1994 Fiscal Year Annual Research Report

長寿命核廃棄物の消滅処理法に関する基礎的研究

Research Project

Project/Area Number	06302081
Research Category	Grant-in-Aid for Co-operative Research (A)
Research Institution	Kyoto University
Principal Investigator	木村逸郎京都大学, 工学部, 教授 (40027404)
Co-Investigator(Kenkyū-buntansha)	関本博東京工業大学, 原子炉工学研究所, 教授 (00108242) 仁科浩二郎名古屋大学, 工学部, 教授 (60023222) 馬場宏大阪大学, 理学部, 教授 (60156536) 平川直弘東北大学, 工学部, 教授 (20005391) 中沢正治東京大学, 工学部, 教授 (00010976)
Keywords	核廃棄物 / 放射性廃棄物 / 消滅処理 / 核分裂 / 核破砕 / 群分離 / アクチニド / 超ウラン元素
Research Abstract	長寿命の核廃棄物を転換・消滅して短寿命化し、リスクを大幅に軽減するための方法を究明し、そのシステムを設計する研究を推進した。具体的な内容を次に示す。1.レーザーによる核崩壊制御、ガンマ線レーザーと光核反応の微細構造について検討した。2.超変形回転バンド、重粒子崩壊と高スピン核異性体ビームの調査と検討を行った。3.核分裂に関連し、入射粒子のエネルギー依存性、角運動量の影響、即発中性子の多重度に関する実験を行うとともに、即発中性子のエネルギー分布計算コードを完成した。共鳴と熱領域における精密な^<237>Npと^<241>Amの核分裂断面Q_β値が得られた。4.Ceなど稀土類10核種の中速中性子捕獲断面積を求めた。5.核破砕に関連し、20-40MeVと80-135MeVの中性子による各種放射化断面積を測定した。また、0.8、1.5および3.0GeV陽子の中性子放出微分断面積の解析を行い、モデルを評価した。6.転換消滅システムとして、鉛冷却高速炉、溶融塩炉および加速器炉などの性能を解析した。またTRU核種の計算におけるマルチバンド法の適用性を示した。さらに臨界集合体による模擬実験を立案した。7.溶融塩と液体金属の二相系におけるアクチニドやランタニド元素の分離分配実験を行った。8.アクチニド(まずはU)の新規3元化合物を探索し、その物性値を求めた。9.核燃焼システムとくにそのダウンストリームにおける消滅処理の意義を評価した。さらに群分離と消滅処理間の関連性も含めた詳細なシステム解析の方法を提案し、実際に計算を行った。全体のこととして、研究の進め方、国内外関係機関との協力の仕方などについて議論し、今後まとめてゆくことになった。

Research Products

(45 results)

All Other

All Publications (45 results)

[Publications] K.Nisio: "Measurement of Fragment Mass Dependent Kinetic Energy and Neutron Multiplicity for Thermal Neutron induced Fission of Pu-239" J.Nucl.Sci.Technol.(in print).
[Publications] A.Odahara: "High-Spin State of ^<146>Sm" Z.Phys.A350. 185-186 (1994)
[Publications] K.Tsukada: "Mass Yield and Angular Distribution of Rare Earth Elements Produced in Proton-Induced Fission of Pu-244" J.Alloys and Compounds. 213/214. 414-416 (1994)
[Publications] I.Nishikawa: "Fragment Mass and Kinetic Energy Distributions from Fission of Light Actinides" J.Alloys and Compounds. 213/214. 417-419 (1994)
[Publications] K.Sueki: "Measurement of Kinetic Energy of Cs isotopes Produced in ^<16>O+^<209>Bi Nuclear Fission by Differential Range Method" J.Alloys and Compounds. 213/214. 420-422 (1994)
[Publications] A.Shinohara: "Pionic X-ray Intensities per Captured Negative Pion in Various Elements" Nucl.Instr.Methods. B84. 14-22 (1994)
[Publications] K.Nisio: "Energy and Neutron Multiplicity for Thermal Neutron Induced Fission of Pu-239" J.Nucl.Sci.Technol.(in print).
[Publications] A.Odahara: "High-Spin State of ^<145>Sm" Z.Phys.A350. 185-186 (1994)
[Publications] K.Tsukada: "Mass Yield and Angular Distribution of Rare Earth Elements Produced in Proton-induced Fission of Pu-244" J.Alloys and Compounds. 213/214. 414-416 (1994)
[Publications] I.Nishikawa: "Fragment Mass and Kinetic Energy Distributions from Fission of Light Actinides" J.Alloys and Compounds. 213/214. 417-419 (1994)
[Publications] K.Sueki: "Measurement of Kinetic Energy of Cs lsotopes Produced in ^<16>O+^<209>Bi Nuclear Fission by Differential Range Method" J.Alloys and Compounds. 213/214. 420-422 (1994)
[Publications] A.Shinohara: "Pionic X-ray Intensities per Captured Negative Pion in Various Elements" Nucl.Instr.Methods. B84. 14-22 (1994)
[Publications] T.Saito: "Measurement of Atomic Capture Probabillities of Negative Pion in Metal Hydrides" Hyperfine Interactions. 84. 193-198 (1994)
[Publications] A.Shinohara: "An Upper Limit for the Probability of Nuclear Excitation by Electron Transition in U-235" Chem.Lett.1995. 19-20 (1995)
[Publications] N.Takahashi: "Two Mode Fission:Existense of Two Independent Paths in the Fission of Actinide Elements" Z.Phys.(in print).
[Publications] H.Baba: "Comments of the Half-life of Pu-237" Appl.Radiat.Isotopes. (in print).
[Publications] T.Ohsawa: "Evaluation of Fission Neutron Spectra for Minor Actindes" Proc.Intern.Conf.on Nuclear Data for Science and Technology. 2. 639-641 (1994)
[Publications] K.Sayama: "Analysis of Post Irradiation Experiments in PWR Using New Nuclear Data Libraries" J.Nucl.Sci.Technol.31. 596-608 (1994)
[Publications] T.Iwasaki: "Neutron Economy of Transmutation of TRU in Thermal and Fast Neutron Fields" J.Nucl.Sci.Technol.31. 1255-1264 (1994)
[Publications] T.Iwasaki: "Transmutation of Minor Actinide in Well Thermalized Neutron Field" J.Nucl.Sci.Technol.32. 8-17 (1995)
[Publications] K.Kobayashi: "Measurement of Thermal Neutron Cross Section and Resonance Integral for ^<237>Np(n,γ)^<238>Np Reaction" J.Nucl.Sci.Technol.31. 1239-1247 (1994)
[Publications] K.Kobayashi: "Fission Cross Section Measurement of Am-241 between 0.1eV and 10keV with Lead Slowing-down Spectrometer" Proc.Intern.Conf.on Nuclear Data for Science and Technology. 1. 242-244 (1994)
[Publications] Y.Uwamino: "Measurement of Neutron Activation Cross Sections for Energies up to 40MeV for Natural Samples of Mg,Si,Ca,V,Cr,Cu,and Zn" J.Nucl.Sci.Technol.31. 1-11 (1994)
[Publications] K.Kimura: "Residual Long-lived Radioactivity Distribution in the Inner Concrete Wall of a Cyclotron Vault" Health Phys.67. 621-631 (1994)
[Publications] T.Ishikawa: "Neutron Penetration through Iron and Concrete Shields with the Use of 22.0 and 32.5MeV Quasi-Monoenergetic Sources" Nucl.Sci.Eng.116. 278-290 (1994)
[Publications] T.Ikuta: "Neutron-rich isotopes in the Mass Region 147≦A≦152" Proc.Intern.Conf.on Nuclear Data for Science and Technology. Vol.1. 331-333 (1994)
[Publications] M.Sibata: "Beta Decay of Pr-151 into Levels in Nd-151" J.Phys.Soc.Japan. 63. 3263-3272 (1994)
[Publications] K.Ishibashi: "Measurement of Neutron-Production Double Differential Cross Sections for Incident Protons of 0.8,1.5 and 3.0GeV" Proc.Intern.Conf.on Nuclear Data for Science and Technology. Vol.1. 347-353 (1994)
[Publications] K.Ishibashi: "High Energy Transport Code HETC-3 STEP Applicable to Incident Energies below 100MeV" Proc.Intern.Conf.on Nuclear Data for Science and Technology. Vol.1. 571-573 (1994)
[Publications] N.Shigyo: "Paramentrization of Fragmentation Cross Section for Proton-Induced Spallation Reaction" J.Nucl.Sci.Technol.32. 1-7 (1995)
[Publications] H.sekimoto: "Physics of Future Equilibrium State of Nuclear Energy Utilization" Proc.Intern.Conf.on Reactor Physics and Reactor Conputation. Vol.1. 515-523 (1994)
[Publications] H.sekimoto: "Lead-Cooled Fast Reactor Use in Future Equilibrium Energy Production" Trans.American Nucl.Soc.71. 496-497 (1994)
[Publications] J.Kimura: "Study on Homageneous Recycling of Minor Actinides in Mox Fueled PWRs" Annu.Rep.Res.Reactor Institute,Kyoto Univ.27. 79-91 (1994)
[Publications] H.Moriyama: "Reductive Extraction Behavior of Actinide and Lanthanide Elements in Molten Salt and Liquid Metal Binary Systems" J.Alloys and Compounds. 213/214. 354-359 (1994)
[Publications] H.Moriyama: "Equilibrium Distributions of Actinides and Lanthanides in Molten Salt and Liquid Metal Binary Phase Systems" Sci.Rep.RITS. A40. 1-4 (1994)
[Publications] Y.Shiokawa: "Structure and Magnetic Properties of U_2Co_<15>Ge_2 and Related Compounds" J.Alloys and Compounds. 213/214. 513-515 (1994)
[Publications] Y.Shiokawa: "Some Uranium Compounds with High Curie Temperature" Sci.Rep.RITS. A40. 9-11 (1994)
[Publications] A.Kitamoto: "Special Characteristics of Fast B/T Reactor for Minimization of High Level Waste and Hazard Index" Proc.Intern.Meeting on Nuclear and Hazardous Waste Management,Spectrum '94. 2. 1422-1427 (1994)
[Publications] A.Kitamoto: "Grouping in Partitioning of HLW for Burning and/or Transmutation with Nuclear Reactors" J.Nucl.Sci.Technol.(in print).
[Publications] A.Kitamoto: "Grouping of HLW in Partitioning for B/T Treatment with Neutron Reactors Based on Three Criteria" Annals Nucl.Energy. (in print).
[Publications] S.Nagasaki: "Influence of Fe(III) Coloids on NP(V) Migration through Quartz-Packed Columus" J.Nucl.Sci.Technol.31. 143-150 (1994)
[Publications] 鈴木篤之: "インポート・プレシアム法によるプルトニウム利用のセキュリティ効果の評価" 原子力学会誌. 36. 245-252 (1994)
[Publications] 鈴木篤之: "レプリケータモデルによる電源構成の最適化" エネルギー・資源. 15. 302-309 (1994)
[Publications] A.Suzuki: "Managing the Plutonium Surplus:Applications and Technical Options" Kluwer Academic Publishers, 219 (1994)
[Publications] A.Suzuki: "Managing the Plutonium Surplus:Applications and Technical Options" Kluwer Academic Publishers, 219 (1994)

1994 Fiscal Year Annual Research Report

長寿命核廃棄物の消滅処理法に関する基礎的研究

Principal Investigator

木村 逸郎 京都大学, 工学部, 教授 (40027404)

Research Products

[Publications] K.Nisio: "Measurement of Fragment Mass Dependent Kinetic Energy and Neutron Multiplicity for Thermal Neutron induced Fission of Pu-239" J.Nucl.Sci.Technol.(in print).

[Publications] A.Odahara: "High-Spin State of ^<146>Sm" Z.Phys.A350. 185-186 (1994)

[Publications] K.Tsukada: "Mass Yield and Angular Distribution of Rare Earth Elements Produced in Proton-Induced Fission of Pu-244" J.Alloys and Compounds. 213/214. 414-416 (1994)

[Publications] I.Nishikawa: "Fragment Mass and Kinetic Energy Distributions from Fission of Light Actinides" J.Alloys and Compounds. 213/214. 417-419 (1994)

[Publications] K.Sueki: "Measurement of Kinetic Energy of Cs isotopes Produced in ^<16>O+^<209>Bi Nuclear Fission by Differential Range Method" J.Alloys and Compounds. 213/214. 420-422 (1994)

[Publications] A.Shinohara: "Pionic X-ray Intensities per Captured Negative Pion in Various Elements" Nucl.Instr.Methods. B84. 14-22 (1994)

[Publications] K.Nisio: "Energy and Neutron Multiplicity for Thermal Neutron Induced Fission of Pu-239" J.Nucl.Sci.Technol.(in print).

[Publications] A.Odahara: "High-Spin State of ^<145>Sm" Z.Phys.A350. 185-186 (1994)

[Publications] K.Tsukada: "Mass Yield and Angular Distribution of Rare Earth Elements Produced in Proton-induced Fission of Pu-244" J.Alloys and Compounds. 213/214. 414-416 (1994)

[Publications] I.Nishikawa: "Fragment Mass and Kinetic Energy Distributions from Fission of Light Actinides" J.Alloys and Compounds. 213/214. 417-419 (1994)

[Publications] K.Sueki: "Measurement of Kinetic Energy of Cs lsotopes Produced in ^<16>O+^<209>Bi Nuclear Fission by Differential Range Method" J.Alloys and Compounds. 213/214. 420-422 (1994)

[Publications] A.Shinohara: "Pionic X-ray Intensities per Captured Negative Pion in Various Elements" Nucl.Instr.Methods. B84. 14-22 (1994)

[Publications] T.Saito: "Measurement of Atomic Capture Probabillities of Negative Pion in Metal Hydrides" Hyperfine Interactions. 84. 193-198 (1994)

[Publications] A.Shinohara: "An Upper Limit for the Probability of Nuclear Excitation by Electron Transition in U-235" Chem.Lett.1995. 19-20 (1995)

[Publications] N.Takahashi: "Two Mode Fission:Existense of Two Independent Paths in the Fission of Actinide Elements" Z.Phys.(in print).

[Publications] H.Baba: "Comments of the Half-life of Pu-237" Appl.Radiat.Isotopes. (in print).

[Publications] T.Ohsawa: "Evaluation of Fission Neutron Spectra for Minor Actindes" Proc.Intern.Conf.on Nuclear Data for Science and Technology. 2. 639-641 (1994)

[Publications] K.Sayama: "Analysis of Post Irradiation Experiments in PWR Using New Nuclear Data Libraries" J.Nucl.Sci.Technol.31. 596-608 (1994)

[Publications] T.Iwasaki: "Neutron Economy of Transmutation of TRU in Thermal and Fast Neutron Fields" J.Nucl.Sci.Technol.31. 1255-1264 (1994)

[Publications] T.Iwasaki: "Transmutation of Minor Actinide in Well Thermalized Neutron Field" J.Nucl.Sci.Technol.32. 8-17 (1995)

[Publications] K.Kobayashi: "Measurement of Thermal Neutron Cross Section and Resonance Integral for ^<237>Np(n,γ)^<238>Np Reaction" J.Nucl.Sci.Technol.31. 1239-1247 (1994)

[Publications] K.Kobayashi: "Fission Cross Section Measurement of Am-241 between 0.1eV and 10keV with Lead Slowing-down Spectrometer" Proc.Intern.Conf.on Nuclear Data for Science and Technology. 1. 242-244 (1994)

[Publications] Y.Uwamino: "Measurement of Neutron Activation Cross Sections for Energies up to 40MeV for Natural Samples of Mg,Si,Ca,V,Cr,Cu,and Zn" J.Nucl.Sci.Technol.31. 1-11 (1994)

[Publications] K.Kimura: "Residual Long-lived Radioactivity Distribution in the Inner Concrete Wall of a Cyclotron Vault" Health Phys.67. 621-631 (1994)

[Publications] T.Ishikawa: "Neutron Penetration through Iron and Concrete Shields with the Use of 22.0 and 32.5MeV Quasi-Monoenergetic Sources" Nucl.Sci.Eng.116. 278-290 (1994)

[Publications] T.Ikuta: "Neutron-rich isotopes in the Mass Region 147≦A≦152" Proc.Intern.Conf.on Nuclear Data for Science and Technology. Vol.1. 331-333 (1994)

[Publications] M.Sibata: "Beta Decay of Pr-151 into Levels in Nd-151" J.Phys.Soc.Japan. 63. 3263-3272 (1994)

[Publications] K.Ishibashi: "Measurement of Neutron-Production Double Differential Cross Sections for Incident Protons of 0.8,1.5 and 3.0GeV" Proc.Intern.Conf.on Nuclear Data for Science and Technology. Vol.1. 347-353 (1994)

[Publications] K.Ishibashi: "High Energy Transport Code HETC-3 STEP Applicable to Incident Energies below 100MeV" Proc.Intern.Conf.on Nuclear Data for Science and Technology. Vol.1. 571-573 (1994)

[Publications] N.Shigyo: "Paramentrization of Fragmentation Cross Section for Proton-Induced Spallation Reaction" J.Nucl.Sci.Technol.32. 1-7 (1995)

[Publications] H.sekimoto: "Physics of Future Equilibrium State of Nuclear Energy Utilization" Proc.Intern.Conf.on Reactor Physics and Reactor Conputation. Vol.1. 515-523 (1994)

[Publications] H.sekimoto: "Lead-Cooled Fast Reactor Use in Future Equilibrium Energy Production" Trans.American Nucl.Soc.71. 496-497 (1994)

[Publications] J.Kimura: "Study on Homageneous Recycling of Minor Actinides in Mox Fueled PWRs" Annu.Rep.Res.Reactor Institute,Kyoto Univ.27. 79-91 (1994)

[Publications] H.Moriyama: "Reductive Extraction Behavior of Actinide and Lanthanide Elements in Molten Salt and Liquid Metal Binary Systems" J.Alloys and Compounds. 213/214. 354-359 (1994)

[Publications] H.Moriyama: "Equilibrium Distributions of Actinides and Lanthanides in Molten Salt and Liquid Metal Binary Phase Systems" Sci.Rep.RITS. A40. 1-4 (1994)

[Publications] Y.Shiokawa: "Structure and Magnetic Properties of U_2Co_<15>Ge_2 and Related Compounds" J.Alloys and Compounds. 213/214. 513-515 (1994)

[Publications] Y.Shiokawa: "Some Uranium Compounds with High Curie Temperature" Sci.Rep.RITS. A40. 9-11 (1994)

[Publications] A.Kitamoto: "Special Characteristics of Fast B/T Reactor for Minimization of High Level Waste and Hazard Index" Proc.Intern.Meeting on Nuclear and Hazardous Waste Management,Spectrum '94. 2. 1422-1427 (1994)

[Publications] A.Kitamoto: "Grouping in Partitioning of HLW for Burning and/or Transmutation with Nuclear Reactors" J.Nucl.Sci.Technol.(in print).

[Publications] A.Kitamoto: "Grouping of HLW in Partitioning for B/T Treatment with Neutron Reactors Based on Three Criteria" Annals Nucl.Energy. (in print).

[Publications] S.Nagasaki: "Influence of Fe(III) Coloids on NP(V) Migration through Quartz-Packed Columus" J.Nucl.Sci.Technol.31. 143-150 (1994)

[Publications] 鈴木篤之: "インポート・プレシアム法によるプルトニウム利用のセキュリティ効果の評価" 原子力学会誌. 36. 245-252 (1994)

[Publications] 鈴木篤之: "レプリケータモデルによる電源構成の最適化" エネルギー・資源. 15. 302-309 (1994)

[Publications] A.Suzuki: "Managing the Plutonium Surplus:Applications and Technical Options" Kluwer Academic Publishers, 219 (1994)

[Publications] A.Suzuki: "Managing the Plutonium Surplus:Applications and Technical Options" Kluwer Academic Publishers, 219 (1994)

木村逸郎京都大学, 工学部, 教授 (40027404)