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Domain Structure and High-load Resistance of Lead-free Niobate Piezoelectrics

Research Project

Project/Area Number 25289227
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypePartial Multi-year Fund
Section一般
Research Field Inorganic materials/Physical properties
Research InstitutionNagoya Institute of Technology

Principal Investigator

KAKIMOTO Ken-ichi  名古屋工業大学, 工学(系)研究科(研究院), 教授 (40335089)

Project Period (FY) 2013-04-01 – 2016-03-31
Project Status Completed (Fiscal Year 2015)
Budget Amount *help
¥18,720,000 (Direct Cost: ¥14,400,000、Indirect Cost: ¥4,320,000)
Fiscal Year 2015: ¥3,380,000 (Direct Cost: ¥2,600,000、Indirect Cost: ¥780,000)
Fiscal Year 2014: ¥7,280,000 (Direct Cost: ¥5,600,000、Indirect Cost: ¥1,680,000)
Fiscal Year 2013: ¥8,060,000 (Direct Cost: ¥6,200,000、Indirect Cost: ¥1,860,000)
Keywords環境材料 / セラミックス / 電子・電気材料 / 無鉛圧電体 / ドメイン構造
Outline of Final Research Achievements

Spectrophotometric techniques including Raman and infrared spectroscopies enabled to characterize the domain structure in lead-free niobate piezoelectric materials, and confirmed that a permittivity increased significantly in the vicinity of domain walls.
Based on the above fact, a manufacturing process was also improved successfully to synthesize the high-density ceramics having controlled microstructures, which could demonstrate excellent high-load resistances against elevated temperature and applied electrical field.

Report

(4 results)
  • 2015 Annual Research Report   Final Research Report ( PDF )
  • 2014 Annual Research Report
  • 2013 Annual Research Report
  • Research Products

    (58 results)

All 2016 2015 2014 2013 Other

All Int'l Joint Research (2 results) Journal Article (6 results) (of which Peer Reviewed: 6 results,  Acknowledgement Compliant: 4 results,  Open Access: 3 results) Presentation (50 results) (of which Int'l Joint Research: 2 results,  Invited: 7 results)

  • [Int'l Joint Research] Univ. Erlangen-Nuremberg(ドイツ)

    • Related Report
      2015 Annual Research Report
  • [Int'l Joint Research]

    • Related Report
      2015 Annual Research Report
  • [Journal Article] Electric Fatigue Process in Lead-free Alkali Niobate Ceramics at Various Pressures and Temperatures2015

    • Author(s)
      A. Martin and K. Kakimoto
    • Journal Title

      Jpn. J. Appl. Phys.

      Volume: 54 Issue: 10S Pages: 10NB06-10NB06

    • DOI

      10.7567/jjap.54.10nb06

    • NAID

      210000145784

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Microscopic Raman Spectroscopy in the Vicinity of Domain Wall of (Na,K)NbO3 Piezoelectrics2015

    • Author(s)
      Y. Taniguchi and K. Kakimoto
    • Journal Title

      Jpn. J. Appl. Phys.

      Volume: 54 Issue: 10S Pages: 10ND09-10ND09

    • DOI

      10.7567/jjap.54.10nd09

    • NAID

      210000145800

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Lead-free Li-modified (Na,K)NbO<sub>3</sub> piezoelectric ceramics fabricated by two-step sintering method2014

    • Author(s)
      K. Kato, K. Kakimoto, K. Hatano, K. Kobayashi and Y. Doshida
    • Journal Title

      Journal of the Ceramic Society of Japan

      Volume: 122 Issue: 1426 Pages: 460-463

    • DOI

      10.2109/jcersj2.122.460

    • NAID

      130004480252

    • ISSN
      1348-6535, 1882-0743
    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Engineering of Lead-free Piezoelectrics in Alkali Niobate Ceramic System: Improvement in Density by Two-step Mixing Process2014

    • Author(s)
      K. Kakimoto, S. Ishihara and M. Watanabe
    • Journal Title

      Key Eng. Mater.

      Volume: 616 Pages: 108-113

    • DOI

      10.4028/www.scientific.net/kem.616.108

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Effect of Domain Structure on the Mechanical and Piezoelectric Properties of Lead-free Alkali Niobate Ceramics2014

    • Author(s)
      A. Martin and K. Kakimoto
    • Journal Title

      Jpn. J. Appl. Phys.

      Volume: 53 Issue: 9S Pages: 09PB09-09PB09

    • DOI

      10.7567/jjap.53.09pb09

    • NAID

      210000144495

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Effect of Crystal Growth Direction on Domain Structure of Mn-Doped (Na,K)NbO3 Crystal2013

    • Author(s)
      K. Tsuchida, K. Kakimoto, I. Kagomiya
    • Journal Title

      Jpn. J. Appl. Phys.

      Volume: 52 Issue: 9S1 Pages: 09KD02-09KD02

    • DOI

      10.7567/jjap.52.09kd02

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Presentation] Evaluation of Domain Switching by Means of Impedance Spectroscopy Method2016

    • Author(s)
      H. Nishiyama, T. Fuchigami, K. Kakimoto
    • Organizer
      7th U3 Material Design Forum
    • Place of Presentation
      Shizuoka
    • Year and Date
      2016-03-28
    • Related Report
      2015 Annual Research Report
  • [Presentation] ニオブ系無鉛圧電セラミックスの圧縮応力依存性と疲労機構2016

    • Author(s)
      大胡健司、渕上輝顕、柿本健一、M. Weiss, S. Rupitsch, R. Lerch
    • Organizer
      日本セラミックス協会2015年年会
    • Place of Presentation
      東京
    • Year and Date
      2016-03-14
    • Related Report
      2015 Annual Research Report
  • [Presentation] 種々のNb2O5混合粉を用いたニオブ系無鉛圧電セラミックスLNKNの作製とその圧電特性2016

    • Author(s)
      松村栄幸、渕上輝顕、柿本健一
    • Organizer
      日本セラミックス協会2015年年会
    • Place of Presentation
      東京
    • Year and Date
      2016-03-14
    • Related Report
      2015 Annual Research Report
  • [Presentation] 高負荷環境下における圧電セラミックスの電界誘起ひずみ計測2015

    • Author(s)
      大胡健司、渕上輝顕、柿本健一、M. Weiss, S. Rupitsch, R. Lerch
    • Organizer
      平成27年度日本セラミックス協会東海支部学術研究発表会
    • Place of Presentation
      名古屋
    • Year and Date
      2015-12-12
    • Related Report
      2015 Annual Research Report
  • [Presentation] Characterization of Lead-free Alkali Niobate Piezoceramics by the Inverse method2015

    • Author(s)
      K. Ogo, M. Weiss, S. Rupitsch, R. Lerch and K. Kakimoto
    • Organizer
      IEEE International Ultrasonics Symposium
    • Place of Presentation
      Taiwan
    • Year and Date
      2015-10-21
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] インバース法を用いたニオブ系無鉛圧電セラミックスの材料定数評価2015

    • Author(s)
      大胡健司、柿本健一、Manuel Weiss、Stefan Rupitsch、Reinhard Lerch
    • Organizer
      日本セラミックス協会第28回秋季シンポジウム
    • Place of Presentation
      富山
    • Year and Date
      2015-09-16
    • Related Report
      2015 Annual Research Report
  • [Presentation] Spectroscopic Analysis of Domain Structure for Lead-free (Na,K)NbO3 Piezoelectrics2015

    • Author(s)
      Y. Taniguchi and K. Kakimoto
    • Organizer
      11th Pacific Rim Conference of Ceramic Societies
    • Place of Presentation
      Jeju, Korea
    • Year and Date
      2015-08-30
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Electric Fatigue Process of Lead-free Alkari Niobate Ceramics under Pressure and Temperature2015

    • Author(s)
      A. Martin and K. Kakimoto
    • Organizer
      第32回強誘電体応用会議
    • Place of Presentation
      京都
    • Year and Date
      2015-05-20
    • Related Report
      2015 Annual Research Report
  • [Presentation] (Na,K)NbO3無鉛圧電体のドメインウォール近傍における顕微ラマン分光評価2015

    • Author(s)
      谷口優也、柿本健一
    • Organizer
      第32回強誘電体応用会議
    • Place of Presentation
      京都
    • Year and Date
      2015-05-20
    • Related Report
      2015 Annual Research Report
  • [Presentation] Effect of Uniaxial Pressure on the Bipolar Fatigue behaveor of Lead-free Alkali Niobate Ceramics2015

    • Author(s)
      A. Martin and K. Kakimoto
    • Organizer
      6th U3 Materials Design Forum
    • Place of Presentation
      Osaka
    • Year and Date
      2015-03-30 – 2015-03-31
    • Related Report
      2014 Annual Research Report
  • [Presentation] Mechanism of High-temperature Electrical Conduction for (Na,K)NbO3-based Ceramics under DC Bias2015

    • Author(s)
      K. Yoshida and K. Kakimoto
    • Organizer
      6th U3 Materials Design Forum
    • Place of Presentation
      Osaka
    • Year and Date
      2015-03-30 – 2015-03-31
    • Related Report
      2014 Annual Research Report
  • [Presentation] The Poling Process for Porous Piezoelectric Alkali Niobate Ceramics2015

    • Author(s)
      Y. Sumiya and K. Kakimoto
    • Organizer
      6th U3 Materials Design Forum
    • Place of Presentation
      Osaka
    • Year and Date
      2015-03-30 – 2015-03-31
    • Related Report
      2014 Annual Research Report
  • [Presentation] ニオブ系無鉛圧電セラミックスの高温インピーダンス測定2015

    • Author(s)
      加藤淳揮、柿本健一
    • Organizer
      日本セラミックス協会2015年年会
    • Place of Presentation
      岡山
    • Year and Date
      2015-03-18 – 2015-03-20
    • Related Report
      2014 Annual Research Report
  • [Presentation] 顕微ラマン分光法による(Na,K)NbO3セラミックスのドメインウォール評価2015

    • Author(s)
      谷口優也、柿本健一
    • Organizer
      日本セラミックス協会2015年年会
    • Place of Presentation
      岡山
    • Year and Date
      2015-03-18 – 2015-03-20
    • Related Report
      2014 Annual Research Report
  • [Presentation] Characterization of Porous LNKN Ceramics Prepared by Foam Impregnation and Pressing2015

    • Author(s)
      Y. Sumiya, K. Kakimoto, T. Fey and P. Greil
    • Organizer
      4th International Symposium on Ceramics Nanotune Technology
    • Place of Presentation
      Nagoya
    • Year and Date
      2015-03-02 – 2015-03-04
    • Related Report
      2014 Annual Research Report
  • [Presentation] Preparation and Piezoelectric Sensor Characterization of Microporous Alkaliniobate Ceramics2015

    • Author(s)
      A. Stenzel, T. Fey, P. Greil and K. Kakimoto
    • Organizer
      4th International Symposium on Ceramics Nanotune Technology
    • Place of Presentation
      Nagoya
    • Year and Date
      2015-03-02 – 2015-03-04
    • Related Report
      2014 Annual Research Report
  • [Presentation] 圧電動ひずみ計測における試料形状およびロゼット解析2014

    • Author(s)
      大胡健司、柿本健一
    • Organizer
      平成26年度日本セラミックス協会東海支部学術研究発表会
    • Place of Presentation
      名古屋
    • Year and Date
      2014-12-06
    • Related Report
      2014 Annual Research Report
  • [Presentation] (Na,K)Nb03系無鉛圧電体における分光学的ドメインウォール評価2014

    • Author(s)
      谷口優也、柿本健一
    • Organizer
      平成26年度日本セラミックス協会東海支部学術研究発表会
    • Place of Presentation
      名古屋
    • Year and Date
      2014-12-06
    • Related Report
      2014 Annual Research Report
  • [Presentation] Alkali Niobate Perovskite for Lead-free Piezoelectrics2014

    • Author(s)
      K. Kakimoto
    • Organizer
      Materials Science & Technology 2014
    • Place of Presentation
      Pittsburgh, USA
    • Year and Date
      2014-10-12 – 2014-10-16
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] Promotion of the Wet Etching Reaction in Lead-free Alkali Niobate Piezoelectric Ceramics by Ultarviolet Irradiation2014

    • Author(s)
      Y. Sumiya and K. Kakimoto
    • Organizer
      6th International Workshop on Advanced Ceramics
    • Place of Presentation
      Erlangen, Germany
    • Year and Date
      2014-09-28 – 2014-09-30
    • Related Report
      2014 Annual Research Report
  • [Presentation] Estimation of Various Mechanical Characteristics of Differently Poled Lead-free Lix(Na0.5K0.5)1-xNbO32014

    • Author(s)
      A. Martin and K. Kakimoto
    • Organizer
      6th International Workshop on Advanced Ceramics
    • Place of Presentation
      Erlangen, Germany
    • Year and Date
      2014-09-28 – 2014-09-30
    • Related Report
      2014 Annual Research Report
  • [Presentation] Non-contact Piezoelectric Evaluation by Using Laser Doppler Vibrometer2014

    • Author(s)
      K. Ogo and K. Kakimoto
    • Organizer
      6th International Workshop on Advanced Ceramics
    • Place of Presentation
      Erlangen, Germany
    • Year and Date
      2014-09-28 – 2014-09-30
    • Related Report
      2014 Annual Research Report
  • [Presentation] ニオブ系無鉛圧電セラミックスの紫外線励起電子によるエッチング効果2014

    • Author(s)
      角谷裕太、柿本健一
    • Organizer
      日本セラミックス協会第27回秋季シンポジウム
    • Place of Presentation
      鹿児島
    • Year and Date
      2014-09-09 – 2014-09-11
    • Related Report
      2014 Annual Research Report
  • [Presentation] レーザドップラ振動計を用いた電界誘起ひずみ評価2014

    • Author(s)
      大胡健司、柿本健一
    • Organizer
      日本セラミックス協会第27回秋季シンポジウム
    • Place of Presentation
      鹿児島
    • Year and Date
      2014-09-09 – 2014-09-11
    • Related Report
      2014 Annual Research Report
  • [Presentation] Poling Field Dependence on Mechanical Property of Li-modified (Na,K)NbO32014

    • Author(s)
      A. Martin and K. Kakimoto
    • Organizer
      平成27年度関西中部誘電体セミナー
    • Place of Presentation
      名古屋
    • Year and Date
      2014-07-26
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] ニオブ系無鉛圧電体に関する研究2014

    • Author(s)
      柿本健一
    • Organizer
      フルラス・岡崎記念会2014年度講演会
    • Place of Presentation
      東京
    • Year and Date
      2014-06-19
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] Influence of Domain Structure on the Mechanical and Piezoelectric Properties of Lead-free Alkali Niobate Ceramics2014

    • Author(s)
      A. Martin and K. Kakimoto
    • Organizer
      第31回強誘電体応用会議
    • Place of Presentation
      京都
    • Year and Date
      2014-05-28 – 2014-05-31
    • Related Report
      2014 Annual Research Report
  • [Presentation] ニオブ系無鉛圧電セラミックスの粒子サイズ制御2014

    • Author(s)
      加藤健佑、柿本健一、波多野桂一、小林圭介、土信田豊
    • Organizer
      第52回セラミックス基礎科学討論会
    • Place of Presentation
      名古屋
    • Related Report
      2013 Annual Research Report
  • [Presentation] Impedance Spectroscopy and Material Design of Lead-free Alkali Niobate Piezoelectric Ceramics2014

    • Author(s)
      M. Watanabe, K. Kakimoto, I. Kagomiya
    • Organizer
      Electronic Materials and Applications 2014
    • Place of Presentation
      Florida, USA
    • Related Report
      2013 Annual Research Report
  • [Presentation] Piezoelectric Properties of Lead-free Niobate Ceramics with Controlled Grain Size2014

    • Author(s)
      K. Kato, K. Kakimoto, K. Hatano, K. Kobayashi, Y. Doshida
    • Organizer
      Electronic Materials and Applications 2014
    • Place of Presentation
      Florida, USA
    • Related Report
      2013 Annual Research Report
  • [Presentation] Processing and Microstructural Control of (Na,K)NbO3-based Lead-free Piezoceramics2014

    • Author(s)
      K. Kakimoto
    • Organizer
      Electronic Materials and Applications 2014
    • Place of Presentation
      Florida, USA
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Mechanical Properties of Lead-free Alkali Niobate Ceramics2014

    • Author(s)
      A. Martin, K. Kakimoto
    • Organizer
      3rd Int. Symp.on Ceram. Nanotune Techn.
    • Place of Presentation
      Nagoya, Japan
    • Related Report
      2013 Annual Research Report
  • [Presentation] 偏光ラマン分光による(Na,K)NbO3のドメイン構造評価2014

    • Author(s)
      谷口優也、柿本健一
    • Organizer
      日本セラミックス協会2014年年会
    • Place of Presentation
      横浜
    • Related Report
      2013 Annual Research Report
  • [Presentation] レーザドップラ振動計を用いた非接触圧電特性評価2014

    • Author(s)
      大胡健司、柿本健一
    • Organizer
      第5回U3マテリアルデザインフォーラム
    • Place of Presentation
      下呂
    • Related Report
      2013 Annual Research Report
  • [Presentation] ニオブ系無鉛圧電セラミックスのエッチング処理およびドメイン構造観察2014

    • Author(s)
      角谷裕太、柿本健一
    • Organizer
      第5回U3マテリアルデザインフォーラム
    • Place of Presentation
      下呂
    • Related Report
      2013 Annual Research Report
  • [Presentation] 偏光ラマン分光による(Na,K)NbO3のドメイン構造評価2014

    • Author(s)
      谷口優也、柿本健一
    • Organizer
      日本セラミックス協会2014年年会
    • Place of Presentation
      下呂
    • Related Report
      2013 Annual Research Report
  • [Presentation] (Na,K)NbO3圧電結晶の育成とドメイン構造2013

    • Author(s)
      土田貢平、柿本健一、籠宮 功
    • Organizer
      第30回強誘電体応用会議
    • Place of Presentation
      京都
    • Related Report
      2013 Annual Research Report
  • [Presentation] Challenges for Lead-free Piezoelectric Ceramics in Alkali Niobate System2013

    • Author(s)
      K. Kakimoto
    • Organizer
      10th Pacific Rim Conf. on Ceram and Glass Techn.
    • Place of Presentation
      Calfolnia, USA
    • Related Report
      2013 Annual Research Report
  • [Presentation] Engineering of Lead-free Piezoelectric (Na,K)NbO3 Ceramics and Film via Aqueous-based Chelate Precurso2013

    • Author(s)
      K. Kakimoto, K. Hattori, I. Kagomiya
    • Organizer
      13th Int. Conf. of the Eur. Ceram. Soc.
    • Place of Presentation
      Limoges, France
    • Related Report
      2013 Annual Research Report
  • [Presentation] Ceramic Processing and Evaluation of (Na,K)NbO3-based Lead-free Piezoelectrics2013

    • Author(s)
      K. Kakimoto
    • Organizer
      12th Int. Conf. on Ceram. Processing Sci.
    • Place of Presentation
      Oregon, USA
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] ニオブ系無鉛圧電セラミックスの粒子サイズ効果2013

    • Author(s)
      加藤健佑、柿本健一、波多野桂一、小林圭介、土信田豊
    • Organizer
      日本セラミックス協会第26回秋季シンポジウム
    • Place of Presentation
      長野
    • Related Report
      2013 Annual Research Report
  • [Presentation] 固体NMRに基づく無鉛圧電材料LNKNセラミックスの局所構造解析2013

    • Author(s)
      山崎哲平、柿本健一
    • Organizer
      日本セラミックス協会第26回秋季シンポジウム
    • Place of Presentation
      長野
    • Related Report
      2013 Annual Research Report
  • [Presentation] ニオブ系無鉛圧電セラミックスのインピーダンス特性2013

    • Author(s)
      渡邉桃子、柿本健一、籠宮 功
    • Organizer
      日本セラミックス協会第26回秋季シンポジウム
    • Place of Presentation
      長野
    • Related Report
      2013 Annual Research Report
  • [Presentation] 粒子サイズ制御した(Li,Na,K)NbO3セラミックスの圧電特性2013

    • Author(s)
      加藤健佑、柿本健一、波多野桂一、小林圭介、土信田豊
    • Organizer
      第33回エレクトロセラミックス研究討論会
    • Place of Presentation
      つくば
    • Related Report
      2013 Annual Research Report
  • [Presentation] ニオブ系無鉛圧電セラミックスの高温導電性2013

    • Author(s)
      渡邉桃子、柿本健一、籠宮 功
    • Organizer
      第33回エレクトロセラミックス研究討論会
    • Place of Presentation
      つくば
    • Related Report
      2013 Annual Research Report
  • [Presentation] 無鉛圧電セラミックスの多機能性:電子部品から創エネルギーおよび医用材料2013

    • Author(s)
      柿本健一
    • Organizer
      粉体粉末冶金協会平成25年度秋季大会
    • Place of Presentation
      名古屋
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] 粒子サイズ制御したニオブ系無鉛セラミックスの圧電特性2013

    • Author(s)
      加藤健佑、柿本健一、波多野桂一、小林圭介、土信田豊
    • Organizer
      平成25年度日本セラミックス協会東海支部学術研究発表会
    • Place of Presentation
      名古屋
    • Related Report
      2013 Annual Research Report
  • [Presentation] ニオブ系無鉛圧電セラミックスの高温導電挙動2013

    • Author(s)
      渡邉桃子、柿本健一、籠宮 功
    • Organizer
      平成25年度日本セラミックス協会東海支部学術研究発表
    • Place of Presentation
      名古屋
    • Related Report
      2013 Annual Research Report
  • [Presentation] フローティングゾーン法により育成したニオブ系無鉛圧電結晶の分極異方性2013

    • Author(s)
      土田貢平、柿本健一
    • Organizer
      平成25年度日本セラミックス協会東海支部学術研究発表会
    • Place of Presentation
      名古屋
    • Related Report
      2013 Annual Research Report
  • [Presentation] Engineering of Lead-free Piezoelectrics in Alkali Niobate Ceramic System2013

    • Author(s)
      K. Kakimoto
    • Organizer
      5th Int. Symp. on Adv. Ceram.
    • Place of Presentation
      Wuhan, China
    • Related Report
      2013 Annual Research Report
    • Invited

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Published: 2013-05-21   Modified: 2019-07-29  

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