Investigations of couplings between are earth quadrupolar orderings and lattice vibrations by dichromatic neutron diffraction

2011 Fiscal Year Final Research Report

• Project/Area Number: 21540350
• Research Category: Grant-in-Aid for Scientific Research (C)
• Allocation Type: Single-year Grants
• Section: 一般
• Research Field: Condensed matter physics II
• Research Institution: Tohoku University
• Principal Investigator: OHOYAMA Kenji 東北大学, 金属材料研究所, 准教授 (60241569)
• Co-Investigator(Kenkyū-buntansha): HIRAKA Haruhiro 東北大学, 金属材料研究所, 助教 (90323097)
• Co-Investigator(Renkei-kenkyūsha): MATSUOKA Eiichi 神戸大学, 理学部, 准教授 (20400228)
• Project Period (FY): 2009 – 2011
• Keywords: 強相関系 / 多極子秩序

Research Abstract

The main purpose of this project was to clarify couplings between lattice and quadrupole and magnetic orderings in rare earth antiferroquadrupolar ordering compounds through observations of thermal vibrations of nucleus and magnetic moments. For the observations, we proposed dichromatic neutron using two different wave lengths. We succeeded in upgrading a neutron powder diffractometer by this project. High resolution diffraction experiments with lower wave length, and wide -Q diffraction experiments with high wave length have been feasible on one diffractometer. Though the main experiments could not be performed because of the earthquake, feasibility of the wide-Q experiments with dichromatic beams has been confirmed. Moreover, by the upgrades, neutron holography experiments, and polarised neutronexperiments are realised on the powder diffractometer.

Research Products

• [Journal Article] Development of a non-adiabatic two-coil spin flipper for a polarised thermal neutron diffractometer with a 3He spin filter (2012)
  • Author(s): K. Ohoyama, K. Tsutsumi,T. Ino, H. Hiraka, Y. Yamaguchi, H. Kira, T. Oku, Y. Sakaguchi, Y. Arimoto,W. Zhang, H. Kimura, K. Iwasa,M. Takeda, J. Suzuki, K. Yamada, K. Kakurai, Nucl
  • Journal Title: Meth. Phys. Res A Volume: 680 Pages: 75-81
  • DOI: DOI:10.1016/j.nima.2012.04.018
• [Journal Article] Modified cross-correlation for efficient white-beam inelastic neutron scattering spectroscopy (2012)
  • Author(s): K. Tomiyasu, M. Matsuura, H. Kimura, K. Iwasa, K. Ohoyama, T. Yokoo,S. Ioth, E. Kudoh, T. Sato, M. Fujita, Nucl.
  • Journal Title: Instrum. Meth. Phys. Res. Volume: A 677 Pages: 89-93
  • DOI: DOI:10.1016/j.nima.2012.03.001
• [Journal Article] 新しい局所構造解析技術としての原子分解能中性子線ホログラフィー (2012)
  • Author(s): 林好一、大山研司
  • Journal Title: 表面科学 Volume: 33 Pages: 290-295
• [Journal Article] Magnetic and Neutron Diffraction Study on Melilite-Type Oxides Sr_2MGe_2O_7 (M = Mn, Co) (2012)
  • Author(s): T. Endo, Y. Doi, Y. Hinatsu, and K. Ohoyama
  • Journal Title: Inorg. Chem Volume: 51 Pages: 3572-3578
  • DOI: DOI:10.1021/ic202386h
• [Journal Article] High Field Neutron Diffraction Studies On Metamagnetic Transition Of Multiferroic BiFeO_3 (2011)
  • Author(s): K. Ohoyama, S. Lee, S. Yoshii, Y. Narumi,T.
  • Journal Title: Morioka, H. Nojiri, G. S. Jeon, S-W Cheong, and J-G Park J. Phys. Soc. Jpn Volume: 80 Pages: 125001(1)-(2)
  • DOI: DOI:10.1143/JPSJ.80.125001
• [Journal Article] Importance of Neutron Scattering for Materials Science: Expectations on Magnetic Holography (2011)
  • Author(s): K. Ohoyama, K. Hayashi, H. Hiraka
  • Journal Title: e-Journal of Surface Science and Nanotechnology Volume: 9 Pages: 422-425
  • URL: http://dx.doi.org/10.1380/ejssnt.2011.422
• [Journal Article] Hot pressing of Ge crystals toward a reflection-plane-selective neutron monochromator (2010)
  • Author(s): Y. Miyake, H. Hiraka, Y. Yamaguchi, K. Ohoyama, K. Yamada, J. Phys.
  • Journal Title: Conf. Ser Volume: 200 Pages: 112006(1)-(4)
  • DOI: doi:10.1088/1742-6596/200/11/112006
• [Journal Article] Universal Magnetic Structure of theHalf-Magnetization Phase in Cr-Based Spinels (2010)
  • Author(s): M. Matsuda, K. Ohoyama, S. Yoshii, H. Nojiri, P. Frings, F. Duc, B. Vignolle, G. L. J. A. Rikken, L.-P. Regnault4, S.-H. Lee, H. Ueda, and Y. Ueda
  • Journal Title: Phys. Rev. Lett Volume: 104 Pages: 047201(1)-(4)
  • DOI: DOI:10.1103/PhysRevLett.104.04720
• [Journal Article] Antiferromagnetic Alignment of Magnetic Dipolar Moments Observed by Neutron Powder Diffraction in Rare-Earth Palladium Bronze PrPd_3S_4 (2010)
  • Author(s): E. Matsuoka, D. Usui, Y. Sasaki, Watahiki, K.Iwasa, H. Shida, K. Ohoyama, H. Onodera
  • Journal Title: J. Phys. Soc. Jpn Volume: 79 Pages: 64708(1)-(4)
  • DOI: DOI:10.1143/JPSJ.79.064708
• [Journal Article] Multimode hydriding/dehydriding reactions of CaPd (2010)
  • Author(s): K. Ikeda, N. Okuda, K. Ohoyama, H.W. Li, H.T. Takeshita, T. Otomo, S. Orimo
  • Journal Title: Chem. Commun Volume: 46 Pages: 8380-8382
  • DOI: DOI:10.1039/C0CC02626C
• [Journal Article] Neutron Diffraction Study on the Multiple Magnetization Plateaus in TbB_4 under Pulsed High Magnetic Field (2009)
  • Author(s): S. Yoshii, K. Ohoyama, K. Kurosawa, H. Nojiri, M. Matsuda, P. Frings, F. Duc, B. Vignolle, G. L. Rikken, L.-P. Regnault, S. Michimura, and F
  • Journal Title: Iga Phys. Rev. Lett Volume: 103 Pages: 077203(1)-(4)
  • DOI: DOI:10.1103/PhysRevLett.103.077203
• [Presentation] 立方晶NdPd3S4の多極子物性III綿引正倫 (2012)
  • Author(s): 松岡英一,中村慎太郎,野島勉,大山研司,岩佐和晃,青木晴善,谷垣勝己,小野寺秀也
  • Organizer: 日本物理学会第66回年次大会
  • Place of Presentation: 新潟大学
  • Year and Date: 20120918-22
• [Presentation] 中性子回折による単結晶YbPdの磁気構造解析 (2012)
  • Author(s): 杉島正樹,光田暁弘,和田裕文,大山研司
  • Organizer: 日本物理学会第66回年次大会
  • Place of Presentation: 新潟大学
  • Year and Date: 20120918-22
• [Presentation] Neutron Holography Measurement as a Novel Probe of Local Structures of Spins and Light Atoms (2012)
  • Author(s): K. Ohoyama, K. Hayashi, T. Oku, T. Shinohara
  • Organizer: international workshop "3D atomic imaging at nano-scale active sites in materials"
  • Place of Presentation: 柏市
  • Year and Date: 20120806-08
• [Presentation] J-PARC偏極分光器POLANO計画およびHERMESでのSEOP偏極回折実験 (2012)
  • Author(s): 大山研司
  • Organizer: ISSPワークショップ定常中性子源三軸分光器の役割と偏極中性子散乱
  • Place of Presentation: 柏市
  • Year and Date: 20120723-24
• [Presentation] Polarised Neutron Diffraction System with a Transportable 3He Spin Filter on a Powder Diffractometer (2012)
  • Author(s): K. Ohoyama, K. Tsutsumi, T. Ino, H. Hiraka, Y. Yamaguchi, H. Kira, T. Oku, Y. Sakaguchie, W. Zhang, H. Kimura, M. Takeda, J. Suzuki, K. Yamada, K. Kakurai
  • Organizer: PNCMI 2012; Polarized Neutrons for Condensed Matter Investigations 2012
  • Place of Presentation: パリ、フランス
  • Year and Date: 20120702-05
• [Presentation] 反強磁性体(Mn,Fe)3Siにおける単結晶育成とその試料評価 (2012)
  • Author(s): 奈良壮,崔純彰,平賀晴弘,大山研司,山口泰男,堀金和正,山田和芳
  • Organizer: 日本物理学会第67回年次大会2
  • Place of Presentation: 関西学院大学
  • Year and Date: 20120324-27
• [Presentation] TmAu_2における強四極子秩序相の自発歪み (2010)
  • Author(s): 小坂昌史,志田裕,今成亜弥,片野進,大山研司,小野寺秀也
  • Organizer: 日本物理学会2010年秋季大会
  • Place of Presentation: 大阪府立大
  • Year and Date: 20100923-26
• [Presentation] AKANEとHERMESにおける装置改修計画と現状 (2010)
  • Author(s): 平賀晴弘,大山研司,山口泰男,山田和芳
  • Organizer: 日本物理学会2010年秋季大会
  • Place of Presentation: 大阪府立大
  • Year and Date: 20100923-26
• [Presentation] 東北大装置での偏極実験装置開発と応用実験の現状 (2010)
  • Author(s): 大山研司,堤健之,平賀晴弘,猪野隆,吉良弘,坂口佳史,奥隆之,有本靖,武田全康,鈴木淳市,堀金和正,岩佐和晃,F.Wu,窪田崇秀,水上成美,宮崎照宣,山田和芳,加倉井和久
  • Organizer: 日本物理学会2010年秋季大会
  • Place of Presentation: 大阪府立大
  • Year and Date: 20100923-26
• [Presentation] 偏極中性子を用いた鉄系合金の磁気散漫散乱の観測 (2010)
  • Author(s): 堤健之,大山研司,平賀晴弘,山口泰男,猪野隆,吉良弘,坂口佳史,奥隆之,有本靖B,武田全康,鈴木淳市,岩佐和晃,加倉井和久,山田和芳
  • Organizer: 日本物理学会2010年秋季大会
  • Place of Presentation: 大阪府立大
  • Year and Date: 20100923-26
• [Presentation] Shastry-Sutherland格子系TmB4における新奇な磁気秩序相 (2010)
  • Author(s): 道村真司,伊賀文俊,松村武,大山研司,山本昭二,道上勇一,綿貫徹,高畠敏郎
  • Organizer: 日本物理学会第65回年次大会
  • Place of Presentation: 岡山大学
  • Year and Date: 20100320-23
• [Presentation] 中性子散乱用Geモノクロメータ結晶の高度化III (2010)
  • Author(s): 平賀晴弘,三宅悠子A,山口泰男,大山研司,鬼柳亮嗣,木村宏之,野田幸男,山田和芳
  • Organizer: 日本物理学会第65回年次大会
  • Place of Presentation: 岡山大学
  • Year and Date: 20100320-23
• [Presentation] ^3Heスピンフィルター法を用いた偏極中性子散乱装置の開発 (2009)
  • Author(s): 大山研司,平賀晴弘,堤健之,猪野隆,奥隆之,吉良弘,坂口佳史,有本靖,武田全康,鈴木淳市,山田和芳,加倉井和久
  • Organizer: 日本物理学会2009年秋季大会
  • Place of Presentation: 熊本大学
  • Year and Date: 20090925-28
• [Presentation] 価数揺動物質YbPdの長周期磁気構造 (2009)
  • Author(s): 杉島正樹,光田暁弘,和田裕文,大山研司
  • Organizer: 日本物理学会2009年秋季大会
  • Place of Presentation: 熊本大学
  • Year and Date: 20090925-28
• [Presentation] Shastry-Sutherland格子系TmB4における長周期磁気構造の競合 (2009)
  • Author(s): 道村真司,松村武,大山研司,伊賀文俊,高畠敏郎
  • Organizer: 日本物理学会2009年秋季大会
  • Place of Presentation: 熊本大学
  • Year and Date: 20090925-28
• [Presentation] 立方晶TbPd_3S_4の多極子物性 (2009)
  • Author(s): 松岡英一,綿引正倫,大山研司,松村武,谷垣勝己,小野寺秀也
  • Organizer: 日本物理学会2009年秋季大会
  • Place of Presentation: 熊本大学
  • Year and Date: 20090925-28
• [Presentation] 中性子散乱用Geモノクロメータ結晶の高度化II (2009)
  • Author(s): 三宅悠子,平賀晴弘,山口泰男,大山研司,山田和芳
  • Organizer: 日本物理学会2009年秋季大会
  • Place of Presentation: 熊本大学
  • Year and Date: 20090925-28