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Fullerene-transition metal hybrid spin injector for nanocarbon spintronics

Research Project

Project/Area Number 24360266
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypePartial Multi-year Fund
Section一般
Research Field Physical properties of metals
Research InstitutionJapan Atomic Energy Agency

Principal Investigator

SAKAI Seiji  独立行政法人日本原子力研究開発機構, 原子力科学研究部門 先端基礎研究センター, グループリーダー (10354929)

Co-Investigator(Kenkyū-buntansha) ENTANI Shiro  独立行政法人日本原子力研究開発機構, 原子力科学研究部門・先端基礎研究センター, 副主任研究員 (40549664)
松本 吉弘  独立行政法人日本原子力研究開発機構, 原子力科学研究部門 先端基礎研究センター, 研究員 (80455287)
Project Period (FY) 2012-04-01 – 2015-03-31
Project Status Completed (Fiscal Year 2014)
Budget Amount *help
¥11,700,000 (Direct Cost: ¥9,000,000、Indirect Cost: ¥2,700,000)
Fiscal Year 2014: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
Fiscal Year 2013: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
Fiscal Year 2012: ¥7,800,000 (Direct Cost: ¥6,000,000、Indirect Cost: ¥1,800,000)
Keywordsフラーレン / ナノ炭素 / スピントロニクス / グラフェン / 分子スピントロニクス / 界面 / X線吸収 / X線磁気円二色性 / スピン注入 / 磁性金属 / トンネル磁気抵抗効果 / スピン偏極 / スピンフィルター / XMCD / グラニュラー薄膜
Outline of Final Research Achievements

Nanocarbons including graphene and fullerenes attract considerable attention as promising candidate materials for future spintronics. In this project, we investigated spintronic properties of fullerene(C60)-transition metal hybrid structures for realizing highly-efficient spin-injection electrodes for nanocarbons.
Our magnetotransport study of the granular-structured hybrid thin films composed of C60 and iron nanocrystals clarified that the spin polarization of the conduction electrons in the hybrid film is remarkably enhanced due to the spin-filetering effect of the C60/Fe interface. Furthermore, according to the depth-resolved XMCD spectroscopy and theoretical calculations, it was demonstrated that at the C60/Fe interface the electronic states of C60 is significantly modified and a visible spin polarization is induced into C60 by the interfacial interactions between C60 and Fe.

Report

(4 results)
  • 2014 Annual Research Report   Final Research Report ( PDF )
  • 2013 Annual Research Report
  • 2012 Annual Research Report
  • Research Products

    (6 results)

All 2016 2014 2013 2012

All Journal Article (2 results) (of which Peer Reviewed: 2 results) Presentation (4 results) (of which Invited: 2 results)

  • [Journal Article] High spin polarization at the Fe/C60 interface in the Fe-doped C_<60> film2013

    • Author(s)
      S. Sakai, Y. Matsumoto, M. Ohtomo, S. Entani, P. V. Avramov, P. B. Sorokin, H. Naramoto
    • Journal Title

      Synth. Met.

      Volume: 173 Pages: 22-22

    • DOI

      10.1016/j.synthmet.2012.10.027

    • Related Report
      2013 Annual Research Report 2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Spin orientation transition across the single-layer graphene/nickel thin film interface2013

    • Author(s)
      Yoshihiro Matsumoto, Shiro Entani, Akihiro Koide, Manabu Ohtomo, Pavel V. Avramov, Hiroshi Naramoto, Kenta Amemiya, Takashi Fujikawa and Seiji Sakai
    • Journal Title

      J. Mater. Chem. C

      Volume: 1 Issue: 35 Pages: 5533-5537

    • DOI

      10.1039/c3tc30872c

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Presentation] Carbon-based hybrid structures for spintronics2016

    • Author(s)
      境 誠司
    • Organizer
      2nd International Symposium on Nanoparticles/Nanomaterials and Applications
    • Place of Presentation
      Lisbon, Portugal
    • Year and Date
      2016-01-18 – 2016-01-21
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] 分子スピントロニクスと界面スピン物性2014

    • Author(s)
      境 誠司
    • Organizer
      第59回物性若手夏の学校
    • Place of Presentation
      浜名湖ロイヤルホテル(浜松)
    • Year and Date
      2014-07-29 – 2014-08-02
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] High interface spin polarization and its mechanism in fullerene-magnetic metal systems2012

    • Author(s)
      S. Sakai
    • Organizer
      4th Worldwide University Network International Conference on Spintronics
    • Place of Presentation
      Sydney, Australia(招待講演)
    • Related Report
      2012 Annual Research Report
  • [Presentation] High spin polarization of tunneling electrons at the interfaces in fullerene-magnetic metal systems2012

    • Author(s)
      S. Sakai
    • Organizer
      4th International Meeting on Spins in Organic Semiconductors
    • Place of Presentation
      London, England
    • Related Report
      2012 Annual Research Report

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Published: 2012-04-24   Modified: 2019-07-29  

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