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Spin Liquid Studies by Pressure Control of Spin-Liquid-Insulating Phase

Research Project

Project/Area Number 25400384
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Condensed matter physics II
Research InstitutionNational Institute for Materials Science

Principal Investigator

UJI Shinya  国立研究開発法人物質・材料研究機構, 機能性材料研究拠点, 副拠点長 (80344430)

Project Period (FY) 2013-04-01 – 2016-03-31
Project Status Completed (Fiscal Year 2015)
Budget Amount *help
¥4,810,000 (Direct Cost: ¥3,700,000、Indirect Cost: ¥1,110,000)
Fiscal Year 2015: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2014: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2013: ¥2,730,000 (Direct Cost: ¥2,100,000、Indirect Cost: ¥630,000)
Keywordsスピン液体 / 磁気トルク / 磁化率 / 三角格子 / 有機磁性体 / 磁化 / スピン / 反強磁性 / 層状有機導体
Outline of Final Research Achievements

In order to investigate unique spin states in triangular lattices with spin S=1/2, we have measured magnetic properties in a wide temperaure and magnetic field region for k-type magnetic organic conductors. We measured the magnetic properties for k-(BDH-TTP)2FeX4 (X = Br, Cl) and developed an analysis technique of the magnetic torque data. We also performed SQUID and torque measurements for k-H-3(Cat-EDT-TTF)2 in detail and clarified the spin-liquid ground state, showing a constant magnetic susceptibility at low temperatures down to 50mK. We observed that the susceptibility shows divengence behavior at low temperature magnetic fields for k-(BEDT-TTF)2Cu2(CN)3, which can be ascribed to quantum critical behavior. This salt is found to show metallic conductivity at 0.5 GPa, but we cound not see quantum oscillations at low temperatures and high magnetic fields.

Report

(4 results)
  • 2015 Annual Research Report   Final Research Report ( PDF )
  • 2014 Research-status Report
  • 2013 Research-status Report
  • Research Products

    (28 results)

All 2016 2015 2014 2013 Other

All Int'l Joint Research (1 results) Journal Article (13 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 13 results,  Acknowledgement Compliant: 1 results) Presentation (11 results) (of which Int'l Joint Research: 2 results,  Invited: 5 results) Book (3 results)

  • [Int'l Joint Research] 国立強磁場研究所/アルゴンヌ国立研究所(米国)

    • Related Report
      2015 Annual Research Report
  • [Journal Article] Anisotropic magnetoresistance of charge-density wave in o-TaS32016

    • Author(s)
      K. Inagaki, T. Matsuura, M. Tsubota, S. Uji, T. Honma, and S. Tanda
    • Journal Title

      Phys. Rev. B

      Volume: 93 Issue: 7

    • DOI

      10.1103/physrevb.93.075423

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Vortex Dynamics and Diamagnetic Torque Signals in Two Dimensional Organic Superconductor λ-(BETS)2GaCl42015

    • Author(s)
      S. Uji, K. Kodama, K. Sugii, T. Terashima, T. Yamaguchi, N. Kurita, S. Tsuchiya, T. Konoike, M. Kimata, A. Kobayashi, B. Zhou, and H. Kobayashi
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 84 Issue: 10 Pages: 104709-104709

    • DOI

      10.7566/jpsj.84.104709

    • NAID

      210000133707

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] In-Plane Anisotropy of Upper Critical Field and Flux-Flow Resistivity in Layered Organic Superconductor β”-(ET)2SF5CH2CF2SO32015

    • Author(s)
      S. Yasuzuka, S. Uji, T. Terashima, K. Sugii, T. Isono, Y. Iida, and J. A. Schlueter
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 84 Issue: 9 Pages: 094709-094709

    • DOI

      10.7566/jpsj.84.094709

    • NAID

      210000133679

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Phase Boundary in a Superconducting State of κ-(BEDT-TTF)2Cu(NCS)2: Evidence of the Fulde–Ferrell–Larkin–Ovchinnikov Phase2015

    • Author(s)
      S. Tsuchiya, J. Yamada, K. Sugii, D. Graf, J. S. Brooks, T. Terashima, and S. Uji
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 84 Issue: 3 Pages: 034703-034703

    • DOI

      10.7566/jpsj.84.034703

    • NAID

      210000133478

    • Related Report
      2014 Research-status Report
    • Peer Reviewed
  • [Journal Article] Gapless Quantum Spin Liquid in an Organic Spin-1/2 Triangular Lattice kappa-H3(Cat-EDT-TTF)22014

    • Author(s)
      T. Isono et al.
    • Journal Title

      Phys. Rev. Lett

      Volume: 112 Issue: 17 Pages: 177201-177201

    • DOI

      10.1103/physrevlett.112.177201

    • Related Report
      2014 Research-status Report
    • Peer Reviewed
  • [Journal Article] Magnetic Torque Studies of πーd System κ-(BDH-TTP)2FeX4 (X = Br, Cl)2014

    • Author(s)
      K. Sugii, K. Takai, S. Tsuchiya, S. Uji, T. Terashima, H. Akutsu, A. Wada, S. Ichikawa, J. Yamada, and T. Enoki
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 83 Issue: 2 Pages: 023704-023704

    • DOI

      10.7566/jpsj.83.023704

    • NAID

      210000132939

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] In-Plane Anisotropy of Flux-Flow Resistivity in Layered Organic Superconductor BETS/GaCl42014

    • Author(s)
      S. Yasuzuka, S. Uji, T. Terashima, S. Tsuchiya, K. Sugii, B. Zhou, A. Kobayashi, H. Kobayashi
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 83 Issue: 1 Pages: 13705-13705

    • DOI

      10.7566/jpsj.83.013705

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Observation of Orbital Resonance Hall Effect in (TMTSF)2ClO42014

    • Author(s)
      K. Kobayashi, H. Satsukawa, J. Yamada, T. Terashima, and S. Uji
    • Journal Title

      Phys. Rev. Lett.

      Volume: 112 Issue: 11

    • DOI

      10.1103/physrevlett.112.116805

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Orbital Effect on FFLO Phase and Energy Dissipation due to Vortex Dynamics in Magnetic-Field-Induced Superconductor λ-(BETS)_2FeCl_42013

    • Author(s)
      S . Uji, K. Kodama, K.Sugii, T. Terashima, T. Yamaguchi, N. Kurita, S. Tsuchiya, M. Kimata, T. Konoike, A. Kobayashi, B. Zhou, H. Kobayashi
    • Journal Title

      J. Phys. Soc. Jpn

      Volume: 82 Issue: 3 Pages: 34715-34715

    • DOI

      10.7566/jpsj.82.034715

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Kosterlitz-Thouless-type transition in a charge ordered state of the layered organic conductorα-(BEDT-TTF)_2I_3, S. Uji2013

    • Author(s)
      S. Uji, K. Kodama, K. Sugii, Y. Takahide, T. Terashima, N. Kurita, S. Tsuchiya, M. Kohno, M. Kimata, K. Yamamoto, and K. Yakushi
    • Journal Title

      Phys. Rev. Lett.

      Volume: 110 Issue: 19 Pages: 196602-196602

    • DOI

      10.1103/physrevlett.110.196602

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Fermi Surface of the Dual-Layered Organic Superconductor ka2'-(BEDT-TTF)2Ag(CF3)4(TCE) with Acentric Charge-Ordered Layers2013

    • Author(s)
      T. Kawamoto, T. Mori, T. Terashima, S. Uji, and J. A. Schlueter
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 82 Issue: 2 Pages: 24704-24704

    • DOI

      10.7566/jpsj.82.024704

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Fluctuating Superconductivity in the Strongly Correlated Organic Superconductor κ-(BEDT-TTF)_2Cu[N(CN)_2]Br2013

    • Author(s)
      S . Tsuchiya, J. Yamada, T. Terashima, N. Kurita, K. Kodama, K. Sugii, and S. Uji
    • Journal Title

      J. Phys.Soc. Jpn.

      Volume: 82 Issue: 6 Pages: 64711-64711

    • DOI

      10.7566/jpsj.82.064711

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Crystal Structure and Physical Properties of π-d System κ-(BDH-TTP)2FeBr42013

    • Author(s)
      K. Sugii, K. Takai, S. Uji, T. Terashima, H. Akutsu, A. Wada, S. Ichikawa, J. Yamada, and T. Enoki
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 82 Issue: 12 Pages: 124709-124709

    • DOI

      10.7566/jpsj.82.124709

    • NAID

      210000132553

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Presentation] β”-(BEDT-TTF)4[(H3O)X(C2O4)3]Y, X=Ga,Fe Y=Nitrobenzeneの強磁場電子状態2016

    • Author(s)
      宇治進也、飯田頼嗣、杉浦栞理、磯野貴之、菊川直樹、寺嶋太一、圷広樹、中澤康浩、P. Day
    • Organizer
      日本物理学会
    • Place of Presentation
      東北学院大学
    • Year and Date
      2016-03-19
    • Related Report
      2015 Annual Research Report
  • [Presentation] High-magnetic-field superconducting phase in layered charge-transfer salts2015

    • Author(s)
      宇治進也、杉井かおり、土屋聡、磯野貴之、杉浦栞理、津田俊輔、菊川直樹、寺嶋太一、H. Akutsu、J. Yamada、D. Graf、P. Day
    • Organizer
      Pacifichem2015
    • Place of Presentation
      Honolulu convention center, Hawaii、アメリカ
    • Year and Date
      2015-12-15
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 有機超伝導体の強磁場物性:フェルミオロジーから磁場誘起超伝導,FFLO状態まで2015

    • Author(s)
      宇治進也
    • Organizer
      日本物理学会
    • Place of Presentation
      関西大学
    • Year and Date
      2015-09-16
    • Related Report
      2015 Annual Research Report
    • Invited
  • [Presentation] Hall resistance anomalies in two dimensional organic conductor a-(BED-TTF)2KHg(SCN)42015

    • Author(s)
      宇治進也、杉井かおり、磯野貴之、寺嶋太一、K. Kobayashi、J. Yamada
    • Organizer
      ISCOM2015
    • Place of Presentation
      Monarch Hotel & Convention Center ,Bad Gogging,ドイツ
    • Year and Date
      2015-09-06
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] κ-(BEDT-TTF)_2_Cu(NCS)_2_の磁束状態2015

    • Author(s)
      藤井友紀、宇治進也、磯野貴之、寺嶋太一、山田順一
    • Organizer
      日本物理学会第70回年次大会
    • Place of Presentation
      早稲田大学
    • Year and Date
      2015-03-21 – 2015-03-24
    • Related Report
      2014 Research-status Report
  • [Presentation] 低温磁気トルクから見たk-(BEDT-TTF)2Cu2(CN)3の量子スピン液体状態2015

    • Author(s)
      磯野貴之、寺嶋太一、宮川和也、鹿野田一司、宇治進也
    • Organizer
      日本物理学会第70回年次大会
    • Place of Presentation
      早稲田大学
    • Year and Date
      2015-03-21 – 2015-03-24
    • Related Report
      2014 Research-status Report
  • [Presentation] 量子スピン液体状態における磁気熱量効果: k-H3(Cat-EDT-TTF)2の場合2014

    • Author(s)
      磯野貴之、寺嶋太一、上田顕、森初果、宇治進也
    • Organizer
      日本物理学会2014秋季大会
    • Place of Presentation
      中部大学
    • Year and Date
      2014-09-07 – 2014-09-10
    • Related Report
      2014 Research-status Report
  • [Presentation] a-(BEDT-TTF)2KHg(SCN)4の角度依存ホール抵抗振動2014

    • Author(s)
      杉井かおり、磯野貴之、寺嶋太一、宇治進也
    • Organizer
      日本物理学会2014秋季大会
    • Place of Presentation
      中部大学
    • Year and Date
      2014-09-07 – 2014-09-10
    • Related Report
      2014 Research-status Report
  • [Presentation] Is FFLO phase a Universal Feature in I-(BETS)2FexGa1-xC14?2013

    • Author(s)
      宇治 進也
    • Organizer
      ISCOM2013
    • Place of Presentation
      Montreal, Canada
    • Related Report
      2013 Research-status Report
    • Invited
  • [Presentation] Kosterlitz-Thouless Transion in Charge Ordered States of Two Dimensional Organic Conductors2013

    • Author(s)
      宇治 進也
    • Organizer
      International School and Symposium on Molecular Materials, ISSMM
    • Place of Presentation
      東京工業大学
    • Related Report
      2013 Research-status Report
    • Invited
  • [Presentation] メゾスコピック超伝導体におけるボルテックスダイナミクス2013

    • Author(s)
      宇治 進也
    • Organizer
      超伝導体における渦糸状態の物理と応用
    • Place of Presentation
      東北大学
    • Related Report
      2013 Research-status Report
  • [Book] 分子性物質の物理2015

    • Author(s)
      宇治進也
    • Total Pages
      21
    • Publisher
      朝倉書店
    • Related Report
      2015 Annual Research Report
  • [Book] アグネ技術センター2014

    • Author(s)
      宇治進也
    • Total Pages
      11
    • Publisher
      層状分子性結晶における新奇超伝導相
    • Related Report
      2014 Research-status Report
  • [Book] アグネ技術センター2014

    • Author(s)
      層状分子性結晶の電荷励起に見るコスタリッツ-サウレス転移的振る舞い
    • Total Pages
      7
    • Publisher
      宇治進也
    • Related Report
      2014 Research-status Report

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Published: 2014-07-25   Modified: 2022-01-27  

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