Catalyst Development for On-Site GTL Process Using Integrated Tool of In-Situ Surface Observation and High Throughput Screening

2009 Fiscal Year Final Research Report

• Project/Area Number: 17106011
• Research Category: Grant-in-Aid for Scientific Research (S)
• Allocation Type: Single-year Grants
• Research Field: Catalyst/Resource chemical process
• Research Institution: Tohoku University
• Principal Investigator: YAMADA Muneyoshi Tohoku University, 校長 (40091764)
• Co-Investigator(Kenkyū-buntansha): OMATA Kohji 東北大学, 大学院・工学研究科, 准教授 (70185669) ; TOMISHIGE Keiichi 筑波大学, 大学院・数理物質科学研究科, 准教授 (50262051) ; KOIZUMI Naoto 東北大学, 大学院・工学研究科, 准教授 (50302188) ; SHINDO Takayoshi 秋田大学, 工学資源学部, 准教授 (50162798) ; MARUYAMA Kohichi 秋田工業高等専門学校, 物質工学科, 准教授 (90302934) ; NONAKA Risehiro 秋田工業高等専門学校, 物質工学科, 助教 (20400525)
• Project Period (FY): 2005 – 2009
• Keywords: High Throughput Screening(HTS) / In-situ表面観察 / 高活性 / 高選択性触媒

Research Abstract

Development of on-site GTL process where natural gas from unused dispersed carbon resources is converted into ultra clean transportation fuel is one of the ultimate solution for trilemma of energy security, environment, and economy issues. In this work, High Throughput Screening method and in-situ catalyst surface observation technique were integrated to develop highly active and selective catalysts for the on-site GTL process.

Research Products

• [Journal Article] (2010)
  • Author(s): Muneyoshi Yamada
  • Journal Title: J. Jpn. Inst. Ener. 89 Pages: 194-199
  • Peer Reviewed
• [Journal Article] (2010)
  • Author(s): Kobayashi, Yasukazu, Omata, Kohji, Yamada, Muneyoshi
  • Journal Title: INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 49 Pages: 1541-1549
  • Peer Reviewed
• [Journal Article] (2010)
  • Author(s): Junpei Horiguchi, Seishiro Kobayashi, Yuichiro Yamazaki, Takayuki Nakanishi, Daisuke Itabashi, Kohji OMATA, Muneyoshi Yamada
  • Journal Title: Applied Catalysis A: General 377 Pages: 9-15
  • Peer Reviewed
• [Journal Article] (2009)
  • Author(s): Naoto Koizumi, Takehisa Mochizuki, Muneyoshi Yamada
  • Journal Title: J. Surf Sci Nanotech. 7 Pages: 633-640
  • Peer Reviewed
• [Journal Article] (2009)
  • Author(s): Naoto Koizumi, Takehisa Mochizuki, Muneyoshi Yamada
  • Journal Title: Catalysis Today 141 Pages: 34-42
  • Peer Reviewed
• [Journal Article] (2009)
  • Author(s): Wensheng Ning, Naoto Koizumi, Muneyoshi Yamada
  • Journal Title: Energy Fuels 23 Pages: 4696-4700
  • Peer Reviewed
• [Journal Article] (2009)
  • Author(s): Kohji Omata, Hidetomo Ishii, Junpei Horiguchi, Seishiro Kobayashi, Yuichiro, Yamazaki, Muneyoshi Yamada
  • Journal Title: Journal of Combinatorial Chemistry 11 Pages: 169-174
  • Peer Reviewed
• [Journal Article] (2009)
  • Author(s): Kohji Omata, Yasukazu Kobayashi, Muneyoshi Yamada
  • Journal Title: Energy Fuels 23 Pages: 1931-1935
  • Peer Reviewed
• [Journal Article] (2009)
  • Author(s): Kohji Omata, Akihiro Masuda, Hidetomo Ishii, Hikotaro Suzuki, Muneyoshi Yamada
  • Journal Title: Applied Catalysis A: General 362 Pages: 14-19
  • Peer Reviewed
• [Journal Article] (2009)
  • Author(s): Kohji Omata, Muneyoshi Yamada
  • Journal Title: Journal of the Japan Petroleum Institute 52,2 Pages: 65-69
  • Peer Reviewed
• [Journal Article] (2008)
  • Author(s): Takehisa Mochizuki, Daichi Hongo, Takuya Satoh, Naoto Koizumi, Muneyoshi Yamada
  • Journal Title: Catalysis Letters 121 Pages: 52-57
  • Peer Reviewed
• [Journal Article] (2008)
  • Author(s): Takehisa MOCHIZUKI, Takuya SATO, Daichi HONGO, Naoto KOIZUMI, Muneyoshi YAMADA
  • Journal Title: Journal of the Japan Institute of Energy 87 Pages: 132-138
  • Peer Reviewed
• [Journal Article] (2008)
  • Author(s): Takehisa MOCHIZUKI, Hiroki OSANAI, Takuya SATO, Daichi HONGO, Naoto KOIZUMI, Muneyoshi YAMADA
  • Journal Title: Journal of the Japan Institute of Energy 87 Pages: 124-131
  • Peer Reviewed
• [Journal Article] (2008)
  • Author(s): Tetsuo Umegaki, Akihiro Masuda, Kohji Omata, Muneyoshi Yamada
  • Journal Title: Applied Catalysis A: General 351 Pages: 210-216
  • Peer Reviewed
• [Journal Article] (2008)
  • Author(s): Kohji Omata, Yosuke Endo, Hidetomo Ishii, Akihiro Masuda, Muneyoshi Yamada
  • Journal Title: Applied Catalysis A: General 351 Pages: 54-58
  • Peer Reviewed
• [Journal Article] (2007)
  • Author(s): Takehisa MOCHIZUKI, Naoto KOIZUMI, Yusuke HAMABE, Takeshi HARA, Hirotsugu TAKIZAWA, Muneyoshi YAMADA
  • Journal Title: Journal of the Japan Petroleum Institute 50,5 Pages: 262-271
  • Peer Reviewed
• [Journal Article] (2007)
  • Author(s): Takehisa Mochizuki, Takeshi Hara, Naoto Koizumi, Muneyoshi Yamada
  • Journal Title: Applied Catalysis A: General 317 Pages: 97-104
  • Peer Reviewed
• [Journal Article] (2007)
  • Author(s): Takehisa Mochizuki, Takeshi Hara, Naoto Koizumi, Muneyoshi Yamada
  • Journal Title: Catalysis Letters 113 Pages: 165-169
  • Peer Reviewed
• [Journal Article] (2007)
  • Author(s): Wen-Sheng Ning, Naoto Koizumi, Muneyoshi Yamada
  • Journal Title: Catalysis Communications 8 Pages: 275-278
  • Peer Reviewed
• [Journal Article] (2007)
  • Author(s): K. Omata, Y. Kobayashi, M. Yamada
  • Journal Title: Catalysis Communications 8 Pages: 1-5
  • Peer Reviewed
• [Journal Article] (2006)
  • Author(s): Wensheng Ning, Naoto Koizumi, Chang-Hai, Takehisa Mochizuki, Takashi Itoh, Muneyoshi Yamada
  • Journal Title: Applied Catalysis A: General 312 Pages: 35-44
  • Peer Reviewed
• [Journal Article] (2006)
  • Author(s): Kohji OMATA, Akihiro MASUDA, Takahisa MOCHIZUKI, YuhsukeWATANABE, Sutarto, Yasukazu KOBAYASHI, Muneyoshi YAMADA
  • Journal Title: Journal of the Japan Petroleum Institute 49,4 Pages: 214-217
  • Peer Reviewed
• [Journal Article] (2006)
  • Author(s): Kohji Omata, Yasukazu Kobayashi, Muneyoshi Yamada
  • Journal Title: Catalysis Today 117 Pages: 311-315
  • Peer Reviewed
• [Journal Article] (2005)
  • Author(s): Kohji Omata, Yasukazu Kobayashi, Muneyoshi Yamada
  • Journal Title: Catalysis Communications 6 Pages: 563-567
  • Peer Reviewed
• [Journal Article] (2005)
  • Author(s): Kohji Omata, Noritoshi Nukui, Muneyoshi Yamada
  • Journal Title: INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 44 Pages: 296-301
  • Peer Reviewed
• [Journal Article]
  • Author(s): Kohji Omata, Seishiro Kobayashi, Junpei Horiguchi, Yuichiro Yamazaki, Daisuke Itabashi, Takayuki Nakanishi, Muneyoshi Yamada
  • Journal Title: Journal of the Japan Petroleum Institute (in-print)
  • Peer Reviewed
• [Presentation] (2009)
  • Author(s): K. Omata, S. Kobayashi, J. Horiguchi, D. Itabashi, M. Yamada
  • Organizer: The 12th Japan-Korea Syposium of Catalysis
  • Place of Presentation: Akita (Japan)
  • Year and Date: 2009-10-15
• [Presentation] (2009)
  • Author(s): 小泉直人
  • Organizer: 第104回触媒討論会
  • Place of Presentation: 宮崎(日本)
  • Year and Date: 2009-09-30
• [Presentation] (2009)
  • Author(s): 山田宗慶
  • Organizer: 日本化学会第3回関東支部大会
  • Place of Presentation: 東京(日本)
  • Year and Date: 2009-09-04
• [Presentation] (2009)
  • Author(s): Kohji Omata
  • Organizer: The 10th Japan-China Symposium on Coal and C1 Chemistry
  • Place of Presentation: つくば(日本)
  • Year and Date: 2009-07-28
• [Presentation] (2009)
  • Author(s): N. Koizumi, T. Satoh, D. Hongo, T. Mochizuki, M. Yamada
  • Organizer: The 10th Japan-China Symposium on Coal and C1 Chemistry
  • Place of Presentation: Tsukuba (Japan)
  • Year and Date: 2009-07-28
• [Presentation] (2009)
  • Author(s): Kohji Omata
  • Organizer: The 10th Japan-China Symposium on Coal and C1 Chemistry
  • Place of Presentation: Tsukuba (Japan)
  • Year and Date: 2009-07-28
• [Presentation] (2009)
  • Author(s): Junpei Horiguchi, Seishiro Kobayashi, Yuichiro Yamazaki, Takayuki Nakanishi, Kohji Omata, Muneyoshi Yamada
  • Organizer: The 10th Japan-China Symposium on Coal and C1 Chemistry
  • Place of Presentation: Tsukuba (Japan)
  • Year and Date: 2009-07-27
• [Presentation] (2008)
  • Author(s): N. Koizumi, D. Hongo, T. Satoh, T. Mochizuki, M. Yamada
  • Organizer: 14th ICC
  • Place of Presentation: Seoul (Korea)
  • Year and Date: 20080713-20080718
• [Presentation] (2008)
  • Author(s): N. Koizumi, T. Mochizuki, D. Hongo, M. Yamada
  • Organizer: International Symposium on Surface Science and Nanotechnology
  • Place of Presentation: Tokyo (Japan)
  • Year and Date: 2008-11-13
• [Presentation] (2008)
  • Author(s): N. Koizumi, D. Hongo, T. Satoh, T. Mochizuki, M. Yamada
  • Organizer: 236th ACS National Meeting
  • Place of Presentation: Philadelphia (USA)
  • Year and Date: 2008-08-17
• [Presentation] (2008)
  • Author(s): 山田宗慶
  • Organizer: 日本学術振興会石炭・炭素資源利用技術第148委員会第112回研究会
  • Place of Presentation: 東京(日本)
  • Year and Date: 2008-05-28
• [Presentation] (2007)
  • Author(s): T. Mochizuki, D. Hongo, T. Satoh, N. Koizumi, M. Yamada
  • Organizer: 12th Asian Chemical Congress
  • Place of Presentation: Kuala Lumpur (Malaysia)
  • Year and Date: 20070823-20070825
• [Presentation] Indo-US seminar (2007)
  • Author(s): M. Yamada
  • Organizer: 18th National Symposium on Catalysis
  • Place of Presentation: Dehradun (India)
  • Year and Date: 20070416-20070418
• [Presentation] (2007)
  • Author(s): 小俣光司
  • Organizer: 日本学術振興会石炭・炭素資源利用技術第148委員会第108回研究会
  • Place of Presentation: 化学会館(日本)
  • Year and Date: 2007-05-23
• [Presentation] (2007)
  • Author(s): K. Omata, A. Masuda, H. Ishii, M. Yamada
  • Organizer: The 11st Korea-Japan Symposium of Catalysis
  • Place of Presentation: Seoul (Korea)
  • Year and Date: 2007-05-22
• [Presentation] (2007)
  • Author(s): 山田宗慶
  • Organizer: 日本表面科学会東北・北海道支部講演会
  • Place of Presentation: 盛岡(日本)
  • Year and Date: 2007-03-13
• [Presentation] (2006)
  • Author(s): W. Ning, Hai-Chang, N. Koizumi, T. Mochizuki, T. Itoh, M. Yamada
  • Organizer: The 9th China-Japan Symposium on Coal and C1 Chemistry
  • Place of Presentation: Chengdu (China)
  • Year and Date: 20061022-20061028
• [Presentation] (2006)
  • Author(s): Takehisa Mochizuki, Hiroki Osanai, Chang-hai, Naoto Koizumi, Muneyoshi Yamada
  • Organizer: The 9th China-Japan Symposium on Coal and C1 Chemistry
  • Place of Presentation: Chengdu (China)
  • Year and Date: 20061022-20061028
• [Presentation] (2006)
  • Author(s): Kohji Omata, Akihiro Masuda, Hidetomo Ishii, Muneyoshi Yamada
  • Organizer: The 9th China-Japan Symposium on Coal and C1 Chemistry
  • Place of Presentation: Chengdu, China
  • Year and Date: 20061022-20061028
• [Presentation] (2006)
  • Author(s): Takehisa Mochizuki, Takeshi Hara, Chang-hai, Naoto Koizumi, Muneyoshi Yamada
  • Organizer: International Symposium on Zeolites and Microporous Crystals 2006 (ZMPC2006)
  • Place of Presentation: Tottori (Japan)
  • Year and Date: 20060730-20060802
• [Presentation] (2006)
  • Author(s): Takehisa Mochizuki, Takeshi Hara, Naoto Koizumi, Chang-hai, Muneyoshi Yamada
  • Organizer: TOCAT5
  • Place of Presentation: Tokyo (Japan)
  • Year and Date: 20060723-20060728
• [Presentation] (2006)
  • Author(s): Chang-hai, Wensheng Ning, Takeshi Hara, Takehisa Mochizuki, Naoto Koizumi, Muneyoshi Yamada
  • Organizer: TOCAT5
  • Place of Presentation: Tokyo (Japan)
  • Year and Date: 20060723-20060728
• [Presentation] (2006)
  • Author(s): K. Omata, N. Nukui, M. Yamada
  • Organizer: Fifth International Conference on Unsteady-State Processes in Catalysis
  • Place of Presentation: Osaka (Japan)
  • Year and Date: 2006-11-24
• [Presentation] (2006)
  • Author(s): Kohji Omata, Akihiro Masuda, Hidetomo Ishii, Muneyoshi Yamada
  • Organizer: The 9th China-Japan Symposium on Coal and C1 Chemistry
  • Place of Presentation: Sichuan, Chengdu (China)
  • Year and Date: 2006-10-24
• [Presentation] (2006)
  • Author(s): Kohji Omata, Akihiro Masuda, Hidetomo Ishii, Takehisa Mochizuki, Yuhsuke Watanabe, Sutarto, Yasukazu Kobayashi, Muneyoshi Yamada
  • Organizer: Tokyo Conference on Advanced Catalytic Science and Technology
  • Place of Presentation: Tokyo (Japan)
  • Year and Date: 2006-07-28
• [Presentation] (2006)
  • Author(s): Muneyoshi Yamada
  • Organizer: TOCAT 5
  • Place of Presentation: 東京(日本)
  • Year and Date: 2006-07-22
• [Presentation] (2005)
  • Author(s): Takehisa Mochizuki, Takeshi Hara, Naoto Koizumi, Wensheng Ning, Chang-hai, Muneyoshi Yamada
  • Organizer: PACIFICHEM 2005
  • Place of Presentation: Honolulu (USA)
  • Year and Date: 20051215-20051222
• [Presentation] (2005)
  • Author(s): Takehisa Mochizuki, Naoto Koizumi, Muneyoshi Yamada
  • Organizer: The International 21st Century COE Symposium of BINDEC Chemistry Network
  • Place of Presentation: Osaka (Japan)
  • Year and Date: 2005-10-11
• [Presentation] (2005)
  • Author(s): K. Omata, Y. Kobayashi, M. Yamada
  • Organizer: 5th World Congress on Oxidation Catalysis
  • Place of Presentation: Sapporo (Japan)
  • Year and Date: 2005-09-26
• [Presentation] (2005)
  • Author(s): K. Omata, N. Nukui, T. Hottai, Y. Showa, M. Yamada
  • Organizer: 5th World Congress on Oxidation Catalysis
  • Place of Presentation: Sapporo (Japan)
  • Year and Date: 2005-09-25
• [Book] 新エネルギーとバイオマスエネルギーの技術と市場2010 (2010)
  • Author(s): 小泉直人, 山田宗慶
  • Total Pages: 3-15
  • Publisher: シーエムシー出版
• [Book] Advances in Fischer-Tropsch Synthesis, Catalysts (2009)
  • Author(s): Naoto Koizumi, Daichi Hongo, Yukiya Ibi, Yasuhiko Hayasaka, Muneyoshi Yamada
  • Total Pages: 95-118
  • Publisher: CRC Press
• [Book] クリーンディーゼル開発の要素技術動向 (2008)
  • Author(s): 山田宗慶, 小泉直人, 濱邊雄輔
  • Total Pages: 267-282
  • Publisher: エヌティーエス
• [Book] Fischer-Tropsch合成用Co触媒の開発に関する最近の動向 (2008)
  • Author(s): 小泉直人, 山田宗慶
  • Total Pages: 5-17
  • Publisher: 月刊ファインケミカル
• [Book] メタン高度化学変換技術集成 (2008)
  • Author(s): 小俣光司, 山田宗慶
  • Total Pages: 1-14
  • Publisher: シーエムシー出版
• [Book] Ultraclean Transportation Fuels (2007)
  • Author(s): Naoto Koizumi, Kazuhito Murai, Satoshi Takasaki, Muneyoshi Yamada
  • Total Pages: 119-134
  • Publisher: American Chemical Society
• [Book] 化学と工業(クリーン燃料合成触媒開発におけるコンビナトリアルケミストリー, Vol.58, No.3) (2005)
  • Author(s): 小俣光司
  • Total Pages: 229-230
• [Book] Syngas: Production Methods(Post Treatment and Economics)
  • Author(s): Naoto Koizumi, Takehisa Mochizuki, Diaich Hongo, Muneyoshi Yamada
  • Publisher: Nova Science Publishers(in-print)
• [Remarks] ホームページ等
  • URL: http://www.che.tohoku.ac.jp/labo/Yamada/index-j.html
• [Patent(Industrial Property Rights)] 一酸化炭素還元用触媒、その製造方法および炭化水素の製造方法 (2007)
  • Inventor(s): 山田宗慶, 小泉直人, 望月剛久, 本郷大地
  • Industrial Property Rights Holder: 東北大学
  • Industrial Property Number: 特許
  • Filing Date: 2007-07-04
  • Acquisition Date: 2007-07-04
• [Patent(Industrial Property Rights)] Fischer-Tropsch合成用触媒の調製法 (2006)
  • Inventor(s): 山田宗慶, 小泉直人, 望月剛久
  • Industrial Property Rights Holder: 東北大学
  • Industrial Property Number: 特許
  • Filing Date: 2006-11-24
  • Acquisition Date: 2006-11-24