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Investigation of spin liquid state near the quantum critical point by high-pressure measurements of quantum kagome lattice antiferromagnets

Research Project

Project/Area Number 22540348
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Condensed matter physics II
Research InstitutionKobe University

Principal Investigator

OKUBO Susumu  神戸大学, 分子フォトサイエンス研究センター, 助教 (80283901)

Project Period (FY) 2010 – 2012
Project Status Completed (Fiscal Year 2012)
Budget Amount *help
¥4,290,000 (Direct Cost: ¥3,300,000、Indirect Cost: ¥990,000)
Fiscal Year 2012: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2011: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Fiscal Year 2010: ¥1,820,000 (Direct Cost: ¥1,400,000、Indirect Cost: ¥420,000)
Keywords磁性 / フラストレーション / 量子相転移 / 圧力下測定 / スピン液体 / カゴメ格子 / スピンフラストレーション
Research Abstract

To investigate spin-liquid state stability for Dzyaloshinski-Moriya (DM) interaction (antisymmetric exchange interaction), magnetic susceptibility measurements of quantum kagome antiferromagnets ZnCu_3(OH)_6Cl_2 (Herbertsmithite) and Cu_3V_2O_7(OH)_2・2H_2O (Volborthite) have been performed under high-pressure at low temperature. Quantum transition from spin-liquid state to Neel state in these systems cannot observed in high-pressure up to 7.9 kbar at low temperature down to 1.8 K. On the other hand, D terms of DM interaction in quantum-spin kagome like antiferromagnet Cu_2O(SO_4) (Dolerophanite), classical-spin kagome lattice antiferromagnet KCr_3(SO_4)_2(OH_6) (Cr-jarosite) and spin-liquid ground state honeycomb lattice antiferromagnet Bi_3Mn_4O_12(NO_3) have been estimated using high-frequency ESR measurements.

Report

(4 results)
  • 2012 Annual Research Report   Final Research Report ( PDF )
  • 2011 Annual Research Report
  • 2010 Annual Research Report
  • Research Products

    (33 results)

All 2013 2012 2011 2010 Other

All Journal Article (9 results) (of which Peer Reviewed: 8 results) Presentation (23 results) (of which Invited: 2 results) Remarks (1 results)

  • [Journal Article] Antiferromagnetic ordering in Sr_2CrO_42013

    • Author(s)
      M. Rani, H. Sakurai, S. Okubo, K. Takamoto, R. Nakata, T. Sakurai, H. Ohta, A. Matsuo, Y. Kohama, K. Kindo, J. Ahmad
    • Journal Title

      J. Phys.: Cond. Mat

      Volume: 25 Issue: 22 Pages: 226001-5

    • DOI

      10.1088/0953-8984/25/22/226001

    • Related Report
      2012 Annual Research Report 2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Developments of Multi-extreme High Field ESR in Kobe2013

    • Author(s)
      H. Ohta, S. Okubo, E. Ohmichi, T. Sakurai, W.-M. Zhang, T. Shimokawa
    • Journal Title

      J. Low Temp Phys

      Volume: 170 Issue: 5-6 Pages: 511-519

    • DOI

      10.1007/s10909-012-0683-7

    • Related Report
      2012 Annual Research Report 2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Dzyaloshinsky-Moriya interaction and field-induced magnetic order in an antiferromagnetic honeycomb lattice compound Bi_3Mn_4O_12(NO_3) studied by high-field electron spin resonance2012

    • Author(s)
      S. Okubo, T. Ueda, H. Ohta, W. Zhang, T. Sakurai, N. Onishi, M. Azuma, Y. Shimakawa, H. Nakano, T. Sakai
    • Journal Title

      Phys. Rev. B

      Volume: 86 Issue: 14

    • DOI

      10.1103/physrevb.86.140401

    • Related Report
      2012 Annual Research Report 2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Possible new temperature phase observed in GeCo_2O_4 spinel by high-field ESR2012

    • Author(s)
      T. Yamasaki, S. Okubo, H. Ohta, T. Sakurai, S. Ikeda, H. Oshima, M. Takahashi, S. Hara, K. Tomiyasu, T. Watanabe
    • Journal Title

      J. Phys.: Conf. Serie

      Volume: 400 Issue: 3 Pages: 32119-4

    • DOI

      10.1088/1742-6596/400/3/032119

    • Related Report
      2012 Annual Research Report 2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Dzyloshinsky-Moriya Interaction Estimated by AFMR of Kagome Like Substance Cu_2O(SO_4)2012

    • Author(s)
      N. Takahashi, S. Okubo, H. Ohta, T. Sakurai, M. Fujisawa, H. Kikuchi
    • Journal Title

      J. Phys.: Conf. Serie.

      Volume: 400 Issue: 3 Pages: 32097-4

    • DOI

      10.1088/1742-6596/400/3/032097

    • Related Report
      2012 Annual Research Report 2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Anomalous Spin Dynamics Observed by High-Frequency ESR in Honeycomb Lattice Antiferromagnet InCu_<2/3>V_<1/3>O_32011

    • Author(s)
      S.Okubo, H.Wada, H.Ohta, T.Tomita, M.Fujisawa, T.Sakurai, E.Ohmichi, H.Kikuchi
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 80 Issue: 2 Pages: 23705-4

    • DOI

      10.1143/jpsj.80.023705

    • Related Report
      2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Spin dynamics of S=1/2 kagome lattice antiferromagnets observed by high-field ESR2010

    • Author(s)
      H. Ohta, W. Zhang, S. Okubo, M. Fujisawa, T. Sakurai, Y. Okamoto, H. Yoshida, Z. Hiroi
    • Journal Title

      Phys. Status Solidi B

      Volume: 247 Issue: 3 Pages: 679-681

    • DOI

      10.1002/pssb.200983033

    • Related Report
      2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] High-Field ESR Measurements of S=1/2 Kagome Lattice Antiferromagnet BaCu_3V_2O_8(OH)_22010

    • Author(s)
      W. Zhang, H. Ohta, S. Okubo, M. Fujisawa, T. Sakurai, Y. Okamoto, H. Yoshida, Z. Hiroi
    • Journal Title

      J. Phys. Soc. Jpn

      Volume: 79 Issue: 2 Pages: 23708-4

    • DOI

      10.1143/jpsj.79.023708

    • Related Report
      2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Spin-Gap Observation in the Triangular Lattice Antiferromagnet InMnO_3by High-Field ESR2010

    • Author(s)
      H. Ohta, N. Matsumi, S. Okubo, M. Fujisawa, T. Sakurai, H. Kikuchi, T. Nakamura
    • Journal Title

      J. Phys.: Conf. Serie.

      Volume: 200 Issue: 2 Pages: 22041-4

    • DOI

      10.1088/1742-6596/200/2/022041

    • Related Report
      2012 Final Research Report
  • [Presentation] 蜂の巣格子反強磁性体のテラヘルツ光ESR 測定2012

    • Author(s)
      大久保晋, 和田秀雄, 張衛民, 櫻井敬博, 太田仁, 冨田崇弘, 藤澤真士, 菊池彦光
    • Organizer
      兵庫県立大学大学院・物質理学研究科「フロンティア機能物質創製センター」シンポジウム
    • Place of Presentation
      フロンティア機能物質創製センター (招待)
    • Year and Date
      2012-12-22
    • Related Report
      2012 Final Research Report
  • [Presentation] S=1/2カゴメ格子反強磁性体のESRによる研究2012

    • Author(s)
      太田仁
    • Organizer
      日本物理学会
    • Place of Presentation
      関西学院大学(兵庫県)
    • Year and Date
      2012-03-25
    • Related Report
      2011 Annual Research Report
  • [Presentation] ハニカム格子反強磁性体の秩序の特異性2012

    • Author(s)
      大久保晋
    • Organizer
      基研研究会「量子スピン系の物理」
    • Place of Presentation
      京都大学基礎物理学研究所パナソニック国際交流ホール (招待)
    • Related Report
      2012 Final Research Report
  • [Presentation] S=3/2 カゴメ格子反強磁性体 KCr_3(SO_4)_2(OH)_6のテラヘルツ ESR 測定2012

    • Author(s)
      大久保晋,中田亮平,高橋直己,下川統久朗,櫻井敬博,張衛民,太田仁,奥田浩司,原茂生,佐藤博彦
    • Organizer
      第22回日本赤外線学会研究発表会
    • Place of Presentation
      関西大学千里山キャンパス 100 周年記念会館ホール
    • Related Report
      2012 Final Research Report
  • [Presentation] Cr-Jarosite の ESR 測定 II2012

    • Author(s)
      中田亮平,高橋直己,櫻井敬博,張衛民,大久保晋,太田仁,奥田浩司,原茂生,佐藤博彦
    • Organizer
      日本物理学会年次大会
    • Place of Presentation
      横浜国立大学常盤台キャンパス
    • Related Report
      2012 Final Research Report
  • [Presentation] 強磁場 ESR 測定による S=3/2 ハニカム格子反強磁性体Bi_3Mn_4O_12(NO_3)のDM 相互作用の研究2012

    • Author(s)
      大久保晋,植田友成,太田仁,張衛民,櫻井敬博,大西希,東正樹,島川祐一,中野博生,坂井徹
    • Organizer
      日本物理学会年次大会
    • Place of Presentation
      横浜国立大学常盤台キャンパス
    • Related Report
      2012 Final Research Report
  • [Presentation] ESR Measurement of S=3/2 Kagome Antiferromagnet Cr-Jarosite2012

    • Author(s)
      R. Nakata, N. Takahashi, W. Zhang, S. Okubo, H. Ohta, T. Sakurai, K. Okuda, S. Hara, H. Sato
    • Organizer
      8th Asia-Pacific EPR/ESR Symposium (APES 2012)
    • Place of Presentation
      Beijing, China
    • Related Report
      2012 Annual Research Report 2012 Final Research Report
  • [Presentation] Origin of Field Induced Magnetic Ordering in Frustrated Honeycomb Lattice Antiferromagnet2012

    • Author(s)
      S. Okubo, T. Ueda, W. Zhang, T. Sakurai, M. Fujisawa, H. Ohta, N. Ohnishi, M. Azuma, Y. Shimakawa, N. Kumada
    • Organizer
      19th International Conference on Magnetism
    • Place of Presentation
      Busan, Korea
    • Related Report
      2012 Annual Research Report 2012 Final Research Report
  • [Presentation] Cr Jarosite の ESR 測定2012

    • Author(s)
      中田亮平, 高橋直己, 張衞民, 大久保晋, 太田仁, 奥田浩司, 原茂生, 佐藤博彦
    • Organizer
      日本物理学会第67回年次大会
    • Place of Presentation
      兵庫県西宮市 関西学院大学
    • Related Report
      2012 Final Research Report
  • [Presentation] 強磁場ESR測定によるS=3/2ハニカム格子反強磁性体Bi3Mn4O12(NO3)のDM相互作用の研究2012

    • Author(s)
      大久保晋
    • Organizer
      日本物理学会
    • Place of Presentation
      横浜国立大学
    • Related Report
      2012 Annual Research Report
  • [Presentation] ハニカム格子反強磁性体の秩序の特異性2012

    • Author(s)
      大久保晋
    • Organizer
      基研研究会「量子スピン系の物理」
    • Place of Presentation
      京都大学基礎物理学研究所
    • Related Report
      2012 Annual Research Report
    • Invited
  • [Presentation] 蜂の巣格子反強磁性体のテラヘルツ光ESR測定2012

    • Author(s)
      大久保晋
    • Organizer
      兵庫県立大学大学院物質理学研究科「フロンティア機能物質創製センター」シンポジウム
    • Place of Presentation
      姫路、日本
    • Related Report
      2012 Annual Research Report
    • Invited
  • [Presentation] 多周波数 ESR 測定によるハニカム格子反強磁性体 InCu_2/3V_1/3O_3 の特異なスピンダイナミクスの観測2011

    • Author(s)
      大久保晋, 和田秀雄, 太田仁, 冨田崇弘, 藤澤真士, 櫻井敬博, 大道英二, 菊池彦光
    • Organizer
      第50回電子スピンサイエンス学会年会(SEST2011)
    • Place of Presentation
      仙台市仙台国際センター
    • Related Report
      2012 Final Research Report
  • [Presentation] Development of High-Frequency High Field ESR system and Its Application to Spin Frustration System2011

    • Author(s)
      S. Okubo
    • Organizer
      29th National Physics Congress
    • Place of Presentation
      College of Science, University of the Philippines Diliman, Philippines (plenary)
    • Related Report
      2012 Final Research Report
  • [Presentation] フラストレートスピン系 Dolerophanite (Cu2O(SO4))の強磁場 ESR2011

    • Author(s)
      大久保晋, 高橋直己, 張衛民, 櫻井敬博, 太田仁, 藤澤真士, 菊池彦光
    • Organizer
      日本物理学会年次大会 2011 年秋季大会
    • Place of Presentation
      富山大学五福キャンパス
    • Related Report
      2012 Final Research Report
  • [Presentation] Dzyaloshinsky-Moriya Interaction Estimated by AFMR of Kagome Like Substance Cu_2O(SO_4) Observed at 1.8K2011

    • Author(s)
      N. Takahashi, M. Tomoo, S. Okubo, T. Sakurai, M. Fujisawa, H. Kikuchi, H. Ohta
    • Organizer
      26th International Conference on Low Temperature Physics
    • Place of Presentation
      Beijing International Convention Center, China (poster)
    • Related Report
      2012 Final Research Report
  • [Presentation] Low-Temperature Multi-frequency ESR Study of Spin 1/2 Kagome lattice Antiferromagnetic Materials2011

    • Author(s)
      W. Zhang, M. Tomoo, S. Okubo, T. Sakurai, H. Ohta, H. Kikuchi, H. Yoshida, Y.Okamoto, and Z. Hiroi
    • Organizer
      26th International Conference on Low Temperature Physics
    • Place of Presentation
      Beijing International Convention Center, China (poster)
    • Related Report
      2012 Final Research Report
  • [Presentation] Spin Dynamics of Frustrated Honeycomb Lattice Antiferromagnet2011

    • Author(s)
      S. Okubo, Y. Yu, W. Zhang, T. Sakurai, M. Fujisawa, H. Ohta, H. Kikuchi, N. Ohnishi, M. Azuma, Y. Shimakawa, and N. Kumada
    • Organizer
      26th International Conference on Low Temperature Physics
    • Place of Presentation
      Beijing International Convention Center, China (invite)
    • Related Report
      2012 Final Research Report
  • [Presentation] Multi-Frequency ESR measurements of Frustrated Honeycomb Lattice Antiferromagnets2011

    • Author(s)
      S. Okubo
    • Organizer
      A joint meeting between the MEXT Japanese Network on "Novel State of Matter Induced by Frustration" and the Quantum Materials Program of the Canadian Institute for Advanced Research
    • Place of Presentation
      Vancouver, Canada (poster)
    • Related Report
      2012 Final Research Report
  • [Presentation] カゴメ格子磁性体 BaCu_3V_20_8(OH)_2のテラヘルツ光ESR2010

    • Author(s)
      張衛民,大久保晋,友尾水樹,櫻井敬博,太田仁,岡本佳比古,吉田紘行,広井善二
    • Organizer
      第20回(平成22 年度)日本赤外線学会
    • Place of Presentation
      立命館大学びわこくさつキャンパス (ポスター)
    • Related Report
      2012 Final Research Report
  • [Presentation] カゴメ格子磁性体 BaCu_3V_2O_8(OH)_2のサブミリ波 ESR III2010

    • Author(s)
      張衛民,大久保晋,太田仁,友尾水樹,櫻井敬博,岡本佳比古,広井善二,吉田紘行
    • Organizer
      日本物理学会2010 年秋季大会
    • Place of Presentation
      大阪府立大学中百舌鳥キャンパス (ポスター)
    • Related Report
      2012 Final Research Report
  • [Presentation] Possible kagome ice state in Co2(OH)3Br studied by high field ESR2010

    • Author(s)
      M. Tomoo, S. Okubo, M. Fujisawa, T. Sakurai, H. Ohta, M. Hagihara, X.-G. Zheng
    • Organizer
      The 5th International Conference on Highly Frustrated Magnetism 2010
    • Place of Presentation
      John Hopkins University, Baltimore, USA (poster)
    • Related Report
      2012 Final Research Report
  • [Presentation] Multi frequency ESR measurements of S=3/2 honeycomb lattice antiferromagnet Bi_3Mn_4O_12(NO_3)2010

    • Author(s)
      S. Okubo, Y. Yu, W. Zhang, M. Fujisawa, T. Sakurai, H. Ohta, N. Ohishi, M. Azuma, Y. Shimakawa, N. Kumada
    • Organizer
      The 5th International Conference on Highly Frustrated Magnetism 2010
    • Place of Presentation
      John Hopkins University, Baltimore, USA (poster)
    • Related Report
      2012 Final Research Report
  • [Remarks]

    • URL

      http://extreme.phys.sci.kobe-u.ac.jp/extreme/staffs/okubo/

    • Related Report
      2012 Final Research Report

URL: 

Published: 2010-08-23   Modified: 2020-05-15  

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