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2013 Fiscal Year Final Research Report

development of light harvesting structure using random medium

Research Project

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Project/Area Number 24651111
Research Category

Grant-in-Aid for Challenging Exploratory Research

Allocation TypeSingle-year Grants
Research Field Nanostructural science
Research InstitutionHokkaido University

Principal Investigator

FUJIWARA Hideki  北海道大学, 電子科学研究所, 准教授 (10374670)

Project Period (FY) 2012-04-01 – 2014-03-31
Keywords不規則構造 / 光局在 / ランダムレーザー
Research Abstract

Towards the development of a novel light-harvesting surface structure, I experimentally validate the controllability of random lasing modes on the basis of the resonant properties of surrounding scatterers and intentionally introduced defect nanoparticles. By adjusting the sizes of scatterers and defects, we experimentally clarified that the random lasing modes (lasing peak wavelength and the number of lasing peaks) at a defect region within a spherical ZnO nanoparticle film can be controlled. In addition, I also demonstrated a novel UV random lasing from a diamond nanoparticle film, in which nonlinear evolution of discrete sharp peaks at wavelengths around 380 nm, a wavelength never before observed, was observed. Because these results suggest the possibility of manipulating the optical characteristics even in random media, these results should provide important knowledge for the realization of highly efficient light harvesting structure.

  • Research Products

    (28 results)

All 2014 2013 2012 Other

All Journal Article (12 results) (of which Peer Reviewed: 10 results) Presentation (9 results) (of which Invited: 5 results) Remarks (6 results) Patent(Industrial Property Rights) (1 results) (of which Overseas: 1 results)

  • [Journal Article] Efficient optical coupling into a single plasmonic nanostructure using a fiber-coupled microspherical cavity2014

    • Author(s)
      H. Takashima, K. Kitajima, Y. Tanaka, H. Fujiwara, and K. Sasaki
    • Journal Title

      Phys. Rev. A

      Volume: 89 Pages: 021801

    • DOI

      10.1103/PhysRevA.89.021801

    • Peer Reviewed
  • [Journal Article] Fabrication of Spherical-Shaped Submicron Particles of ZnO Using Laser-induced Melting of Submicron-sized Source Materials2013

    • Author(s)
      T. Tsuji, Y. Higashi, M. Tsuji, H. Fujiwara, Y. Ishikawa, and N. Koshizaki
    • Journal Title

      Journal of Laser Micro/Nanoengineering

      Volume: 8 Pages: 292-295

    • DOI

      10.2961/jlmn.2013.03.0017

    • Peer Reviewed
  • [Journal Article] Two-photon excited fluorescence from a PIC-attached Au-coated tip via a thin tapered fiber under a weak CW excitation2013

    • Author(s)
      F. Ren, H. Takashima, Y. Tanaka, H. Fujiwara, and K. Sasaki
    • Journal Title

      Opt. Express

      Volume: 21 Pages: 27759-27769

    • DOI

      10.1364/OE.21.027759

    • Peer Reviewed
  • [Journal Article] Randomization of gold nano-brick arrays : a tool for SERS enhancement2013

    • Author(s)
      Y. Nishijima, J. B. Khurgin, L. Rosa, H. Fujiwara, and S. Juodkazis
    • Journal Title

      Opt. Express

      Volume: 21 Pages: 13502-13514

    • DOI

      10.1117/12.2003372

    • Peer Reviewed
  • [Journal Article] Low-threshold and quasi-single-mode random laser within a submicrometer-sized ZnO spherical particle film2013

    • Author(s)
      H. Fujiwara, R. Niyuki, Y. Ishikawa, N. Koshizaki, T. Tsuji, K. Sasaki
    • Journal Title

      Appl. Phys. Lett

      Volume: 102 Pages: 61110

    • DOI

      10.1063/1.4792349

    • Peer Reviewed
  • [Journal Article] Quasi-single-mode random lasing within a ZnO nanoparticle film2013

    • Author(s)
      H. Fujiwara, R. Niyuki, Y. Ishikawa, N. Koshizaki, T. Tsuji, K. Sasaki
    • Journal Title

      Proc. SPIE

      Volume: 8599 Pages: 859912

    • DOI

      10.1117/12.2003372

    • Peer Reviewed
  • [Journal Article] Analysis of Trap State Dynamics of Single CdSe/ZnS Quantum Dots on an Indium Tin Oxide Thin Film with Applying External Electric Field2013

    • Author(s)
      T. Chiba, J. Qi, H. Fujiwara, K. Sasaki
    • Journal Title

      J. Phys. Chem. C

      Volume: 117 Pages: 2507-2510

    • DOI

      10.1021/jp306408s

    • Peer Reviewed
  • [Journal Article] Fabrication of Spherical Particles Using Laser-induced Melting of Submicron-sized Materials2013

    • Author(s)
      T. Tsuji, Y. Higashi, M. Tsuji, H. Fujiwara, Koshizaki, and Y. Ishikawa
    • Journal Title

      Proceedings of The 14th International Symposium on Laser Precision Microfabrication

      Volume: 14 Pages: 205

  • [Journal Article] Fabrication of Spherical-Shaped Submicron Particles of ZnO Using Laser-induced Melting of Submicron-sized Source Materials2013

    • Author(s)
      Y. Higashi, T. Tsuji, M. Tsuji, H. Fujiwara, Koshizaki, and Y. Ishikawa
    • Journal Title

      Proceedings of The 10th Conference on Lasers and Electro-Optics Pacific Rim

      Volume: 10 Pages: WPE-12

  • [Journal Article] Nonlinear phenomena from a PIC attached gold tip using a plasmonic-whispering gallery mode hybrid system2013

    • Author(s)
      F. Ren, H. Takashima, Y. Tanaka, H. Fujiwara, and K. Sasaki
    • Journal Title

      Proc. SPIE

      Volume: 8816 Pages: 881612

    • DOI

      10.1117/12.2022626

    • Peer Reviewed
  • [Journal Article] Experimental evaluation of diffusion constant in a thin polymer film by triplet lifetime analysis of single molecules2012

    • Author(s)
      T. Chiba, H. Fujiwara, J. Hotta, S. Takeuchi, and K. Sasaki
    • Journal Title

      J. Photochem. & Photobiol. A

      Volume: 238 Pages: 24-28

    • DOI

      10.1016/j.jphotochem.2012.04.013

    • Peer Reviewed
  • [Journal Article] Second harmonic generation from the top of an Au-coated tip via a tapered fiber coupled microsphere resonator2012

    • Author(s)
      F. Ren, K. Kitajima, H. Takashima, H. Fujiwara, and K. Sasaki
    • Journal Title

      Proc. SPIE

      Volume: 8463 Pages: 846305

    • DOI

      10.1117/12.929437

    • Peer Reviewed
  • [Presentation] 酸化亜鉛サブミクロン球状粒子で光を操る~新奇ランダムレーザーの実現2013

    • Author(s)
      藤原英樹
    • Organizer
      東京工業大学応用セラミックス研究所共同利用研究ワークショップ(サブミクロン球状粒子の合成とその応用)
    • Place of Presentation
      東工大田町キャンパス,東京都港区
    • Year and Date
      2013-12-17
    • Invited
  • [Presentation] Manipulation of photon localized fields within a random medium : realization of low-threshold and quasi-single-mode random laser2013

    • Author(s)
      H. Fujiwara
    • Organizer
      The 14th RIES-Hokudai International Symposium"網[mou]"
    • Place of Presentation
      Chateraise Gateaux Kingdom Sapporo
    • Year and Date
      2013-12-11
    • Invited
  • [Presentation] Nonlinear phenomena from a PIC attached gold tip using a plasmonic-whispering gallery mode hybrid system2013

    • Author(s)
      F. Ren, H. Takashima, Y. Tanaka, H. Fujiwara, and K. Sasaki
    • Organizer
      SPIE Optics & Photonics
    • Place of Presentation
      San Diego
    • Year and Date
      2013-08-29
  • [Presentation] Fabrication of Spherical-Shaped Submicron Particles of ZnO Using Laser-induced Melting of Submicron-sized Source Materials2013

    • Author(s)
      T. Tsuji, Y. Higashi, M. Tsuji, H. Fujiwara, Y. Ishikawa, and N. Koshizaki
    • Organizer
      The 6th International Congress on Laser Advanced Materials Processing
    • Place of Presentation
      TOKI MESSE Niigata Convention Center, Niigata
    • Year and Date
      2013-07-25
  • [Presentation] Direct imaging of localized fields in a gold nanostructure using a scattering-type near-field microscope2013

    • Author(s)
      H. Fujiwara, Y. Tanaka, and K. Sasaki
    • Organizer
      The 10th Conference on Lasers and Electro-Optics Pacific Rim
    • Place of Presentation
      International Conference Center, Kyoto
    • Year and Date
      2013-07-04
  • [Presentation] Quasi-single mode random laser2013

    • Author(s)
      H. Fujiwara, R. Niyuki, T. Tsuji, Y. Ishikawa, N. Koshizaki, and K. Sasaki
    • Organizer
      Collaborative Conference on Materials Research
    • Place of Presentation
      Ramada Plaza Jeju Hotel, South Korea
    • Year and Date
      2013-06-27
    • Invited
  • [Presentation] ZnOナノ粒子薄膜からの疑似単一モードランダムレーザー発振2013

    • Author(s)
      藤原英樹
    • Organizer
      日本化学会第93春季年会
    • Place of Presentation
      立命館大学びわこ・くさつキャンパス,草津市
    • Year and Date
      2013-03-22
    • Invited
  • [Presentation] Second harmonic generation from the top of an Au-coated tip via a tapered fiber coupled microsphere resonator2012

    • Author(s)
      H. Fujiwara, R. Niyuki, Y. Ishikawa, N. Koshizaki, T. Tsuji, and K. Sasaki
    • Organizer
      SPIE Optics+Photonics
    • Place of Presentation
      San Diego convention center, USA
    • Year and Date
      2012-08-14
  • [Presentation] ランダムな構造で光を操る~ランダムレーザー発振の制御2012

    • Author(s)
      藤原英樹
    • Organizer
      第2回光科学異分野横断萌芽研究会
    • Place of Presentation
      岡崎コンファレンスセンター、岡崎市
    • Year and Date
      2012-08-07
    • Invited
  • [Remarks]

    • URL

      http://optsys.es.hokudai.ac.jp/~optsys/

  • [Remarks] 2013年9月「ランダムレーザで良好な発振を実現—球状のサブマイクロ粒子が成功のカギ」Laser Focus World Japan 2013.9(研究室探訪), 16-17、(2013)

  • [Remarks] 2013年2月14日「発振特性優れるランダムレーザー素子開発、ZnO粒子利用」化学工業日報

  • [Remarks] 2013年2月13日「酸化亜鉛のサブマイクロ粒子、ランダムレーザー素子に」日刊工業新聞

  • [Remarks] 2013年2月12日「酸化亜鉛粒子を用いた発振特性に優れたランダムレーザー素子を開発」産総研プレスリリース

    • URL

      http://www.aist.go.jp/aist_j/press_release/pr2013/pr20130212/pr20130212.html

  • [Remarks] 2013年2月12日「酸化亜鉛粒子を用いた発振特性に優れたランダムレーザー素子を開発」日経電子板プレスリリース

  • [Patent(Industrial Property Rights)] ランダムレーザー素子とその作製方法2012

    • Inventor(s)
      藤原英樹、笹木敬司、辻剛志、越崎 直人、石川善恵
    • Industrial Property Rights Holder
      藤原英樹、笹木敬司、辻剛志、越崎 直人、石川善恵
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      特願2012-183134
    • Filing Date
      2012-08-22
    • Overseas

URL: 

Published: 2015-06-25  

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