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Design of high efficiency electrolysis cell for liquid ammonia utilization as hydrogen storage carrier

Research Project

Project/Area Number 24760726
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeMulti-year Fund
Research Field Energy engineering
Research InstitutionUniversity of Tsukuba

Principal Investigator

HANADA Nobuko  筑波大学, システム情報系, 助教 (00606634)

Project Period (FY) 2012-04-01 – 2014-03-31
Project Status Completed (Fiscal Year 2013)
Budget Amount *help
¥4,420,000 (Direct Cost: ¥3,400,000、Indirect Cost: ¥1,020,000)
Fiscal Year 2013: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2012: ¥3,380,000 (Direct Cost: ¥2,600,000、Indirect Cost: ¥780,000)
Keywords水素貯蔵媒体 / 液体アンモニア / 水素生成 / 電気分解 / 過電圧低減 / 電気めっき
Research Abstract

The overvoltage reduction effects of electrode morphology and materials on liquid ammonia electrolysis were investigated to design high efficiency electrolysis cell for generating hydrogen from liquid ammonia. For Pt-black electrodes prepared by electrodeposition, it is clarified that the overvoltage reduction does not relate to the electrode surface area, but relates to both of Pt deposition amount and size of deposited Pt particles. For the electrolysis by using Pt plate electrode, anode overvoltage is five times as large as cathode one. Ammonia electrolysis with the emission of hydrogen gas was performed at 0.1 V around theoretical electrolysis voltage by adapting Pt-Ru electrode which can reduce the anode overvoltage.

Report

(3 results)
  • 2013 Annual Research Report   Final Research Report ( PDF )
  • 2012 Research-status Report
  • Research Products

    (11 results)

All 2014 2013 2012 Other

All Presentation (11 results) (of which Invited: 3 results)

  • [Presentation] Hydrogen generation by electrolysis of liquid ammonia2014

    • Author(s)
      Nobuko Hanada
    • Organizer
      6^<th> Forum on New Materials
    • Place of Presentation
      Montecatini Terme, Italy
    • Year and Date
      2014-06-16
    • Related Report
      2013 Final Research Report
    • Invited
  • [Presentation] 液体アンモニア電気分解へのRu電極触媒適用による過電圧低減2014

    • Author(s)
      北川卓, 花田信子, 石田政義
    • Organizer
      2014年電気化学会第81回大会
    • Place of Presentation
      関西大学
    • Year and Date
      2014-03-31
    • Related Report
      2013 Final Research Report
  • [Presentation] Hydrogen generation by electrolysis of liquid ammonia2014

    • Author(s)
      Nobuko Hanada
    • Organizer
      6th Forum on New Materials
    • Place of Presentation
      Montecatini Terme, Italy
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Reduction of electrolysis voltage of liquid ammonia for hydrogen generation2013

    • Author(s)
      Nobuko Hanada, Rai Dan, Suguru Kitagawa, Masayoshi Ishida, Takayuki Ichikawa and Yoshitsugu Kojima
    • Organizer
      THERMEC'2013
    • Place of Presentation
      Rio Hotel, Las Vegas, USA
    • Year and Date
      2013-12-06
    • Related Report
      2013 Annual Research Report 2013 Final Research Report
    • Invited
  • [Presentation] 液体アンモニア電気分解におけるアノード及びカソード反応での過電圧特性評価2013

    • Author(s)
      段磊, 花田信子, 石田政義
    • Organizer
      化学工学会第45回秋季大会
    • Place of Presentation
      岡山大学
    • Year and Date
      2013-09-18
    • Related Report
      2013 Final Research Report
  • [Presentation] 液体アンモニア電気分解への白金黒電極適用による過電圧の低減2013

    • Author(s)
      北川卓, 花田信子, 石田政義, 市川貴之, 小島由継
    • Organizer
      2013年電気化学会第80回大会
    • Place of Presentation
      東北大学
    • Year and Date
      2013-03-31
    • Related Report
      2013 Final Research Report
  • [Presentation] 液体アンモニア電気分解における電気化学特性2012

    • Author(s)
      花田信子, 段磊, 北川卓, 石田政義, 市川貴之, 小島由継
    • Organizer
      化学工学会第44回秋季大会
    • Place of Presentation
      東北大学
    • Year and Date
      2012-09-21
    • Related Report
      2013 Final Research Report
  • [Presentation] 液体アンモニア電気分解におけるアノード及びカソード反応での過電圧特性評価

    • Author(s)
      段磊、花田信子、石田政義
    • Organizer
      化学工学会第45回秋季大会
    • Place of Presentation
      岡山大学
    • Related Report
      2013 Annual Research Report
  • [Presentation] 液体アンモニア電気分解へのRu電極触媒適用による過電圧低減

    • Author(s)
      北川卓、花田信子、石田政義
    • Organizer
      2014年電気化学会第81回大会
    • Place of Presentation
      関西大学千里山キャンパス
    • Related Report
      2013 Annual Research Report
  • [Presentation] 液体アンモニア電気分解の遷移金属電極における電気化学特性

    • Author(s)
      花田信子、段磊、北川卓、石田政義、市川貴之、小島由継
    • Organizer
      化学工学会第44回秋季大会
    • Place of Presentation
      東北大学川内キャンパス
    • Related Report
      2012 Research-status Report
  • [Presentation] 液体アンモニア電気分解への白金黒電極適用による過電圧の低減

    • Author(s)
      北川卓、花田信子、石田政義、市川貴之、小島由継
    • Organizer
      2013年電気化学会第80回大会
    • Place of Presentation
      東北大学川内キャンパス
    • Related Report
      2012 Research-status Report

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Published: 2013-05-31   Modified: 2019-07-29  

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