of Scientific Instruments

      Volume: 83

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Spin-polarization of radioactive 123In by the tilted-foil method2011

    • Author(s)
      Y.Hirayama, H.Ishiyama, 9番目,計23名
    • Journal Title

      European Physical Journal

      Volume: A47

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Li diffusion in Li ionic conductors of NaTl-type intermetallic compounds2010

    • Author(s)
      H.Sugai, H.Ishiyama, 11番目, 計16名
    • Journal Title

      JAEA-Review

      Volume: 2010-056 Pages: 91-92

    • Related Report
      2010 Annual Research Report
  • [Journal Article] Development of the GEM-MSTPC for measurements of low-energy nuclear reactions2010

    • Author(s)
      K.Yamaguchi, H.Ishiyama, 2番目, 計16名
    • Journal Title

      Nuclear Instruments and Methods A

      Volume: 623 Pages: 135-137

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Diffusion coefficient measurements on perovskite-type lithium ion conductor2010

    • Author(s)
      S.Takai, H.Ishiyama, 5番目, 計13名
    • Journal Title

      JAEA-Review

      Volume: 2010-056 Pages: 93-94

    • Related Report
      2010 Annual Research Report
  • [Journal Article] Development of GEM-MSTPC for measurements of the 8Li(alpha, n)11B reaction2010

    • Author(s)
      H.Ishiyama, et al., 計21名
    • Journal Title

      JAEA-Review

      Volume: 2010-056 Pages: 60-61

    • Related Report
      2010 Annual Research Report
  • [Presentation] 放射性核種トレーサー8Liによる電池材料中のナノスケールリチウム拡散測定~現状と将来~2013

    • Author(s)
      石山 博恒
    • Organizer
      ワークショップ「J-PARC 核変換実験施設の多目的利用」
    • Place of Presentation
      TKP 御茶ノ水カンファレンスセンター、 東京都
    • Year and Date
      2013-03-18
    • Related Report
      2012 Final Research Report
  • [Presentation] 放射性核種トレーサー8Liによる電池材料中のナノスケールリチウム拡散測定~現状と将来~2013

    • Author(s)
      石山博恒
    • Organizer
      ワークショップ「J-PARC核変換実験施設の多目的利用」
    • Place of Presentation
      東京都、TKP御茶ノ水カンファレンスセンター
    • Related Report
      2012 Annual Research Report
    • Invited
  • [Presentation] In-situ diffusion measurements in solids using short lived radioactive tracers of ^8Li and ^<20>Na2012

    • Author(s)
      H. Ishiyama, S.C. Jeong, Y.X. Watanabe, Y. Hirayama, N. Imai, H. Miyatake, M. Oyaizu, I. Katayama, M. Sataka, A. Osa, Y. Otokawa, M. Matsuda, H. Makii
    • Organizer
      XVI International Conference on Electromagnetic Isotope Separators and Techniques Related to their Application (EMIS 2012)
    • Place of Presentation
      Matsue, Japan
    • Related Report
      2012 Final Research Report
  • [Presentation] Online Diffusion Experiments in Solids by implanting Radiotracer Beam of ^8Li2012

    • Author(s)
      S.C. Jeong, H. Ishiyama, N. Imai, Y. Hirayama, H. Miyatake, Y.X. Watanabe, I. Katayama, H. Kawakami, M. Sataka, S. Okayasu, S. Ichikawa, K. Nishio, S. Mitsuoka, T. Nakanoya, M. Yahagi, T. Hashimoto
    • Organizer
      Eights International Symposium on Swift Heavy Ions in Matter (SHIM 2012)
    • Place of Presentation
      Kyoto Univ., Japan
    • Related Report
      2012 Final Research Report
  • [Presentation] In-situ diffusion measurements in solids using short lived radioactive tracers of 8Li and 20Na2012

    • Author(s)
      H. Ishiyama
    • Organizer
      XVI International Conference on Electromagnetic Isotope Separators and Techniques Related to their Application (EMIS 2012)
    • Place of Presentation
      島根県松江市、くにびきメッセ
    • Related Report
      2012 Annual Research Report
  • [Presentation] Online Diffusion Experiments in Solids by Implanting Radiotracer Beam of 8Li2012

    • Author(s)
      S.C. Jeong
    • Organizer
      Eighth International Symposium on Swift Heavy Ions in Matter (SHIM 2012)
    • Place of Presentation
      京都大学
    • Related Report
      2012 Annual Research Report
  • [Presentation] Experimental studies of astrophysical reaction rates using low-energy radioactive nuclear beams2011

    • Author(s)
      石山博恒
    • Organizer
      2011年韓国物理学会Korea-Japan Common Symposium
    • Place of Presentation
      釜山、韓国(招待講演)
    • Year and Date
      2011-10-20
    • Related Report
      2011 Annual Research Report
  • [Presentation] 放射性核種トレーサー8Liによるナノスケールでのリチウム拡散係数測定2010

    • Author(s)
      石山 博恒
    • Organizer
      第54回固体イオニクス研究会・第14回超イオン導電体物性研究会
    • Place of Presentation
      徳島大学
    • Year and Date
      2010-05-26
    • Related Report
      2012 Final Research Report
  • [Presentation] 放射性核種トレーサー8Liによるナノスケールでのリチウム拡散係数測定2010

    • Author(s)
      石山博恒
    • Organizer
      第54回固体イオニクス研究会・第14回超イオン導電体物性研究科医
    • Place of Presentation
      徳島大学
    • Year and Date
      2010-05-26
    • Related Report
      2010 Annual Research Report
  • [Remarks] ホームページ

    • URL

      http://kekrnb.kek.jp/

    • Related Report
      2012 Final Research Report
  • [Remarks] KEK RNB Group

    • URL

      http://kekrnb.kek.jp/index.php?FrontPage

    • Related Report
      2012 Annual Research Report
  • [Remarks]

    • URL

      http://kekrnb.kek.jp/index.php?FrontPage

    • Related Report
      2011 Annual Research Report
  • [Remarks]

    • URL

      http://triac.kek.jp/

    • Related Report
      2010 Annual Research Report

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Published: 2010-08-23   Modified: 2019-07-29  

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