Ultra-fast electric field measurement by E-O effect in oragnic nonlinear optical crystal

• Project/Area Number: 24560535
• Research Category: Grant-in-Aid for Scientific Research (C)
• Allocation Type: Multi-year Fund
• Section: 一般
• Research Field: Measurement engineering
• Research Institution: The Institute of Physical and Chemical Research
• Principal Investigator: MINAMIDE Hiroaki 独立行政法人理化学研究所, 光量子工学研究領域, チームリーダー (10322687)
• Co-Investigator(Kenkyū-buntansha): TOMIZAWA Hiromitsu 公益財団法人高輝度光科学研究センター, 加速器部門, 副主幹研究員 (40344395)
• Co-Investigator(Renkei-kenkyūsha): MATSUKAWA Takeshi 茨城大学, フロンティア応用原子科学研究センター, 助教 (60580876)
• Project Period (FY): 2012-04-01 – 2015-03-31
• Project Status: Completed (Fiscal Year 2014)
• Budget Amount: ¥5,460,000 (Direct Cost: ¥4,200,000、Indirect Cost: ¥1,260,000); Fiscal Year 2014: ¥1,300,000 (Direct Cost: ¥1,000,000、Indirect Cost: ¥300,000); Fiscal Year 2013: ¥1,690,000 (Direct Cost: ¥1,300,000、Indirect Cost: ¥390,000); Fiscal Year 2012: ¥2,470,000 (Direct Cost: ¥1,900,000、Indirect Cost: ¥570,000)
• Keywords: 非線形光学 / 有機非線形光学結晶 / 電気光学効果 / 電気光学サンプリング / 電子ビームバンチング / 高速応答 / 単結晶成長 / テラヘルツ / 電場応答 / 結晶成長

Outline of Final Research Achievements

Organic DAST crystal has much larger nonlinearity and faster response time compared to those of conventional inorganic materials. We aim to measure ultra-short pulse electron beam bunching by using electric-optical effect in DAST.
Quality of DAST crystals was improved by optimizing solution grwoth method. Moreover, we have developed special process method for fragile DAST crystals using diamond edge to optimize shape of DAST crystals. Besides, off-line measurement system was developed to evaluate E-O effect capability in DAST in detail.
Consequently, we have demonstrated E-O measurement and sucessfully measured eletron beam bunching with femto-time scale using DAST.

Research Products

• [Journal Article] Diffraction-limited real-time terahertz imaging by optical frequency up-conversion in a DAST crystal (2015)
  • Author(s): Shuzhen Fan, Feng Qi, Takashi Notake, Kouji Nawata, Yuma Takida, Takeshi Matsukawa, and Hiroaki Minamide
  • Journal Title: Optics Express, Volume: 23 Issue: 6 Pages: 7611-7618
  • DOI: 10.1364/oe.23.007611
  • Peer Reviewed / Open Access / Acknowledgement Compliant
• [Journal Article] An ultra-broadband frequency-domain terahertz measurement system based on frequency conversion via DAST crystal with an optimized phase-matching condition (2014)
  • Author(s): Feng Qi, Shuzhen Fan, Takashi Notake, Kouji Nawata, Takeshi Matsukawa, Yuma Takida and Hiroaki Minamide
  • Journal Title: Laser Phys. Lett., Volume: 11 Issue: 8 Pages: 085403-085403
  • DOI: 10.1088/1612-2011/11/8/085403
  • Peer Reviewed / Acknowledgement Compliant
• [Journal Article] Terahertz-wave generation from 4-dimethylamino-N’-methyl-4’-stilbazolium p-bromobenzenesulfonate crystal: Effect of halogen substitution in a counter benzenesulfonate of stilbazolium derivatives (2014)
  • Author(s): Takeshi Matsukawa, Takashi Notake, Kouji Nawata, Shunsuke Inada, Shuji Okada, and Hiroaki Minamide
  • Journal Title: Opt. Mater. Volume: 36 Pages: 1995-1999
  • Peer Reviewed / Acknowledgement Compliant
• [Journal Article] 高出力テラヘルツ波光源の最先端と広がる応用 (2014)
  • Author(s): 南出泰亜
  • Journal Title: 電子情報通信学会誌 Volume: 97 Pages: 924-930
  • Peer Reviewed / Acknowledgement Compliant
• [Journal Article] Kilowatt-peak terahertz-wave generation and sub-femtojoule terahertz-wave pulse detection based on nonlinear optical wavelength-conversion at room temperature (2014)
  • Author(s): H. Minamide, S. Hayashi, K. Nawata, T. Taira, J. Shikata, and K. Kawase
  • Journal Title: J. Infrared, Millimeter, and Terahertz Waves Volume: vol.35 Issue: 1 Pages: 25-37
  • DOI: 10.1007/s10762-013-0041-0
  • Peer Reviewed
• [Journal Article] 10 aJ-level detection of ns pulse below 10 THz by frequency upconversion detection via DAST crystal : more than a 4 K bolometer (2014)
  • Author(s): F. Qi, S. Fan, T. Notake, K. Nawata, T. Matsukawa, Y. Takida, and H. Minamide
  • Journal Title: Opt. Lett. Volume: Vol.39 Issue: 5 Pages: 1294-1297
  • DOI: 10.1364/ol.39.001294
  • Peer Reviewed
• [Journal Article] Terahertz-wave generation from 4-dimethylamino-N'-methyl-4'-stilbazolium p-bromobenzenesulfonate crystal: Effect of halogen substitution in a counter benzenesulfonate of stilbazolium derivatives Optical Materials (2014)
  • Author(s): Takeshi Matsukawa, Takashi Notake, Kouji Nawata, Shunsuke Inada, Shuji Okada, Hiroaki Minamide
  • Journal Title: Optical Materials Volume: -
  • Peer Reviewed
• [Journal Article] Real-time terahertz wave imaging by nonlinear optical frequency up-conversion in a 4-dimethylamino-N-methyl-4-stilbazolium tosylate crystal (2014)
  • Author(s): S. Fan, F. Qi, T. Notake, K. Nawata, T. Matsukawa, Y. Takida, and H. Minamide
  • Journal Title: Appl. Phys. Lett. Volume: Vol.104 Issue: 10
  • DOI: 10.1063/1.4868134
  • Peer Reviewed
• [Journal Article] Pump-beam-induced optical damage depended on repetition frequency and pulse width in 4-dimethylamino-N’-methyl-4’-stilbazolium tosylate crystal (2013)
  • Author(s): T. Matsukawa, K. Nawata, T. Notake, F. Qi, H. Kawamata, and H. Minamide
  • Journal Title: Appl. Phys. Lett. Volume: 103 Issue: 2
  • DOI: 10.1063/1.4813602
  • Peer Reviewed
• [Presentation] 有機非線形光学結晶DAST及びBNAを用いたE-O変調に関する研究 (2015)
  • Author(s): 野竹 孝志，縄田 耕二，瀧田 佑馬，時実 悠，岡安 雄一，富澤 宏光，南出 泰亜
  • Organizer: 第62回応用物理学会春季学術講演会
  • Place of Presentation: 東海大学（神奈川）、日本
  • Year and Date: 2015-03-10 – 2015-03-13
• [Presentation] 二波長光注入型光パラメトリック発生を励起光に用いたサブテラヘルツ波発生 (2015)
  • Author(s): 時実悠，三宅良宜，范書振，縄田耕二，野竹孝志，瀧田佑馬，林伸一郎，南出泰亜
  • Organizer: 第2回理化学研究所－情報通信研究機構合同テラヘルツ研究交流会
  • Place of Presentation: 東北大学（仙台）、日本
  • Year and Date: 2015-02-09 – 2015-02-10
• [Presentation] 電波と光波の境界、テラヘルツ電磁波領域を拓く (2014)
  • Author(s): 南出泰亜
  • Organizer: 千葉大学大学院融合科学研究科セミナー
  • Place of Presentation: 千葉大学（千葉）、日本
  • Year and Date: 2014-12-18
• [Presentation] Real-time terahertz-wave imaging using nonlinear up-conversion detection (2014)
  • Author(s): Hiroaki Minamide, Feng Qi, and Shuzhen Fan
  • Organizer: The Fifth International Symposium on Terahertz Nanoscience
  • Place of Presentation: Martinique, France
  • Year and Date: 2014-12-01 – 2014-12-05
  • Invited
• [Presentation] Real-Time Terahertz Imaging By Optical Frequency Up-Conversion in a DAST Crystal with Sub-mm Resolution (2014)
  • Author(s): Shuzhen Fan, Feng Qi, and Hiroaki Minamide
  • Organizer: 理研シンポジウム
  • Place of Presentation: 仙台産業プラザ（仙台）、日本
  • Year and Date: 2014-11-25 – 2014-11-26
• [Presentation] 新テラヘルツ光応用を切り開く非線形光学テラヘルツ光発生/検出 (2014)
  • Author(s): 南出泰亜
  • Organizer: 理研と親しむ会
  • Place of Presentation: 如水会館（東京）、日本
  • Year and Date: 2014-11-14
• [Presentation] 非線形光学波長変換による波長可変テラヘルツ光源と高感度検出 (2014)
  • Author(s): 南出泰亜
  • Organizer: レーザー学会技術専門委員会
  • Place of Presentation: 宮古島（沖縄）、日本
  • Year and Date: 2014-10-31 – 2014-11-01
• [Presentation] 最先端非線形光学を基礎とした高強度テラヘルツ波光源の研究 (2014)
  • Author(s): 南出泰亜
  • Organizer: 第24回先端光量子アライアンスセミナー
  • Place of Presentation: 理研（和光）、日本
  • Year and Date: 2014-09-05
• [Presentation] バンチ内6D位相空間電荷密度分布の実時間計測可能な非破壊モニター開発 (2014)
  • Author(s): 冨澤宏光, 富樫格, 松原伸一, 伊達伸, 出羽英紀, 谷内努, 鈴木伸介, 岡安雄一, 下崎義人, 柳田謙一, 深見健司, 増田剛正, 清道明男, 黒田隆之助, 平義隆, 大和田成起, 小川奏, 南出泰亜, 野竹孝志
  • Organizer: 第11回日本加速器学会年会
  • Place of Presentation: リンクステーションホール青森（青森）、日本
  • Year and Date: 2014-08-12
• [Presentation] 有機ポッケルス EO 結晶を用いた電子バンチ電荷分布測定 (2014)
  • Author(s): 岡安雄一，小川奏，松原伸一，冨澤宏光，南出泰亜，野竹孝志，松川健
  • Organizer: 第11回日本加速器学会年会
  • Place of Presentation: リンクステーションホール青森（青森）、日本
  • Year and Date: 2014-08-12
• [Presentation] Real-Time Terahertz Imaging By Optical Frequency Up-Conversion in a DAST Crystal with Sub-mm Resolution (2014)
  • Author(s): Shuzhen Fan, Feng Qi, Takashi Notake, Kouji Nawata, Yuma Takida, Takeshi Matsukawa, Hiroaki Minamide
  • Organizer: International Symposium on Frontier of Terahertz Science
  • Place of Presentation: OIST Univ. (Okinawa）, JAPAN
  • Year and Date: 2014-08-04 – 2014-08-06
• [Presentation] Study on THz E-O modulation using Organic Nonlinear Materials (2014)
  • Author(s): Takashi Notake, Kouji Nawata, Shuzhen Fan, Yuma Takida, Yu Tokizane and Hiroaki Minamide
  • Organizer: International Symposium on Frontier of Terahertz Science
  • Place of Presentation: OIST Univ. (Okinawa), Japan
  • Year and Date: 2014-08-04 – 2014-08-06
• [Presentation] マイクロチップレーザーによる高出力THz波発生 (2014)
  • Author(s): 南出泰亜
  • Organizer: 第９回レーザー学会「マイクロ固体フォトニクス」専門委員会
  • Place of Presentation: 分子研（岡崎）、日本
  • Year and Date: 2014-06-26
• [Presentation] An ultra-broadband coherent THz measurement system based on frequency conversion via DAST crystal with optimized phase matching condition (2014)
  • Author(s): Feng Qi, Shuzhen Fan, Takashi Notake, Kouji Nawata, Takeshi Matsukawa, Yuma Takida, and Hiroaki Minamide
  • Organizer: Global Symposium on Millimeter Waves
  • Place of Presentation: Seoul, Korea
  • Year and Date: 2014-05-21 – 2014-05-23
• [Presentation] 10 aJ-level sensing of ns THz pulse by frequency upconversion detection below 10 THz (2014)
  • Author(s): Feng Qi, Shuzhen Fan, Kouji Nawata, Takeshi Notake, Takashi Matsukawa, Yuma Takida, and Hiroaki Minamide
  • Organizer: SPIE Sensing Technology+Applications
  • Place of Presentation: Baltimore, USA
  • Year and Date: 2014-05-05 – 2014-05-09
• [Presentation] THz Light: Light Our Life (2014)
  • Author(s): Feng Qi, Shuzhen Fan, and Hiroaki Minamide
  • Organizer: BIT's 3rd Annual Conference and EXPO of Analytix 2014
  • Place of Presentation: Dalian, China
  • Year and Date: 2014-04-25 – 2014-04-28
• [Presentation] Real-time THz imaging by difference frequency generation in a DAST crystal at room temperature (2014)
  • Author(s): S. Fan, F. Qi, T. Notake, K. Nawata, T. Matsukawa, Y. Takida, and H. Minamide
  • Organizer: The 3rd Advanced Lasers and Photon Sources
  • Place of Presentation: Pacific yokohama (Kanagawa),Japan
  • Year and Date: 2014-04-24
• [Presentation] High-peak-power Terahertz-wave generation and sensitive detection using second nonlinear optical effect (2014)
  • Author(s): Hiroaki Minamide
  • Organizer: Photonics Europe
  • Place of Presentation: Brussels, Belgium
  • Year and Date: 2014-04-14 – 2014-04-17
  • Invited
• [Presentation] Room temperature terahertz wave imaging at 60 fps by frequency up-conversion in DAST crystal (2014)
  • Author(s): Shuzhen Fan, Feng Qi, Takashi Notake, Kouji Nawata, Takeshi Matsukawa, Yuma Takida, and Hiroaki Minamide
  • Organizer: Photonics West 2014
  • Place of Presentation: San Francisco, USA
• [Presentation] 非線形光学効果によるテラヘルツ波発生検出技術開発の最先端 (2014)
  • Author(s): 南出泰亜
  • Organizer: 電子情報通信学会総合大会
  • Place of Presentation: 新潟県新潟市
  • Invited
• [Presentation] Design of sub-THz-wave generation based on DAST-DFG pumped by injection-seeded OPG (2013)
  • Author(s): Yoshiki Miyake, Kouji Nawata, Masatsugu Yamashita, Atsushi Sato and Hiroaki Minamide
  • Organizer: International workshop on Optical Terahertz Science and Technology (OTST 2013)
  • Place of Presentation: Kyoto, Japan
• [Presentation] Frequency up-conversion detection of THz waves by DAST-DFG: approaching more than 4K bolometer (2013)
  • Author(s): Feng Qi, Koji Nawata, Takashi Notake, Hiroshi Kawamata, Takeshi Matsukawa and Hiroaki Minamide
  • Organizer: International workshop on Optical Terahertz Science and Technology (OTST 2013)
  • Place of Presentation: Kyoto, Japan
• [Presentation] Ultra-widely tunable DFG THz-wave source using organic DAST and BNA crystals pumped by a dual-wavelength β-BaB2O4 optical parametric oscillator (2013)
  • Author(s): Takashi Notake , Koji Nawata, Takeshi Matsukawa, Feng Qi, Hiroshi Kawamata and Hiroaki Minamide
  • Organizer: The Advanced Lasers & Photon Sources Conference (ALPS'13)
  • Place of Presentation: Yokohama, Japan
• [Presentation] Study of efficient optical parametric generation in KTP crystal as pump source for DAST-DFG (2013)
  • Author(s): Kouji Nawata, Yoshiki Miyake, Shin’ichiro HAYASHI, Takashi Notake, Hiroshi Kawamata, Takeshi Matsukawa, Feng Qi, Hiroaki Minamide
  • Organizer: The Conference on Lasers and Electro Optics (CLEO:2013)
  • Place of Presentation: San Jose, USA
• [Presentation] Intense Terahertz-wave Generation and Sensitive Detection Using Nonlinear Optical Effect (2013)
  • Author(s): Hiroaki Minamide
  • Organizer: The 10th Conference on Lasers and Electro-Optics Pacific Rim (CLEO-PR 2013)
  • Place of Presentation: kyoto, Japan
  • Invited
• [Presentation] Efficient wavelength-conversion between terahertz wave and infrared light using nonlinear optical susceptibility (2013)
  • Author(s): Hiroaki Minamide
  • Organizer: International Symposium on Microwave/Terahertz Science and Application (MTSA 2013)
  • Place of Presentation: Shanghai, China
  • Invited
• [Presentation] Development of a single-crystalline stilbazolium derivative with halogenated benzenesulfonate for terahertz-wave generation (2013)
  • Author(s): Takeshi Matsukawa, Shunsuke Inada, Shuji Okada, and Hiroaki Minamide
  • Organizer: The 6th International Symposium on Lasers, Scintillators and Non-Linear Optical Materials (ISLOM-6)
  • Place of Presentation: Shanghai, China
• [Presentation] Terahertz‐Wave Detection using Nonlinear Optical Up‐Conversion by DAST (2013)
  • Author(s): Hiroaki Minamide, Feng Qi, Shuzhen Fan
  • Organizer: 21st International Conference on Applied Electromagnetics and Communications (ICECom 2013)
  • Place of Presentation: Dubrovnik, Croatia
  • Invited
• [Presentation] 高出力テラヘルツ波発生に向けたスチルバゾリウム誘導体単結晶の開発 (2013)
  • Author(s): 松川健
  • Organizer: 電子情報通信学会 POC研究会
  • Place of Presentation: 宮城県仙台市
• [Presentation] 非線形光学波長変換による最先端テラヘルツ波発生および検出技術の開発 (2013)
  • Author(s): 南出泰亜
  • Organizer: 電子情報通信学会電子デバイス研究会
  • Place of Presentation: 宮城県仙台市
  • Invited
• [Presentation] The First Demonstration of EOS 3D-BCD Monitor to Maximize 3D-Overlapping for HHG-Seeded FEL (2013)
  • Author(s): H. Tomizawa, T. Togashi, K. Ogawa, H. Tanaka, M. Yabashi, S. Matsubara, Y. Okayasu, and T. Ishikawa
  • Organizer: the 2nd International Beam Instrumentation Conference (IBIC2013)
  • Place of Presentation: Oxford, UK
  • Invited
• [Presentation] EOS-locked seeding system toward FT-limited XFEL pulses (2013)
  • Author(s): H. Tomizawa
  • Organizer: The High Brightness Electron Beams 2013: Toward to a fifth generation light source (HBEB 2013)
  • Place of Presentation: San Juan, Puerto Rico
  • Invited
• [Presentation] The operation status and future plans of SACLA accelerator (2013)
  • Author(s): H. Tomizawa
  • Organizer: The 6th Workshop on FEL Science, “New Horizon of XFEL science”
  • Place of Presentation: Tainan, Taiwan
  • Invited
• [Presentation] Stable Operation of HHG-Seeded EUV-FEL at the SCSS Test Accelerator (2013)
  • Author(s): H. Tomizawa, T. Hara, T. Ishikawa, K. Ogawa, H. Tanaka, T. Tanaka, T. Togashi, K. Togawa, M. Yabashi, M. Aoyama, K. Yamakawa, A. Iwasaki, S. Owada, T. Sato, K. Yamanouchi, S. Matsubara, Y. Okayasu, T. Watanabe, E. J. Takahashi, M. Aoyama, A. Iwasaki, S. Owada, H. Minamide, T. Matsukaw
  • Organizer: the 35th International Free Electron Laser Conference
  • Place of Presentation: Manhattan, USA
• [Presentation] Development of cutting-edge terahertz-wave source and detection using a nonlinear optical effect (2013)
  • Author(s): Hiroaki Minamide
  • Organizer: RIKEN Metamaterials Symposium 2012
  • Place of Presentation: Wako, Jaan
  • Invited
• [Presentation] テラヘルツ波の発生と検出 -テラヘルツ波と光波の間を自在に変換- (2013)
  • Author(s): 南出泰亜
  • Organizer: 学術講演会
  • Place of Presentation: 福島県、日本大学
  • Invited
• [Presentation] Ultra-broadband Terahertz generation and detection using a nonlinear optical effect (2012)
  • Author(s): Hiroaki Minamide, Hiromasa Ito
  • Organizer: Laser Seminer
  • Place of Presentation: ETH Zurich, Switzerland
  • Invited
• [Presentation] Terahertz-wave generation and detection using organic nonlinear optical crystals (2012)
  • Author(s): Hiroaki Minamide
  • Organizer: Electronics and Telecommunications Research Institute (ETRI) THz Seminar
  • Place of Presentation: Daejeon, Korea
  • Invited
• [Presentation] Tunable and high peak-power Terahertz-wave generation using nonlinear optical wavelength-conversion (2012)
  • Author(s): Hiroaki Minamide
  • Organizer: Korea Advanced Institute of Science and Technology (KAIST) THz Seminar
  • Place of Presentation: Daejeon, Korea
  • Invited
• [Presentation] High peak-power, tunable terahertz-wave generation and sensitive detection using nonlinear optical wavelength-conversion (2012)
  • Author(s): Hiroaki Minamide
  • Organizer: 2012 THz workshop
  • Place of Presentation: Seoul, Korea
  • Invited
• [Presentation] High-power and Tunable Terahertz-wave Generation and Sensitive Detection by using Nonlinear Parametric Conversion (2012)
  • Author(s): Shin'ichiro Hayashi, Koji Nawata, Kodo Kawase, Hiroaki Minamide
  • Organizer: 37th International conference on infrared, millimeter and terahertz waves (IRMMW-THz 2012)
  • Place of Presentation: University of Wollongong, Australia
  • Invited
• [Presentation] Efficient frequency conversion between light and terahertz waves (2012)
  • Author(s): H. Ito, S. Hayashi, H. Minamide
  • Organizer: 50 Years of Nonlinear Optics, International Symposium
  • Place of Presentation: Barcelona, Spain
  • Invited
• [Presentation] Highly efficient THz-wave parametric generation and detection (2012)
  • Author(s): K. Kawase, S. Hayashi H. Minamide
  • Organizer: International Symposium on Frontiers in THz Technology (FTT 2012)
  • Place of Presentation: Nara, Japan
  • Invited
• [Presentation] 有機非線形光学結晶の光損傷下での繰り返し周波数及びパルス幅依存性 (2012)
  • Author(s): 松川健, 縄田 耕二, 野竹 孝志, 祁 峰, 川俣 大志, 南出 泰亜
  • Organizer: 第73回応用物理学会学術講演会
  • Place of Presentation: 愛媛県、愛媛大学