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Development of New Kagome Antiferromagnets to Realize a Novel Quantum Magnetic Phase

Research Project

Project/Area Number 25800188
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeMulti-year Fund
Research Field Condensed matter physics II
Research InstitutionNagoya University

Principal Investigator

Okamoto Yoshihiko  名古屋大学, 工学(系)研究科(研究院), 准教授 (90435636)

Project Period (FY) 2013-04-01 – 2016-03-31
Project Status Completed (Fiscal Year 2015)
Budget Amount *help
¥4,160,000 (Direct Cost: ¥3,200,000、Indirect Cost: ¥960,000)
Fiscal Year 2015: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2014: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
Fiscal Year 2013: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Keywords幾何学的フラストレート磁性体 / 新物質開拓 / カゴメ格子 / 反強磁性体 / 銅鉱物 / 幾何学的フラストレーション / 新物質探索
Outline of Final Research Achievements

We developed novel geometrically frustrated magnets such as spin-1/2 kagome antiferromagnet Edwardsite, spin-5/2 kagome-triangular antiferromagnet NaBa2Mn3F11, and spin-3/2 breathing pyrochlore antiferromagnets LiGaCr4O8 and LiInCr4O8 toward the discovery of anomalous magnetic phases as typified by the quantum spin liquid. By measuring various physical properties of the synthesized samples of these magnets, we found interesting phenomena such as a spin-gap behavior accompanied by the formation of the tetramer singlet, a magnetic transition located at the vicinity of the tricritical point, and ferroelectricity induced by the incommensurate spiral magnetic order.

Report

(4 results)
  • 2015 Annual Research Report   Final Research Report ( PDF )
  • 2014 Research-status Report
  • 2013 Research-status Report
  • Research Products

    (22 results)

All 2016 2015 2014 2013 Other

All Int'l Joint Research (1 results) Journal Article (12 results) (of which Int'l Joint Research: 3 results,  Peer Reviewed: 12 results,  Acknowledgement Compliant: 4 results,  Open Access: 1 results) Presentation (9 results) (of which Invited: 5 results)

  • [Int'l Joint Research] Universitet Paris-Sud/LNCMI-CNRS/Institut Laue Langevin(フランス)

    • Related Report
      2015 Annual Research Report
  • [Journal Article] Superconductivity in the Hexagonal Ternary Phosphide ScIrP2016

    • Author(s)
      Y. Okamoto, T. Inohara, Y. Yamakawa, A. Yamakage, and K. Takenaka
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 85 Issue: 1 Pages: 013704-013704

    • DOI

      10.7566/jpsj.85.013704

    • NAID

      40020699678

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Complex Magnetostructural Order in the Frustrated Spinel LiInCr4O82015

    • Author(s)
      G. J. Nilsen, Y. Okamoto, T. Masuda, J. Rodriguez-Carvajal, H. Mutka, T. Hansen, and Z. Hiroi,
    • Journal Title

      Physical Review B

      Volume: 91 Issue: 17

    • DOI

      10.1103/physrevb.91.174435

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] One-Third Magnetization Plateau with a Preceding Novel Phase in Volborthite2015

    • Author(s)
      Hajime Ishikawa, Makoto Yoshida, Kazuhiro Nawa, Minki Jeong, Steffen Kramer, Mladen Horvatic, Claude Berthier, Masashi Takigawa, Mitsuru Akaki, Atsushi Miyake, Masashi Tokunaga, Koichi Kindo, Junichi Yamaura, Yoshihiko Okamoto, Zenji Hiroi
    • Journal Title

      Physical Review Letters

      Volume: 114 Issue: 22 Pages: 2272021-5

    • DOI

      10.1103/physrevlett.114.227202

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Frozen State and Spin Liquid Physics in Na4Ir3O8: an NMR Study2015

    • Author(s)
      A. C. Shockley, F. Bert, J-C. Orain, Y. Okamoto, and P. Mendels
    • Journal Title

      Physical Review Letters

      Volume: 115 Issue: 4

    • DOI

      10.1103/physrevlett.115.047201

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Magnetic Phase Diagram of the Breathing Pyrochlore Antiferromagnet LiGa1-xInxCr4O82015

    • Author(s)
      Y. Okamoto, G. J. Nilsen, T. Nakazono, and Z. Hiroi
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 84 Issue: 4 Pages: 043707-043707

    • DOI

      10.7566/jpsj.84.043707

    • NAID

      210000133502

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Lifshitz metal-insulator transition induced by the all-in/all-out magnetic order in the pyrochlore oxide Cd2Os2O72015

    • Author(s)
      Zenji Hiroi, Jun-ichi Yamaura, Takahiro Hirose, Issei Nagashima, Yoshihiko Okamoto
    • Journal Title

      APL Materials

      Volume: 3 Issue: 4 Pages: 041501-041501

    • DOI

      10.1063/1.4907734

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Helical Order and Multiferroicity in the S = 1/2 Quasi-Kagome System KCu3As2O7(OD)32014

    • Author(s)
      G. J. Nilsen, Y. Okamoto, H. Ishikawa, V. Shimonet, C. V. Colin, A. Cano, L. C. Chapon, T. Hansen, H. Mutka, and Z. Hiroi
    • Journal Title

      Phys. Rev. B

      Volume: 89 Issue: 14

    • DOI

      10.1103/physrevb.89.140412

    • Related Report
      2014 Research-status Report
    • Peer Reviewed
  • [Journal Article] Novel Phase Transitions in the Breathing Pyrochlore Lattice:7Li-NMR on LiInCr4O8 and LiGaCr4O82014

    • Author(s)
      Yu Tanaka, Makoto Yoshida, Masashi Takigawa, Yoshihiko Okamoto, and Zenji Hiroi
    • Journal Title

      Phys. Rev. Lett

      Volume: 113 Issue: 22

    • DOI

      10.1103/physrevlett.113.227204

    • Related Report
      2014 Research-status Report
    • Peer Reviewed
  • [Journal Article] Kagome-Triangular Lattice Antiferromagnet NaBa2Mn3F112014

    • Author(s)
      Hajime Ishikawa, Tsuyoshi Okubo, Yoshihiko Okamoto, and Zenji Hiroi
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 83 Issue: 4 Pages: 043703-043703

    • DOI

      10.7566/jpsj.83.043703

    • NAID

      210000133024

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Magnetic Properties of the Spin-1/2 Deformed Kagome Antiferromagnet Edwardsite2013

    • Author(s)
      Hajime Ishikawa, Yoshihiko Okamoto, and Zenji Hiroi
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 82 Issue: 6 Pages: 063710-063710

    • DOI

      10.7566/jpsj.82.063710

    • NAID

      210000132580

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Breathing Pyrochlore Lattice Realized in A-site Ordered Spinel Oxides LiGaCr4O8 and LiInCr4O82013

    • Author(s)
      Yoshihiko Okamoto, Goran J. Nilsen, J. Paul Attfield, and Zenji Hiroi
    • Journal Title

      Phys. Rev. Lett.

      Volume: 110 Issue: 9

    • DOI

      10.1103/physrevlett.110.097203

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Magnetic Order in the Spin-1/2 Antiferromagnet Vesignieite2013

    • Author(s)
      M. Yoshida, Y. Okamoto, M. Takigawa, and Z. Hiroi
    • Journal Title

      J. Phys. Soc. Jpn

      Volume: 82 Issue: 1 Pages: 013702-013702

    • DOI

      10.7566/jpsj.82.013702

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Presentation] 銅鉱物におけるスピン1/2カゴメ格子反強磁性体の物質開拓2016

    • Author(s)
      岡本佳比古
    • Organizer
      科研費基盤(S)研究会「フラストレーション系物質の科学:協奏と競合の世界」
    • Place of Presentation
      トヨタ産業技術館
    • Year and Date
      2016-02-19
    • Related Report
      2015 Annual Research Report
    • Invited
  • [Presentation] ブリージングパイロクロア格子反強磁性体の強磁場磁化過程2015

    • Author(s)
      岡本佳比古、三宅厚志、徳永将史、松尾晶、金道浩一、G. J. Nilsen、竹中康司、広井善二
    • Organizer
      物性研短期研究会「スピン系科学の深化と最前線」
    • Place of Presentation
      東京大学物性研究所
    • Year and Date
      2015-11-17
    • Related Report
      2015 Annual Research Report
  • [Presentation] ブリージングパイロクロア格子反強磁性体LiInCr4O8の強磁場磁化過程2015

    • Author(s)
      岡本佳比古、三宅厚志、徳永将史、G. J. Nilsen、中園敦巳、竹中康司、広井善二
    • Organizer
      日本物理学会2015年秋季大会
    • Place of Presentation
      関西大学
    • Year and Date
      2015-09-19
    • Related Report
      2015 Annual Research Report
  • [Presentation] ブリージングパイロクロア格子反強磁性体におけるフラストレーションとボンド交替2015

    • Author(s)
      岡本佳比古
    • Organizer
      第14回CROSSroads「スピン系とフラストレーション」
    • Place of Presentation
      いばらき量子ビーム研究センター
    • Year and Date
      2015-02-04
    • Related Report
      2014 Research-status Report
    • Invited
  • [Presentation] ブリージングパイロクロアをもつCrスピネル酸化物におけるフラストレーションとボンド交替2014

    • Author(s)
      岡本佳比古
    • Organizer
      研究環「特異な結晶構造に創出する新奇量子相の解明」第2回研究会
    • Place of Presentation
      首都大学東京
    • Year and Date
      2014-09-26
    • Related Report
      2014 Research-status Report
    • Invited
  • [Presentation] Geometrical Frustration and Bond Alternation on the Breathing Pyrochlore Lattice2014

    • Author(s)
      Yoshihiko Okamoto
    • Organizer
      OIST International Workshop on Novel Quantum Materials and Physics
    • Place of Presentation
      沖縄科学技術大学院大学
    • Year and Date
      2014-05-15
    • Related Report
      2014 Research-status Report
    • Invited
  • [Presentation] Breathing Pyrochlore Lattice Realized in the A-Site Ordered Spinel Oxides LiGaCr4O8 and LiInCr4O82014

    • Author(s)
      Yoshihiko Okamoto
    • Organizer
      APS March Meeting 2014
    • Place of Presentation
      Colorado Convention Center
    • Related Report
      2013 Research-status Report
    • Invited
  • [Presentation] ブリージングパイロクロア格子反強磁性体LiGa0.1In0.9Cr4O8の基底状態2014

    • Author(s)
      岡本佳比古、G. J. Nilsen、中園敦巳、広井善二
    • Organizer
      日本物理学会第69回年次大会
    • Place of Presentation
      東海大学
    • Related Report
      2013 Research-status Report
  • [Presentation] ブリージングパイロクロア格子反強磁性体LiGaCr4O8とLiInCr4O8の磁気構造と磁気励起2013

    • Author(s)
      岡本佳比古、中園敦巳、G. J. Nilsen、H. Mutka、T. Hansen、益田隆嗣、広井善二
    • Organizer
      日本物理学会2013年秋季大会
    • Place of Presentation
      徳島大学
    • Related Report
      2013 Research-status Report

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Published: 2014-07-25   Modified: 2020-05-15  

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