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2013 Fiscal Year Final Research Report

Elucidation of pulsed laser-induced morphological changes of gold nanoparticles using transient absorption and single particle spectroscopies

Research Project

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Project/Area Number 23310065
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Nanostructural science
Research InstitutionThe University of Tokushima

Principal Investigator

HASHIMOTO Shuichi  徳島大学, ソシオテクノサイエンス研究部, 教授 (70208445)

Co-Investigator(Renkei-kenkyūsha) FURUBE Akihiro  独立行政法人産業技術総合研究所, 計測フロンティア研究部門, 主任研究員 (30357933)
UWADA Takayuki  奈良先端科学技術大学院大学, 物質創成科学研究科, 非常勤研究員 (30455448)
Research Collaborator WERNER Daniel  徳島大学, 大学院ソシオテクノサイエンス研究部, 徳島大学特別研究員(日本学術振興会特別研究員
Project Period (FY) 2011-04-01 – 2014-03-31
Keywordsナノ材料 / 金ナノ粒子 / レーザー / 光熱効果
Research Abstract

We focused our attention to the fundamental aspects of the laser-gold nanoparticle (Au NP) interaction that leads to the particle heating as well as energy deposition to the surrounding media. The former gives rise to the particle melting, deformation, and ablation, which has discussion on the mechanism. The latter generates medium temperature gradients and bubbles resulting from local heating through the heat transfer from the particle to the surroundings. The laser-Au NP interaction can be applied to the material fabrication such as fine tuning of particle size and size distribution by applying high pressures and nanohole fabrication on glass substrates. We also refer to the importance of temperature measurements in dimension smaller than the diffraction limit. We show that this can be achieved by CW laser-Au NP interaction by using the single particle spectroscopy.

  • Research Products

    (14 results)

All 2013 2012 2011 Other

All Journal Article (7 results) (of which Peer Reviewed: 7 results) Presentation (6 results) (of which Invited: 4 results) Remarks (1 results)

  • [Journal Article] Observation of Nanoscale Cooling Effects by Substrates and the Surrounding Media for Single Gold Nanoparticles under CW-laser Illumination2013

    • Author(s)
      K. Setoura, Y. Okada, D. Werner, S. Hashimoto
    • Journal Title

      ACS Nano

      Volume: Vol.7 Pages: 7874-7885

    • DOI

      10.1021/nn402863s

    • Peer Reviewed
  • [Journal Article] Controlling the pulsed-laser-induced size reduction of Au and Ag nanoparticles via changes in the external pressure, laser intensity, and excitation wavelength2013

    • Author(s)
      D. Werner, S. Hashimoto
    • Journal Title

      Langmuir

      Volume: Vol.29 Pages: 1295-1302

    • DOI

      10.1021/la3046143

    • Peer Reviewed
  • [Journal Article] Optical Scattering Spectral Thermometry and Refractometry of a Single Gold Nanoparticle under CW laser excitation2012

    • Author(s)
      K. Setoura, D. Werner, S. Hashimoto
    • Journal Title

      The Journal of Physical Chemistry C

      Volume: Vol.116 Pages: 15458-15466

    • DOI

      10.1021/jp304271d

    • Peer Reviewed
  • [Journal Article] Studies on the Interaction of Pulsed Lasers with Plasmonic Gold Nanoparticles toward Light Manipulation, Heat Management, and Nanofabrication2012

    • Author(s)
      S. Hashimoto, D. Werner, T. Uwada
    • Journal Title

      Journal of Photochemistry and Photobiology C : Reviews

      Volume: Vol.13 Pages: 28-54

    • DOI

      10.1016/j.jphotochemrev.2012.01.001

    • Peer Reviewed
  • [Journal Article] Femtosecond Laser-Induced Size Reduction of Aqueous Gold Nanoparticles : In situ and Pump-Probe Spectroscopy Investigations Revealing Coulomb Explosion2011

    • Author(s)
      D. Werner, A. Furube, T. Okamoto, S. Hashimoto
    • Journal Title

      The Journal of Physical Chemistry C

      Volume: Vol.115 Pages: 8503-8512

    • DOI

      10.1021/jp112262u

    • Peer Reviewed
  • [Journal Article] Improved working model for interpreting the excitation wavelength-and fluence-dependent response in nanosecond pulsed laser-induced size reduction of aqueous gold nanoparticles2011

    • Author(s)
      D. Werner, S. Hashimoto
    • Journal Title

      The Journal of Physical Chemistry C

      Volume: Vol.115 Pages: 5063-5072

    • DOI

      10.1021/jp109255g

    • Peer Reviewed
  • [Journal Article] Mechanistic aspect of surface modification on glass substrates assisted by single shot pulsed laser-induced fragmentation of gold nanoparticles2011

    • Author(s)
      S. Hashimoto, T. Uwada, M. Hagiri, R. Shiraishi
    • Journal Title

      The Journal of Physical Chemistry C

      Volume: Vol.115 Pages: 4986-4993

    • DOI

      10.1021/jp106830x

    • Peer Reviewed
  • [Presentation] Plasmonic Nanobubble Dynamics on Excitation of Aqueous Colloidal Gold Nanoparticles Observed by Picosecond Transient Spectroscopy2013

    • Author(s)
      Shuichi Hashimoto
    • Organizer
      Symposium on Plasmon-based Chemistry and Physics
    • Place of Presentation
      Leuven Catholic University (Leuven, Belgium)
    • Year and Date
      20130719-20
    • Invited
  • [Presentation] Interaction of lasers with gold nanopaticles : remarkable effects on the particles and the surrounding media2013

    • Author(s)
      Shuichi Hashimoto
    • Organizer
      International Symposium : Molecular Plasmonics 2013
    • Place of Presentation
      Institute of Photonic Technology, Jena, Germany
    • Year and Date
      20130523-25
    • Invited
  • [Presentation] Ensemble and single particle measurements of photothermal response of gold nanoparticles2013

    • Author(s)
      Shuichi Hashimoto
    • Organizer
      The 9th Korea-Japan Symposium on Frontier of Photoscience-2013
    • Place of Presentation
      Seoul National University (Seoul, Korea)
    • Year and Date
      2013-11-25
    • Invited
  • [Presentation] 単一金ナノ粒子を用いた光熱効果の研究(特別企画講演)2013

    • Author(s)
      橋本修一
    • Organizer
      日本化学会第93春季年会
    • Place of Presentation
      慶応大学日吉キャンパス(神奈川県)
    • Year and Date
      2013-03-22
  • [Presentation] Interactions of Lasers with Gold Nanoparticles Leading to the Phase Transformations of the Particles and the Surrounding Media2012

    • Author(s)
      Shuichi Hashimoto, Daniel Werner, Kenji Setoura
    • Organizer
      Japan-India Bilateral Seminar on Supramolecular Nanomaterials for Energy Innovation
    • Place of Presentation
      Alpha Anabuki Hall (Takamatsu, Japan)
    • Year and Date
      20121015-16
    • Invited
  • [Presentation] 金ナノ粒子とパルスレーザーの相互作用を利用したナノ加工(特別企画講演)2012

    • Author(s)
      橋本修一
    • Organizer
      日本化学会第92春季年会
    • Place of Presentation
      立命館大学びわこ・草津キャンパス(滋賀県)
    • Year and Date
      2012-03-28
  • [Remarks] 橋本研究室ウェブサイト

    • URL

      http://www.opt.tokushima-u.ac.jp/lab/a-4/index.html

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Published: 2015-06-25  

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