Heavy Ion Irradiation Effects on Fuel Simulation Materials Doped with Impurities

2012 Fiscal Year Final Research Report

• Project/Area Number: 21360469
• Research Category: Grant-in-Aid for Scientific Research (B)
• Allocation Type: Single-year Grants
• Section: 一般
• Research Field: Nuclear engineering
• Research Institution: Osaka Prefecture University
• Principal Investigator: IWASE Akihiro 大阪府立大学, 工学研究科, 教授 (60343919)
• Co-Investigator(Kenkyū-buntansha): HORI Fuminobu 大阪府立大学, 工学研究科, 准教授 (20275291) ; OKAMOTO Yoshihiro 独立行政法人・日本原子力研究開発機構, 量子応用部門, 研究主幹 (70370369) ; ISHIKAWA Norito 独立行政法人・日本原子力研究開発機構, 原子力基礎部門, 研究主幹 (90354828) ; SASAJIMA Yasushi 茨城大学, 工学部, 教授 (80187137)
• Project Period (FY): 2009 – 2012
• Keywords: 原子力材料 / 核燃料

Research Abstract

To simulate the effect of high energy fission fragments on nuclear fuels doped with burnable poisons, we doped CeO2 with Gd2O3or Er2O3 and irradiated them with high energy heavy ions. The change in lattice structures by the irradiation was studied. We have found that the doping of GdO3 or Er2O3 enhanced the irradiation effect. The result of the computer simulation showed that the irradiation mainly destroyed the oxygen atom arrangements and the disordering of oxygen atom arrangement in UO2 is much stable than in CeO2.

Research Products

• [Journal Article] Computer simulation of structural modifications induced by highly energetic ions in uranium dioxide (2013)
  • Author(s): Y.Sasajima, T.Osada, N.Ishikawa, A. Iwase
  • Journal Title: Nucl. Instr. Meth. B Volume: accepted for publication
• [Journal Article] Molecular dynamics simulation of fast particle irradiation on the single crystal CeO_2 (2013)
  • Author(s): Y.Sasajima, N.Ajima, T.Osada, N.Ishikawa, A. Iwase
  • Journal Title: Nucl. Instrm. Meth. B Volume: accepted for publication
• [Journal Article] Effects of high-energy heavy ion irradiation on the crystal structure in CeO_2thin films (2013)
  • Author(s): T.Kishino, K.Shimizu, Y,Saitoh, N.Ishikawa, F.Hori, ,A,Iwase
  • Journal Title: Nucl. Instrm. Meth. B Volume: accepted for publication
  • DOI: DOI:http://dx.doi.org/10.1016/j.nimb.2013.04.028
• [Journal Article] Change in magnetic properties induced by swift heavy ion irradiation in CeO_2 (2012)
  • Author(s): K.Shimizu, S.Kosugi, Y.Tahara, K.Yasunaga, Y.Kaneta, N.Ishikawa, F.Hori, T.Matsui, A.Iwase
  • Journal Title: Nucl. Instr. Meth. B Volume: 286 Pages: 291-294
  • DOI: DOI:10.1016/j.nimb.2012.01.008
• [Journal Article] Study on effects of energetic ion irradiation in Gd2O3-doped CeO2 by means of synchrotron radiation X-ray spectroscopy (2012)
  • Author(s): Y.Tahara, K.Shimizu, N.Ishikawa, Y.Okamoto, F.Hori, T.Matsu, A.Iwase
  • Journal Title: Nucl. Instr. Meth. B Volume: 277 Pages: 53-57
  • DOI: DOI:10.1016/j.nimb.2011.12.048
• [Journal Article] Study on effects of swift heavy ion irradiation on the crystal structure in CeO_2 doped with Gd_2O_3 (2011)
  • Author(s): Y. Tahara, B. Zhu, S. Kosugi, N. Ishikawa, Y. Okamoto, F. Hori, T. Matsui, A. Iwase
  • Journal Title: Nucl. Instr. Meth. B Volume: 269 Pages: 886-889
  • DOI: DOI:10.1016/j.nimb.2010.12.032
• [Journal Article] Effects of swift heavy ion irradiation on the structure of Er_2O_3-doped CeO_2 (2010)
  • Author(s): B. Zhu, H. Ohno, S. Kosugi, F. Hori, K. Yasunaga, N. Ishikawa, A. Iwase
  • Journal Title: Nucl. Instr. Meth. B Volume: 268 Pages: 3199-3202
  • DOI: DOI:10.1016/j.nimb.2010.05.088
• [Journal Article] Study on analysis of crystal structure in CeO_2doped with Er_2O_3or Gd_2O_3 (2010)
  • Author(s): B. Zhu, Y.Tahara, K.Yasunaga, T.Matsui, F.Hori, A. Iwase
  • Journal Title: J. Rare Earths Volume: 28 Pages: 164-167
  • DOI: DOI:10.1016/S1002-0721(10)60378-X
• [Presentation] Effects of swift heavy ion irradiation and high temperature annealing on the structure and magnetic propeties of CeO2 (2012)
  • Author(s): K. Shimizu, T. Kishino Y. Tahara, K. Yasunaga, N. Ishikawa, Y. Okamoto, Y. Baba, N. Hirao, Y. Saitoh, F. Hori, T. Matsui, A. Iwase
  • Organizer: 8th International Symposium on Swift Heavy Ions in Matter
  • Place of Presentation: Kyoto, Japan
  • Year and Date: 2012-10-26
• [Presentation] Effects of Gd2O3 doping and swift heavy ion irradiation on CeO2 bulk pellets and thin films (2012)
  • Author(s): A. Iwase, T. Kishino, K. Shimizu, Y. Tahara, F. Hori, T. Matsui, N. Ishikawa, Y. Okamoto
  • Organizer: 8th International Symposium on Swift Heavy Ions in Matter
  • Place of Presentation: Kyoto, Japan
  • Year and Date: 2012-10-26
• [Presentation] Computer simulation of high-energy-ion irradiation of uranium dioxide (2012)
  • Author(s): Y.Sasajima, T.Osada, N.Ishikawa, A. Iwase
  • Organizer: 8th International Symposium on Swift Heavy Ions in Matter
  • Place of Presentation: Kyoto, Japan
  • Year and Date: 2012-10-26
• [Presentation] Computer simulation of high energy beam of ceria (2012)
  • Author(s): Y.Sasajima, N.Ajima, T.Osada, N.Ishikawa, A. Iwase
  • Organizer: 8th International Symposium on Swift Heavy Ions in Matter
  • Place of Presentation: Kyoto, Japan
  • Year and Date: 2012-10-26
• [Presentation] Computer Simulation of High Energy Beam Irradiation of Ceria and Uranium Dioxide (2012)
  • Author(s): Y.Sasajima, T.Osada, N.Ajima, N. Ishikawa A.Iwase
  • Organizer: IUMRS-ICEM
  • Place of Presentation: Yokohama, Japan
  • Year and Date: 2012-09-25
• [Presentation] RF スパッタリング法で作製した CeO_2薄膜の高エネルギー重イオン照射効果 (2012)
  • Author(s): 岸野孝典,石川法人,斉藤勇一,清水浩貴,堀史説,岩瀬彰宏
  • Organizer: 日本物理学会秋季大会
  • Place of Presentation: 横浜
  • Year and Date: 2012-09-19
• [Presentation] 単結晶への高速粒子線照射の分子動力学シミュレーション (2012)
  • Author(s): 安島直紀,長田卓也,篠嶋妥,石川法人,岩瀬彰宏
  • Organizer: 日本金属学会秋季大会
  • Place of Presentation: 松山
  • Year and Date: 2012-09-19
• [Presentation] Gd_2O_3添加 CeO_2への高速粒子線照射に関する分子動力学シミュレーション (2012)
  • Author(s): 長田卓也,安島直紀,篠嶋妥,石川法人,岩瀬彰宏
  • Organizer: 日本金属学会秋季大会
  • Place of Presentation: 松山
  • Year and Date: 2012-09-19
• [Presentation] Modification of Magnetic Properties of CeO_2by using swift heavy ion irradiation (2011)
  • Author(s): K. Shimizu, Y. Tahara, K. Yasunaga, N. Ishikawa, Y. Baba, N. Hirao, Y. Okamoto, F. Hori, Y. Kaneta ,T. Matsui, A. Iwase
  • Organizer: 21th MRS-J Academic Symposium
  • Place of Presentation: Yokohama, Japan
  • Year and Date: 2011-12-20
• [Presentation] UO_2の高エネルギービーム照射に関するシミュレーション実験 (2011)
  • Author(s): 長田卓也、小貫英昭、篠嶋 妥、石川法人、岩瀬彰宏
  • Organizer: 日本金属学会秋季大会
  • Place of Presentation: 沖縄
  • Year and Date: 2011-11-08
• [Presentation] SiO_2の高エネルギービーム照射によるトラック形成シミュレーション (2011)
  • Author(s): 小貫英昭、篠嶋 妥、岩瀬彰宏
  • Organizer: 日本金属学会秋季大会
  • Place of Presentation: 沖縄
  • Year and Date: 2011-11-08
• [Presentation] 高速イオンビームによる固体内高密度励起反応と物質改質への応用 (2011)
  • Author(s): 岩瀬彰宏
  • Organizer: 第7回励起ナノプロセス研究会
  • Place of Presentation: 大阪
  • Year and Date: 2011-11-01
• [Presentation] 高エネルギーイオンと物質の相互作用-その基礎過程と物質改質への応用- (2011)
  • Author(s): 岩瀬彰宏
  • Organizer: 日本原子力学会九州支部講演会
  • Place of Presentation: 福岡
  • Year and Date: 2011-09-28
• [Presentation] 高速重イオンビームによる CeO_2の磁性制御 (2011)
  • Author(s): 岩瀬彰宏,清水浩貴,堀史説,松井利之,石川法人,金田保則
  • Organizer: 日本物理学会秋季大会
  • Place of Presentation: 富山
  • Year and Date: 2011-09-21
• [Presentation] 高速重イオン照射による原子力材料の特性分析 (2011)
  • Author(s): 岩瀬彰宏
  • Organizer: 第21回格子欠陥フォーラム
  • Place of Presentation: 立山
  • Year and Date: 2011-09-20
• [Presentation] Effects of MeV-GeV ion irradiations on Gd_2O_3-doped CeO_2 (2011)
  • Author(s): Y.Tahara, K.Shimizu, N.Ishikawa, Y.Okamoto, Y.Baba,N. Hirao,Y. Saitoh, R. Neumann, C. Trautmann, F. Hori, T. Matsui, A. Iwase
  • Organizer: 16th International Conference on Radiation Effects in Insulators
  • Place of Presentation: Beijing, China
  • Year and Date: 2011-08-16
• [Presentation] Change in magnetic properties induced by swift heavy ion irradiation in CeO_2 (2011)
  • Author(s): K. Shimizu,S. Kosugi, Y. Tahara, K. Yasunaga, Y. Kaneta, N. Ishikawa, F. Hori, T. Matsui,A. Iwase
  • Organizer: International Conference on Radiation Effects in Insulators
  • Place of Presentation: Beijing, China
  • Year and Date: 2011-08-16
• [Presentation] Study on Effects of Energetic Ion Irradiation in Gd_2O_3-doped CeO_2by Means of Synchrotron Radiation X-ray Spectroscopy (2011)
  • Author(s): Y.Tahara, K.Shimizu, N.Ishikawa, Y.Okamoto, F. Hori, T. Matsui, A.Iwase
  • Organizer: European Materials Research Society Spring Meeting
  • Place of Presentation: Nice, France
  • Year and Date: 2011-05-10
• [Presentation] UO2の高エネルギービーム照射によるトラック形成の解析 (2011)
  • Author(s): 長田卓也、小貫英昭、篠嶋妥、石川法人、岩瀬彰宏
  • Organizer: 日本金属学会春季大会
  • Year and Date: 2011-03-26
• [Presentation] Interaction between energetic ions and solids, -fundamental study and their application to the modification of magnetic properties of materials (2011)
  • Author(s): A.Iwase
  • Organizer: Workshop on Osaka University HVEM
  • Place of Presentation: 大阪
  • Year and Date: 2011-01-28
• [Presentation] Computer Simulation on high-energy-beam irradiation of Uranium dioxide (2010)
  • Author(s): H.Onuki, Y.Sasajima, N.Ishikawa, A. Iwase
  • Organizer: 20th MRS-J Academic Symposium
  • Place of Presentation: Yokohama, Japan
  • Year and Date: 2010-12-21
• [Presentation] Computer simulation of high energy beam irradiation of single crystalline silicon and β-cristobalite (2010)
  • Author(s): H.Ohuki, Y.Sasajima, N.Ishikawa, A. Iwase
  • Organizer: 20th MRS-J Academic Symposium
  • Place of Presentation: Yokohama, Japan
  • Year and Date: 2010-12-21
• [Presentation] 高エネルギー重イオン照射による CeO_2への磁性付加京都大学原子炉実験所材料照射効果の解明と照射技術の高度化ワークショップ (2010)
  • Author(s): 清水浩貴、松井利之、小杉晋也、田原佑規、藤田直樹、堀史説、岩瀬彰宏
  • Place of Presentation: 大阪
  • Year and Date: 2010-12-17
• [Presentation] Gd2O3, Er2O3をドープしたCeO2の高速重イオン照射効果 (2010)
  • Author(s): 田原佑規、岩瀬彰宏
  • Organizer: 日本原子力懇談会
  • Place of Presentation: 大阪
  • Year and Date: 2010-12-17
• [Presentation] SiO2 の高エネルギービーム照射によるトラック形成の解析 (2010)
  • Author(s): 小貫英昭、篠嶋妥、岩瀬彰宏
  • Organizer: 日本金属学会秋季大会
  • Place of Presentation: 札幌
  • Year and Date: 2010-09-26
• [Presentation] Gd2O3 を添加した CeO2 における高エネルギー重イオン照射効果 (2010)
  • Author(s): 田原佑規、朱宝琳、小杉晋也、堀史説、松井利之、岩瀬彰宏、石川法人、岡本芳浩、馬場祐治、平尾法恵
  • Organizer: 日本金属学会秋季大会
  • Place of Presentation: 札幌
  • Year and Date: 2010-09-25
• [Presentation] Study on analysis of crystal structure in CeO_2doped with Er_2O_3or Gd_2O_3 (2010)
  • Author(s): B. Zhu, Y. Tahara, K. Yasunaga, T. Matsui, F. Hori, A. Iwase
  • Organizer: 6th International Conference Rare Earth Development and Application
  • Place of Presentation: Beijing, China
  • Year and Date: 2010-08-08
• [Presentation] SiO_2の高エネルギービーム照射に関する分子動力学シミュレーション (2010)
  • Author(s): 小貫英昭 、篠嶋妥 、岩瀬彰宏
  • Organizer: 日本金属学会春季大会
  • Place of Presentation: 筑波
  • Year and Date: 2010-03-29
• [Presentation] Er_2O_3をドープしたCeO_2の高エネルギー重イオン照射効果 (2009)
  • Author(s): 朱 宝琳、大野裕隆、堀 史説、安永和史、石川法人、岩瀬彰宏
  • Organizer: 量子理工学研究実験センター第10回QSEC公開シンポジウム
  • Place of Presentation: 京都
  • Year and Date: 2009-10-23
• [Presentation] CeO_2の高エネルギー重イオン照射効果におけるEr_2O_3添加の影響 (2009)
  • Author(s): 朱宝琳、大野裕隆、岩瀬彰宏、安永和史、石川法人
  • Organizer: 日本金属学会秋季大会
  • Place of Presentation: 京都
  • Year and Date: 2009-09-17
• [Presentation] Effects of swift heavy ion irradiation on the structure of Er2O3-doped CeO2 (2009)
  • Author(s): A. Iwase, B. Zhu, N. Ishikawa, T. Matsui
  • Organizer: 15th International Conference on Radiation Effects on Insulators
  • Place of Presentation: Padova ,Italy
  • Year and Date: 2009-09-01