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Experimental search for a muliple quantum-liquid state in organic magnets

Research Project

Project/Area Number 25620052
Research Category

Grant-in-Aid for Challenging Exploratory Research

Allocation TypeMulti-year Fund
Research Field Functional solid state chemistry
Research InstitutionNational Institute for Materials Science

Principal Investigator

ISONO Takayuki  独立行政法人物質・材料研究機構, 超伝導物性ユニット, NIMSポスドク研究員 (70625631)

Project Period (FY) 2013-04-01 – 2015-03-31
Project Status Completed (Fiscal Year 2014)
Budget Amount *help
¥3,640,000 (Direct Cost: ¥2,800,000、Indirect Cost: ¥840,000)
Fiscal Year 2014: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2013: ¥2,600,000 (Direct Cost: ¥2,000,000、Indirect Cost: ¥600,000)
Keywords量子スピン液体 / 磁気トルク / 有機固体 / スピンフラストレーション / 複合物性 / 量子常誘電 / 強相関電子系 / 分子性固体
Outline of Final Research Achievements

In order to reveal magnetic excitations at low temperatures in quantum spin-liquid states of triangular-lattice organic magnets, we performed torque magnetometry on kappa-H_3(Cat-EDT-TTF)_2 and kappa-(BEDT-TTF)_2Cu_2(CN)_3. We found that magnetic susceptibility shows a nearly temperature-independent behavior with a finite value below the temperature of 3 K for both the magnets. The comparison of the finite values among the triangular-lattice organic magnets revealed the common nature of the quantum spin-liquid states; the values are scaled by antiferromagnetic exchange-coupling constants.

Report

(3 results)
  • 2014 Annual Research Report   Final Research Report ( PDF )
  • 2013 Research-status Report
  • Research Products

    (15 results)

All 2015 2014 Other

All Journal Article (4 results) (of which Peer Reviewed: 4 results,  Acknowledgement Compliant: 2 results) Presentation (11 results)

  • [Journal Article] Gapless Quantum Spin Liquid in an Organic Spin-1/2 Triangular Lattice kappa-H3(Cat-EDT-TTF)22014

    • Author(s)
      T. Isono et al.
    • Journal Title

      Phys. Rev. Lett

      Volume: 112 Issue: 17 Pages: 177201-177201

    • DOI

      10.1103/physrevlett.112.177201

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Hydrogen-Bond-Dynamics-Based Switching of Conductivity and Magnetism: A Phase Transition Caused by Deuterium and Electron Transfer in a Hydrogen-Bonded Purely Organic Conductor Crystal2014

    • Author(s)
      A. Ueda, S. Yamada, T. Isono, H. Kamo, A. Nakao, R. Kumai, H. Nakao, Y. Murakami, K. Yamamoto, Y. Nishio, and H. Mori
    • Journal Title

      J. Am. Chem. Soc

      Volume: 136(34) Issue: 34 Pages: 12184-12192

    • DOI

      10.1021/ja507132m

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Uniaxial Strain Effect of the Moderately Dimerized Molecular Conductor β-(meso-DMBEDT-TTF)2PF62014

    • Author(s)
      Y. Nishida, T. Isono, A. Ueda, and H. Mori
    • Journal Title

      Eur. J. Inorg. Chem.

      Volume: 2014 Issue: 24 Pages: 3845-3849

    • DOI

      10.1002/ejic.201402463

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] 電子とプロトンが協奏する新しい分子機能性結晶の展開2014

    • Author(s)
      森初果,上田顕,磯野貴之
    • Journal Title

      固体物理

      Volume: 49 Pages: 147-158

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Presentation] 低温磁気トルクから見たkappa-(BEDT-TTF)2Cu2(CN)3の量子スピン液体状態2015

    • Author(s)
      磯野貴之,寺嶋太一,宮川和也,鹿野田一司,宇治進也
    • Organizer
      日本物理学会2015年年次大会
    • Place of Presentation
      早稲田大学
    • Year and Date
      2015-03-21 – 2015-03-24
    • Related Report
      2014 Annual Research Report
  • [Presentation] 量子スピン液体状態における磁気熱量効果:kappa-H3(Cat-EDT-TTF)2の場合2014

    • Author(s)
      磯野貴之,寺嶋太一,上田 顕,森 初果,宇治進也
    • Organizer
      日本物理学会2014年秋季大会
    • Place of Presentation
      中部大学
    • Year and Date
      2014-09-07 – 2014-09-10
    • Related Report
      2014 Annual Research Report
  • [Presentation] Frustrated Magnetic Order in the Organic Spin-1/2 Square Lattice beta-(BDA-TTP)2I32014

    • Author(s)
      T. Isono, T. Terashima, K. Kikuchi, J. Yamada, and S. Uji
    • Organizer
      International Conferences of Strongly Correlated Electron System (SCES2014)
    • Place of Presentation
      フランス
    • Year and Date
      2014-07-07 – 2014-07-11
    • Related Report
      2014 Annual Research Report
  • [Presentation] Anomalous Antiferromagnetic Order in the Organic Mott Insulator beta-(BDA-TTP)2I32014

    • Author(s)
      T. Isono, T. Terashima, K. Kikuchi, J. Yamada, and S. Uji
    • Organizer
      International Conferences on Science and Technology of Synthetic Metals (ICSM2014)
    • Place of Presentation
      フィンランド
    • Year and Date
      2014-06-30 – 2014-07-05
    • Related Report
      2014 Annual Research Report
  • [Presentation] Gapless Quantum Spin Liquid in an Organic Spin-1/2 Triangular Lattice kappa-H3(Cat-EDT-TTF)2

    • Author(s)
      T. Isono, H. Kamo, A. Ueda, K. Takahashi, M. Kimata, H. Tajima, S. Tsuchiya, T. Terashima, S. Uji, and H. Mori
    • Organizer
      The International Conference on Strongly Correlated Electron Systems (SCES2013)
    • Place of Presentation
      東京大学本郷キャンパス
    • Related Report
      2013 Research-status Report
  • [Presentation] 低温磁気トルクから見た有機三角格子における 量子スピン液体の普遍性

    • Author(s)
      磯野貴之,加茂博道,上田 顕,高橋一志,木俣 基,田島裕之, 土屋 聡,寺嶋太一,宇治進也,森 初果
    • Organizer
      日本物理学会2013年秋季大会
    • Place of Presentation
      徳島大学常三島キャンパス
    • Related Report
      2013 Research-status Report
  • [Presentation] 低温磁気トルクから見た圧力誘起超伝導体beta-(BDA-TTP)2X系における特異な磁気秩序

    • Author(s)
      磯野貴之,寺嶋太一,菊地耕一,山田順一,宇治進也
    • Organizer
      日本物理学会第69回年次大会
    • Place of Presentation
      東海大学湘南キャンパス
    • Related Report
      2013 Research-status Report
  • [Presentation] ダイマーモット系kappa-D3(Cat-EDT-TTF)2における水素結合由来の電荷秩序化

    • Author(s)
      山田翔太,上田顕,磯野貴之,李相哲,加茂博道,中尾朗子,熊井玲児,中尾裕則,村上洋一,吉澤英樹,西尾豊,田嶋尚也,梶田晃示,森初果
    • Organizer
      日本物理学会2013年秋季大会
    • Place of Presentation
      徳島大学常三島キャンパス
    • Related Report
      2013 Research-status Report
  • [Presentation] kappa-D3(Cat-EDT-TTF)2における重水素置換効果

    • Author(s)
      山田翔太,上田顕,磯野貴之,吉田順哉,中尾朗子,熊井玲児,中尾裕則,村上洋一,吉澤英樹,西尾豊,田嶋尚也,梶田晃示,森初果
    • Organizer
      日本物理学会第69回年次大会
    • Place of Presentation
      東海大学湘南キャンパス
    • Related Report
      2013 Research-status Report
  • [Presentation] 超伝導と電荷秩序が競合する分子性導体beta-(meso-DMBEDT-TTF)2PF6の一軸性圧縮効果

    • Author(s)
      西田容平,磯野貴之,上田顕,森初果
    • Organizer
      日本物理学会第69回年次大会
    • Place of Presentation
      東海大学湘南キャンパス
    • Related Report
      2013 Research-status Report
  • [Presentation] beta''-(BEDT-TTF)4[(H3O)X(C2O4)]Y,X=Ga Y=Nitrobenzeneにおける異方的超伝導

    • Author(s)
      飯田頼嗣,杉井かおり,磯野貴之,菊川直樹,津田俊輔,寺嶋太一,圷広樹,山田順一,中辻愼一,Peter Day,宇治進也
    • Organizer
      日本物理学会第69回年次大会
    • Place of Presentation
      東海大学湘南キャンパス
    • Related Report
      2013 Research-status Report

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Published: 2014-07-25   Modified: 2019-07-29  

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