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EDUCATION OF ANALYTICAL METHOD FOR THE MIGRATION STUDY OF ENVIRONMENTAL PLUTONIUM

Research Project

Project/Area Number 11450198
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Civil and environmental engineering
Research InstitutionKYOTO UNIVERSITY

Principal Investigator

KUDO Akira  KYOTO UNIVERSITY, RESEARCH REACTOR INSTITUTE, PROFESSOR, 原子炉実験所, 教授 (00281113)

Co-Investigator(Kenkyū-buntansha) SASAKI Takayuki  KYOTO UNIVERSITY, RESEARCH REACTOR INSTITUTE, RESEACH ASSOCIATE, 原子炉実験所, 助手 (60314291)
MATSUI Saburo  KYOTO UNIVERSITY, FACULTY OF ENGINEERING, PROFESSOR, 工学研究科, 教授 (90092808)
SUGAWARA Masataka  OSAKA SANGYO UNIVERSITY, PROFESSOR, 工学部, 教授 (60026119)
KUBOTA Takumi  KYOTO UNIVERSITY, RESEARCH REACTOR INSTITUTE, RESEACH ASSOCIATE, 原子炉実験所, 助手 (90335240)
寺島 泰  京都大学, 工学研究科, 教授 (50019717)
松田 知成  京都大学, 工学研究科, 助手 (50273488)
藤川 陽子  京都大学, 原子炉実験所, 助教授 (90178145)
Project Period (FY) 1999 – 2001
Project Status Completed (Fiscal Year 2001)
Budget Amount *help
¥14,700,000 (Direct Cost: ¥14,700,000)
Fiscal Year 2001: ¥4,200,000 (Direct Cost: ¥4,200,000)
Fiscal Year 2000: ¥4,600,000 (Direct Cost: ¥4,600,000)
Fiscal Year 1999: ¥5,900,000 (Direct Cost: ¥5,900,000)
KeywordsPLUTONIUM / ENVIRONMENT / ANALYSIS / EDUCATION / PLUTHERMAL / TRAINING / 環境試料 / 前処理 / アルファ線スペクトロメトリー / 電着法 / 分離精製
Research Abstract

An artificial single dose contaminant was released at Nagasaki, Japan on August 9,1945 detonating Plutonium (10-15kg) atomic bomb. A portion, 1.2 kg of 239Pu was fissioned releasing 21 kt TNT energy along with various fission products. The rest of the unexpended fissile material, 239+240Pu, 13.8 kg (3.49 x 10^<13> Bq), was dispersed into the atmosphere along with a fission product, 137Cs, 23.4 g (7.44 x 10^<13>Bq). The fate of 239+240Pu and 137Cs was investigated by analysing both local and global fallout. The highest concentration of 239+240Pu was 64.5 mBq/g (181 mBq/cm2) while it was 188 mBq/g (526 mBq/cm2) for 137Cs both at 2.8 km east from the hypocentre. The total amount of deposition in the local fallout region of 264 km2 was 37.5 g (9.48 x 10^<10>Bq) for 239+240Pu and 3.14 mg (5.88 x 10^<10>Bq) for 137Cs. The ratio of the local fallout against the total amount of the radionuclides released was 0.27% for 239+240Pu and 0.134% for 137Cs. Recent advancements in analytical technology made it possible for artificial radionuclides released from the Nagasaki explosion to be detected in the Arctic ice core layer of 1945. The 239+240Pu and the 137Cs, were measured by collecting 10 ice cores on the Agassiz ice cap, Ellesmere Island, Canada. The deposition was 0.16 μBq/cm2 for 239+240Pu and 20 μBq/cm2 for 137Cs. During the atmospheric testing, the deposition of 239+240Pu and 137Cs varied more than 100 times with the highest peaks of over 50 μBq/cm2 for 239+240Pu and over 800 μBq/cm2 for 137Cs both occurred in 1962. Analyzing Arctic data, there are many new information for long global transport, the history of nuclear weapons development etc.

Report

(4 results)
  • 2001 Annual Research Report   Final Research Report Summary
  • 2000 Annual Research Report
  • 1999 Annual Research Report
  • Research Products

    (25 results)

All Other

All Publications (25 results)

  • [Publications] A.Kudo, T.Kubota, J.Zheng, T.Sasaki, et al.: "Measurement of Nagasaki Pu Global Transport Rates, Comparing with SO_2 from Historic Volcanic Eruptions"Journal of Nuclear Science and Technology. (印刷中). (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] T.Sasaki, T.Kubota, S.Mito, T.Kauri, A.Kudo: "Radionuclides Sorption to a Mixture of Anaerobic Bacteria in the Repository environment"Journal of Nuclear Science and Technology. (印刷中). (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] T.Sasaki, A.Kudo: "Pu Sorption to Activated Conglomerate Anaerobic Bacteria"Chemistry Letters. 196-197 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] A.Kudo, Y.Mahara, et al.: "Global Transport of Plutonium from Nagasaki to the Arctic-Review of Nagasaki Pu Investigation and Future"PLUTONIUMU IN THE ENVIRONMENT, Proc. of 2nd Interna. Symposium. Vol.1. 233-250 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] A.Kudo, et al.: "Behaviour of Plutonium at the Surface and in Geologic environment"J. OF RADIOCHEMICA ACTA. 82. 159-166 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] A.Kudo: "Radioactivity in the Environment, Volume 1., "Plutonium in the Enviroment""Elsevier Science. 447 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] KUDO A., ZHENG J., KOERNER R.M, FISHER D.A., SANTRY, D.C., MAHARA, Y: "GLOBAL TRANSPORT RATES OF 137CS AND 239+240PU ORIGINATING FROM NAGASAKI A-BOMB IN 1945 AS DETERMINED FROM ANALYSIS OF CANADIAN ARCTICICE CORES"J. OF ENVIRONMENTAL RADIOACTIVITY. 40. 289-298 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] KUDO, A.: "BEHAVIOUR OF PLUTONIUM AT THE SURFACE AND IN GEOLOGIC ENVORNMENT"J. OF RADIOCHEMICA ACTA. 82. 159-166 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] MAHARA. A, KUDO A.: "PROBABILITY OF PRODUCTION OF MOBILE PLUTONIUM IN ENVIRONMENTS OF SOIL AND SEDIMENT"J. OF RADIOCHEMICA ACTA. 82. 339-404 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] A. KUDO, J. ZHENG, R. YAMADA, G. TAO. T: "GLOBAL TRANSPORT RATES AND FUTURE PREDICTION OF HAZARDOUS MATERIALS : PU AND CS-FROM NAGASAKI TO CANADEAN ARCTIC"WaT.SCI. TECH. 42. 163-169 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] T. SASAKI, A. KUDO: "PU SORPTION TO ACTIVATED CONGLOMERATE ANAEROBIC BACTERIA"CHEM.LETT. 196-197 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] A. KUDO, T. KUBOTA, J. ZHENG, T. SASAKI, T. KAURI, S. MIYAHARA: "MEASUREMENT OF NAGASAKI PU GLOBAL TRANSPORT RATES, COMPARING WITH SO2 FROM HISTORIC VOLCANIC ERUPTIONS"J. OF NUCLEAR SCIENCE AND TECHNOLOGY. (in press). (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] T. KUBOTA, T. SASAKI, O. TOCHIYAMA, A. KUDO: "INTERACTION OFNEPTUNIUM WITH HUMIC ACID AND ANAEROVIC BACTERIA"J. OF NUCLEAR SCIENCE AND TECHNOLOGY. (in press). (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] A. KUDO(EDITOR): "RADIOACTIVITY IN THE ENVIRONMENT, VOLUME1.,"PLUTONIUM IN THE ENVIRONMENT", BOOK"ELSEVIER SCIENCE, UK. 447. (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] A.Kudo, T.Kubota, J.Zheng, T.Sasaki, et al.: "Measurement of Nagasaki Pu Global Transport Rates, Comparing with SO_2 from Historic Volcanic Eruptions"Journal of Nuclear Science and Technology. (印刷中). (2002)

    • Related Report
      2001 Annual Research Report
  • [Publications] T.Sasaki, T.Kubota, S.Mito, T.Kauri, A.Kudo: "Radionuclides Sorption to a Mixture of Anaerobic Bacteria in the Repository Environment"Journal of Nuclear Science and Technology. (印刷中). (2002)

    • Related Report
      2001 Annual Research Report
  • [Publications] T.Sasaki, A.Kudo: "Pu Sorption to Activated Conglomerate Anaerobic Bacteria"Chemistry Letters. 196-197 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] A.Kudo: "Radioactivity in the Environment, Volume 1., "Plutonium in the Environment""Elsevier Science. 447 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] A.Kudo,Y.Mahara, et al.: "Global Transport of Plutonium from Nagasaki to the Arctic-Review of Nagasaki Pu Investigation and Future"PLUTONIUM IN THE ENVIRONMENT, Proc. of 2nd Interna. Symposium. vol.1. 233-250 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] T.Sasaki,J.Zheng,H.Asano and A.Kudo: "Interaction of Pu, Np and Pa with Anaerobic Microorganisms at Geologic Repositories"PLUTONIUM IN THE ENVIRONMENT, Proc. of 2nd Interna. Symposium. vol.1. 221-232 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] Y.Mahara and A.Kudo: "Plutonium Mobility and Its Fate in Soil and Sediment Environments"PLUTONIUM IN THE ENVIRONMENT, Proc. of 2nd Interna. Symposium. vol.1. 347-362 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] A.Kudo: "PLUTONIUM IN THE ENVIRONMENT"Elsevier(未定) . (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] Kudo A.et al.: "Global Transport Rates and Future Prediction of Hazardrous Materials: Pu and Cs-from Nagasaki to Canadian Arctic"Int. Water Association, Ecohazard 99. 1. 229-236 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] Kudo A.: "A Lesson from the First Japanese Fission Accident Caused by an Accidental Critical Mass Creation"J of Environmental Conservation and Technology. 28. 711-718 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] Fujikawa Y.,Sugahara M.and Kudo A.: ""Strong association of fallout plutonium with humic and fulvic acid as compared to uranium and ^<137>Cs in Nishiyama soils from Nagasaki, Japan""Water, Air and Soil Pollution. 240. 69-74 (1999)

    • Related Report
      1999 Annual Research Report

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Published: 1999-04-01   Modified: 2016-04-21  

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