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Fabrication of single-crystalline AlN layer using a novel LPE technique and discussion of the growth mechanism

Research Project

Project/Area Number 24760611
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeMulti-year Fund
Research Field Metal making engineering
Research InstitutionTohoku University

Principal Investigator

ADACHI Masayoshi  東北大学, 多元物質科学研究所, 助教 (90598913)

Project Period (FY) 2012-04-01 – 2014-03-31
Project Status Completed (Fiscal Year 2013)
Budget Amount *help
¥4,550,000 (Direct Cost: ¥3,500,000、Indirect Cost: ¥1,050,000)
Fiscal Year 2013: ¥1,820,000 (Direct Cost: ¥1,400,000、Indirect Cost: ¥420,000)
Fiscal Year 2012: ¥2,730,000 (Direct Cost: ¥2,100,000、Indirect Cost: ¥630,000)
Keywords窒化アルミニウム / 液相成長 / Ga-Alフラックス / 結晶育成 / 窒化アルニミウム
Research Abstract

AlN is a promising substrate material for AlGaN-based deep UV-LED. Recently, authors investigate an original liquid phase epitaxial growth technique using Ga-Al solution. In this study, it was clarified the role of oxygen in the liquid phase epitaxy technique, and, based on the results, growth mechanism of this technique was discussed. Moreover, we have attempted to grow AlN on nitrided a-plane sapphire template. In consequence, high-quality AlN layer successfully grew using nitrided a-plane sapphire.

Report

(3 results)
  • 2013 Annual Research Report   Final Research Report ( PDF )
  • 2012 Research-status Report
  • Research Products

    (41 results)

All 2014 2013 2012

All Journal Article (2 results) (of which Peer Reviewed: 2 results) Presentation (36 results) (of which Invited: 3 results) Patent(Industrial Property Rights) (3 results)

  • [Journal Article] High-quality AlN layer homoepitaxially grown on nitrided a-plane sapphire2013

    • Author(s)
      Masayoshi Adachi, Kenji Tsuda, Masashi Sugiyama, Junji Iida, Akikazu Tanaka, and Hiroyuki Fukuyama
    • Journal Title

      Applied Physics Express

      Volume: 6 Issue: 9 Pages: 91001-3

    • DOI

      10.7567/apex.6.091001

    • Related Report
      2013 Annual Research Report 2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Analysis of the Dislocation and polarity in an AlN layer grown using Ga-Al flux2012

    • Author(s)
      Masayoshi Adachi, Mari Takasugi, Daisuke Morikawa, Kenji Tsuda, Akikazu Tanaka, Hiroyuki Fukuyama
    • Journal Title

      Applied Physics express

      Volume: vol.5 Issue: 10 Pages: 101001-3

    • DOI

      10.1143/apex.5.101001

    • NAID

      40019455578

    • Related Report
      2013 Final Research Report 2012 Research-status Report
    • Peer Reviewed
  • [Presentation] Ga-Al液相法を用いた窒化サファイア基板上AlN膜成長2014

    • Author(s)
      安達正芳,福山博之,杉山正史,飯田潤二
    • Organizer
      日本鉄鋼協会
    • Place of Presentation
      東京
    • Year and Date
      2014-03-22
    • Related Report
      2013 Final Research Report
  • [Presentation] 固液界面制御による単結晶AlN膜の結晶成長2014

    • Author(s)
      福山博之,安達正芳
    • Organizer
      日本金属学会
    • Place of Presentation
      東京
    • Year and Date
      2014-03-22
    • Related Report
      2013 Final Research Report
  • [Presentation] Al極性AlN膜基板上への低酸素分圧下におけるAlN膜液相成長2014

    • Author(s)
      関谷竜太,安達正芳,大塚誠,福山博之
    • Organizer
      日本金属学会
    • Place of Presentation
      東京
    • Year and Date
      2014-03-22
    • Related Report
      2013 Final Research Report
  • [Presentation] Ga-Al液相法を用いた窒化サファイア基板上AlN膜成長2014

    • Author(s)
      安達正芳,福山博之,杉山正史,飯田潤二
    • Organizer
      日本鉄鋼協会 第167回春季講演大会
    • Place of Presentation
      東京
    • Related Report
      2013 Annual Research Report
  • [Presentation] 固液界面制御による単結晶AlN膜の結晶成長2014

    • Author(s)
      福山博之,安達正芳
    • Organizer
      日本金属学会 2014春季講演大会
    • Place of Presentation
      東京
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Al極性AlN膜基板上への低酸素分圧下におけるAlN膜液相成長2014

    • Author(s)
      関谷竜太,安達正芳,大塚誠,福山博之
    • Organizer
      日本金属学会 2014年春季講演大会
    • Place of Presentation
      東京
    • Related Report
      2013 Annual Research Report
  • [Presentation] Ga-Alを用いたAlNの液相成長における結晶極性と成長機構2013

    • Author(s)
      安達正芳,杉山正史,飯田潤二,田中明和,福山博之
    • Organizer
      日本結晶成長学会
    • Place of Presentation
      長野
    • Year and Date
      2013-11-07
    • Related Report
      2013 Final Research Report
  • [Presentation] Ga-Alフラックスを用いたAlNの液相エピタキシャル成長法の開発2013

    • Author(s)
      安達正芳,福山博之,杉山正史,飯田潤二,田中明和
    • Organizer
      日本金属学会
    • Place of Presentation
      金沢
    • Year and Date
      2013-09-19
    • Related Report
      2013 Final Research Report
  • [Presentation] 大気中熱処理によるa面サファイア基板の表面性状の変化と表面窒化に及ぼす影響2013

    • Author(s)
      関谷竜太,安達正芳,大塚誠,福山博之
    • Organizer
      日本金属学会
    • Place of Presentation
      金沢
    • Year and Date
      2013-09-19
    • Related Report
      2013 Final Research Report
  • [Presentation] Liquid phase epitaxial growth of AlN on nitrided sapphire substrate using Ga-Al solution2013

    • Author(s)
      Masayoshi Adachi, Mari Takasugi, Masashi Sugiyama, Junji Iida, Akikazu Tanaka, Hiroyuki Fukuyama
    • Organizer
      2013JSAP-MRS Joint Symposia
    • Place of Presentation
      京都
    • Year and Date
      2013-09-18
    • Related Report
      2013 Final Research Report
  • [Presentation] Polarity inversion and growth mechanism of AlN layer grown on nitrided sapphire using Ga-Al flux2013

    • Author(s)
      Masayoshi Adachi,Mari Takasugi,Masashi Sugiyama, Junji Iida, Akikazu Tanaka, Hiroyuki Fukuyama
    • Organizer
      10th International Conference on Nitrided Semiconductors
    • Place of Presentation
      アメリカ,ワシントンDC
    • Year and Date
      2013-08-28
    • Related Report
      2013 Final Research Report
  • [Presentation] Ga-Al液相成長法により成長したAlNの極性と成長メカニズム2013

    • Author(s)
      安達正芳,高杉茉里,杉山正史,飯田潤二,田中明和,福山博之
    • Organizer
      日本結晶成長学会ナノ構造エピタキシャル成長分科会
    • Place of Presentation
      大阪
    • Year and Date
      2013-06-21
    • Related Report
      2013 Final Research Report
  • [Presentation] Ga-Al solution growth of high-quality AlN on nitrided a-plane sapphire2013

    • Author(s)
      Masayoshi Adachi, Kenji Tsuda, Masashi Sugiyama, Junji Iida, Akikazu Tanaka, Hiroyuki Fukuyama
    • Organizer
      The Sixth Asia-Pacific Workshop on Widegap Semiconductors
    • Place of Presentation
      台湾,淡水
    • Year and Date
      2013-05-14
    • Related Report
      2013 Final Research Report
  • [Presentation] Ga-Al液相法により成長したAlN膜の極性反転構造2013

    • Author(s)
      安達正芳,津田健治,渡邊郁磨,杉山正史,飯田潤二,田中明和,福山博之
    • Organizer
      応用物理学会
    • Place of Presentation
      神奈川
    • Year and Date
      2013-03-28
    • Related Report
      2013 Final Research Report
  • [Presentation] Growth of high quality AlN layer and its polarity control by LPE using Ga-Al flux2013

    • Author(s)
      Hiroyuki Fukuyama, Masayoshi Adachi, Mari Takasugi, Masashi Sugiyama, Junji Iida, Akikazu Tanaka
    • Organizer
      Photonics West-OPTO
    • Place of Presentation
      アメリカ,サンフランシスコ
    • Year and Date
      2013-02-04
    • Related Report
      2013 Final Research Report
  • [Presentation] Ga-Al solution growth of high-quality AlN on nitrided a-plane sapphire2013

    • Author(s)
      Masayoshi Adachi, Kenji Tsuda, Masashi Sugiyama, Junji Iida, Akikazu Tanaka, and Hiroyuki Fukuyama
    • Organizer
      The Sixth Asia-Pacific Workshop on Widegap Semiconductors (APWS 2013)
    • Place of Presentation
      Tamsui, Taiwan
    • Related Report
      2013 Annual Research Report
  • [Presentation] Polarity inversion and growth mechanism of AlN layer grown on nitrided sapphire using Ga-Al flux2013

    • Author(s)
      Masayoshi Adachi, Mari Takasugi, Masashi Sugiyama, Junji Iida, Akikazu Tanaka, and Hiroyuki Fukuyama
    • Organizer
      10th International Conference on Nitride Semiconductors
    • Place of Presentation
      Washington, DC, USA
    • Related Report
      2013 Annual Research Report
  • [Presentation] Liquid phase epitaxial growth of AlN on nitirded sapphire substrate using Ga-Al solution2013

    • Author(s)
      Masayoshi Adachi, Masashi Sugiyama, Junji Iida, Akikazu Tanaka, and Hiroyuki Fukuyama
    • Organizer
      2013 JSAP-MRS Joint Symposia
    • Place of Presentation
      Kyoto, Japan
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Ga-Al液相成長法により成長したAlNの極性と成長メカニズム2013

    • Author(s)
      安達正芳,高杉茉里,杉山正史,飯田潤二,田中明和,福山博之
    • Organizer
      日本結晶成長学会 ナノ構造・エピタキシャル成長分科会 2013春季講演会
    • Place of Presentation
      大阪
    • Related Report
      2013 Annual Research Report
  • [Presentation] Ga-Alフラックスを用いたAlNの液相エピタキシャル成長法の開発2013

    • Author(s)
      安達正芳,福山博之,杉山正史,飯田潤二,田中明和
    • Organizer
      日本金属学会 2013秋季講演大会
    • Place of Presentation
      金沢
    • Related Report
      2013 Annual Research Report
  • [Presentation] 大気中熱処理によるa面サファイア基板の表面性状の変化と表面窒化に及ぼす影響2013

    • Author(s)
      関谷竜太,安達正芳,大塚誠,福山博之
    • Organizer
      日本金属学会 2013秋季講演大会
    • Place of Presentation
      金沢
    • Related Report
      2013 Annual Research Report
  • [Presentation] Ga-Alを用いたAlNの液相成長における結晶極性と成長機構2013

    • Author(s)
      安達正芳,杉山正史,飯田潤二,田中明和,福山博之
    • Organizer
      日本結晶成長学会 結晶成長国内会議
    • Place of Presentation
      長野
    • Related Report
      2013 Annual Research Report
  • [Presentation] Growth of high quality AlN layer and its polarity control by LPE using Ga-Al flux2013

    • Author(s)
      Hiroyuki Fukuyama, Masayoshi Adachi, Mari Takasugi, Masashi Sugiyama, Junji Iida, and Akikazu Tanaka
    • Organizer
      Photonics West-OPTO
    • Place of Presentation
      San Francisco, USA
    • Related Report
      2012 Research-status Report
    • Invited
  • [Presentation] Ga-Al液相法により成長したAlN膜の極性反転構造2013

    • Author(s)
      安達正芳,津田健治,渡邊郁磨,杉山正史,飯田潤二,田中明和,福山博之
    • Organizer
      2013年春季 第60回応用物理学会学術講演会
    • Place of Presentation
      神奈川
    • Related Report
      2012 Research-status Report
  • [Presentation] High quality AlN layer homoepitaxially grown on nitrided a-plane sapphire using Ga-Al flux2012

    • Author(s)
      Masayoshi Adachi, Masashi Sugiyama, Akikazu Tanaka, Hiroyuki Fukuyama
    • Organizer
      International Workshop on Nitride Semiconductors
    • Place of Presentation
      札幌
    • Year and Date
      2012-10-18
    • Related Report
      2013 Final Research Report
  • [Presentation] Influence of oxygen partial pressure on the growth of aluminum nitride layer using Ga-Al flux2012

    • Author(s)
      Mari Takasugi, Masayoshi Adachi, Masashi Sugiyama, Akikazu Tanaka, Hiroyuki Fukuyama
    • Organizer
      International Workshop on Nitride Semiconductors
    • Place of Presentation
      札幌
    • Year and Date
      2012-10-18
    • Related Report
      2013 Final Research Report
  • [Presentation] Ga-Alフラックスを用いた窒化a面サファイア基板上への高品質AlN成長2012

    • Author(s)
      安達正芳,杉山正史,田中明和,福山博之
    • Organizer
      応用物理学会
    • Place of Presentation
      愛媛
    • Year and Date
      2012-09-13
    • Related Report
      2013 Final Research Report
  • [Presentation] Ga-Al液相成長法を用いたAlN成長における酸素分圧の影響2012

    • Author(s)
      高杉茉里,安達正芳,杉山正史,田中明和,福山博之
    • Organizer
      応用物理学会
    • Place of Presentation
      愛媛
    • Year and Date
      2012-09-13
    • Related Report
      2013 Final Research Report
  • [Presentation] Annealing effect for unification of in-plane domain in AlN layers grown from Ga-Al flux2012

    • Author(s)
      Masayoshi Adachi, Masashi Sugiyama, Akikazu Tanaka, Hiroyuki Fukuyama
    • Organizer
      International Symposium on Growth of III-Nitrides
    • Place of Presentation
      サンクトペテルブルグ,ロシア
    • Year and Date
      2012-07-17
    • Related Report
      2013 Final Research Report
  • [Presentation] Effect of oxygen partial pressure on the growth of single-crystalline aluminum nitride layer using liquid phase epitaxy technique2012

    • Author(s)
      Mari Takasugi, Masayoshi Adachi, Masashi Sugiyama, Akikazu Tanaka, Hiroyuki Fukuyama
    • Organizer
      International Symposium on Growth of III-Nitrides
    • Place of Presentation
      サンクトペテルブルグ,ロシア
    • Year and Date
      2012-07-17
    • Related Report
      2013 Final Research Report
  • [Presentation] Annealing effect for unification of in-plane domain in AlN layers grown from Ga-Al flux2012

    • Author(s)
      Masayoshi Adachi, Masashi Sugiyama, Akikazu Tanaka, and Hiroyuki Fukuyama
    • Organizer
      International Symposium On Growth of III-Nitrides (ISGN)
    • Place of Presentation
      St. Petersburg, Russia
    • Related Report
      2012 Research-status Report
  • [Presentation] Effect of oxygen partial pressure on the growth of single-crystalline aluminum nitride layer using liquid phase epitaxy technique2012

    • Author(s)
      Mari Takasugi, Masayoshi Adachi, Masashi Sugiyama, Akikazu Tanaka, and Hiroyuki Fukuyama
    • Organizer
      International Symposium On Growth of III-Nitrides (ISGN)
    • Place of Presentation
      St. Petersburg, Russia
    • Related Report
      2012 Research-status Report
  • [Presentation] High quality AlN layer homoepitaxially grown on nitrided a-plane sapphire using Ga-Al flux2012

    • Author(s)
      Masayoshi Adachi, Masashi Sugiyama, Akikazu Tanaka, and Hiroyuki Fukuyama
    • Organizer
      International Workshop on Nitride semiconductor (IWN)
    • Place of Presentation
      札幌
    • Related Report
      2012 Research-status Report
  • [Presentation] Influence of oxygen partial pressure on the growth of aluminum nitride layer using Ga-Al flux2012

    • Author(s)
      Mari Takasugi, Masayoshi Adachi, Masashi Sugiyama, Akikazu Tanaka, and Hiroyuki Fukuyama
    • Organizer
      International Workshop on Nitride semiconductor (IWN)
    • Place of Presentation
      札幌
    • Related Report
      2012 Research-status Report
  • [Presentation] Ga-Alフラックスを用いた窒化a面サファイア基板上への高品質AlN成長2012

    • Author(s)
      安達正芳,杉山正史,田中明和,福山博之
    • Organizer
      2012年秋季 第73回応用物理学会学術講演会
    • Place of Presentation
      松山
    • Related Report
      2012 Research-status Report
  • [Presentation] Ga-Al液相成長法を用いたAlN成長における酸素分圧の影響2012

    • Author(s)
      高杉茉里,安達正芳,杉山正史,田中明和,福山博之
    • Organizer
      2012年秋季 第73回応用物理学会学術講演会
    • Place of Presentation
      松山
    • Related Report
      2012 Research-status Report
  • [Patent(Industrial Property Rights)] 窒化アルミニウム結晶の製造方法2013

    • Inventor(s)
      大保安宏,杉山正史,飯田潤二,福山博之,安達正芳
    • Industrial Property Number
      2013-111290
    • Filing Date
      2013-05-27
    • Related Report
      2013 Final Research Report
  • [Patent(Industrial Property Rights)] 窒化アルミニウム結晶の製造方法2013

    • Inventor(s)
      福山博之,安達正芳,飯田潤二,杉山正史,大保安宏
    • Industrial Property Number
      2013-156766
    • Filing Date
      2013-07-29
    • Related Report
      2013 Final Research Report
  • [Patent(Industrial Property Rights)] 窒化アルミニウム結晶の製造方法2013

    • Inventor(s)
      福山博之,安達正芳,飯田潤二,杉山正史,大保安宏
    • Industrial Property Number
      2013-261161
    • Filing Date
      2013-12-18
    • Related Report
      2013 Final Research Report

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Published: 2013-05-31   Modified: 2019-07-29  

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