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Study of pressure induced valence transition and orbital effect on Ce compounds under high field

Research Project

Project/Area Number 15K05146
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Condensed matter physics II
Research InstitutionShimane University

Principal Investigator

Fujiwara Kenji  島根大学, 総合理工学研究科, 教授 (50238630)

Project Period (FY) 2015-10-21 – 2018-03-31
Project Status Completed (Fiscal Year 2017)
Budget Amount *help
¥4,550,000 (Direct Cost: ¥3,500,000、Indirect Cost: ¥1,050,000)
Fiscal Year 2017: ¥650,000 (Direct Cost: ¥500,000、Indirect Cost: ¥150,000)
Fiscal Year 2016: ¥780,000 (Direct Cost: ¥600,000、Indirect Cost: ¥180,000)
Fiscal Year 2015: ¥3,120,000 (Direct Cost: ¥2,400,000、Indirect Cost: ¥720,000)
Keywords超伝導 / 重い電子系 / 圧力効果 / 強磁場 / 核磁気共鳴 / 高圧 / NMR / 価数揺らぎ / 磁場誘起転移 / 強磁場誘起価数転移
Outline of Final Research Achievements

Cu-NMR of heavy fermion superconductor CeCu2Si2 was performed under high pressure (5.4, 6.2 and 7.0 GPa) and high field (5~22 T). Ce valence and spin state were investigated by electric field gradient (EFG) at Cu sites, and by Knight Shift (K) and nuclear spin lattice relaxation time (T1), respectively. Above 5 GPa, EFG, K and 1/T1 decrease below identical temperature (T*). These behavior suggest that new crossover with valence change occurs below T*. T* monotonically increases with applying pressure (ex. T*=20, 40, 55K at 5.4, 6.2 and 7.0 GPa). Furthermore, T* is independent of magnetic field between 7 and 22 T. Therefore, the crossover at T* field induced valence transition does not result from field induced valence transition predicted by valence fluctuation model.

Report

(4 results)
  • 2017 Annual Research Report   Final Research Report ( PDF )
  • 2016 Research-status Report
  • 2015 Research-status Report
  • Research Products

    (16 results)

All 2018 2017 2016 2015 Other

All Int'l Joint Research (3 results) Journal Article (1 results) (of which Peer Reviewed: 1 results) Presentation (12 results) (of which Int'l Joint Research: 2 results)

  • [Int'l Joint Research] Max Planck Institute(ドイツ)

    • Related Report
      2017 Annual Research Report
  • [Int'l Joint Research] Max Planck Institute(Germany)

    • Related Report
      2016 Research-status Report
  • [Int'l Joint Research] Max Planck Institutes(Germany)

    • Related Report
      2015 Research-status Report
  • [Journal Article] Point-Contact Spectroscopy of Heavy Fermion Compounds CeCu6 and CeAl3 in Mangetic Field2015

    • Author(s)
      G. Motoyama, S. Ogawa, K. Matsubayashi, K. Fujiwara, K. MIyoshi, S. Nishigori, T. Mutou, A. Yamaguchi, A. Sumiyama, Y. Uwatoko
    • Journal Title

      Physics Procedia

      Volume: 75 Pages: 296-302

    • DOI

      10.1016/j.phpro.2015.12.035

    • Related Report
      2015 Research-status Report
    • Peer Reviewed
  • [Presentation] NMR Study of CeCu2Si2 under High Field and Pressure2018

    • Author(s)
      Kenji Fujiwara, Tatsuo C. Kobayashi, Kentaro Kitagawa, Michihiro Hirata, Takahiko Sasaki, Hisashi Kotegawa, Hideki Tou, Takayuki Goto, Silvia Seiro, Christoph Geibel, Frank Steglich
    • Organizer
      J-Physics Annual Meeting FY2017
    • Related Report
      2017 Annual Research Report
  • [Presentation] NMR study of CeCu2Si2 under high field and pressure2017

    • Author(s)
      Kenji FUJIWARA, Yuuya TAKAMATSU, Yuuki SUWADA, Tatsuo C. KOBAYASHI, Takahiko SASAKI, Takayuki GOTO, Silvia SEIRO, Christoph GEIBEL, Frank STEGLICH
    • Organizer
      Conference on Strongly Correlated Electron Systems
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] CeCu2Si2の高圧・強磁場領域のCu-NMR2017

    • Author(s)
      藤原賢二, 高松祐弥, 本山岳, 三好清貴, 小林達生, 北川健太郎, 佐々木孝彦, 後藤貴行, 小手川恒, 藤秀樹, S. Seiro, C. Geibel, F. Steglich
    • Organizer
      日本物理学会 2017年秋季大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 高圧・強磁場下におけるCe化合物のNM2017

    • Author(s)
      大谷篤, 藤原賢二, 本山岳, 三好清貴, 西郡至誠
    • Organizer
      日本物理学会 2017年秋季大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 新奇重い電子系化合物Ce3TiBi5の圧力下電気抵抗測定2017

    • Author(s)
      本山岳, 瀬崎真澄, 郷地順, 三好清貴, 西郡至誠, 武藤哲也, 藤原賢二, 上床美也
    • Organizer
      日本物理学会 第72回年次大会
    • Place of Presentation
      大阪大学
    • Related Report
      2016 Research-status Report
  • [Presentation] CeCu2Si2の強磁場・高圧下における価数状態の研究-III2017

    • Author(s)
      高松祐弥, 藤原賢二, 須和田裕貴, 本山岳, 三好清貴, 小林達生, 北川健太郎, 佐々木孝彦, 後藤貴行, S. Seiro, C. Geibel, F. Steglich
    • Organizer
      日本物理学会 第72回年次大会
    • Place of Presentation
      大阪大学
    • Related Report
      2016 Research-status Report
  • [Presentation] CeCu2Si2の強磁場・高圧下における価数状態の研究2016

    • Author(s)
      藤原賢二,須和田裕貴,本山岳,三好清貴,小林達生,北川健太郎,佐々木孝彦,後藤貴行,S. Seiro,C. Geibel,F. Steglich
    • Organizer
      日本物理学会第71回年次大会
    • Place of Presentation
      東北学院大学
    • Year and Date
      2016-03-19
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] LaFeAsO1-xFx(x=0.03~0.04)のパルス通電焼結試料を用いた圧力下物性測定2016

    • Author(s)
      大塚啓右, 三好清貴, 本山岳, 藤原賢二, 西郡至誠, 北川裕之
    • Organizer
      日本物理学会 2016年秋季大会
    • Place of Presentation
      金沢大学
    • Related Report
      2016 Research-status Report
  • [Presentation] FeSe純良単結晶の圧力下直流磁化測定2016

    • Author(s)
      加藤駿一, 三好清貴, 本山岳, 藤原賢二
    • Organizer
      日本物理学会 2016年秋季大会
    • Place of Presentation
      金沢大学
    • Related Report
      2016 Research-status Report
  • [Presentation] CeCu2Si2の強磁場・高圧下における価数状態の研究-II2016

    • Author(s)
      高松祐弥, 藤原賢二, 須和田裕貴, 本山岳, 三好清貴, 小林達生, 北川健太郎, 佐々木孝彦, 後藤貴行, S. Seiro, C. Geibel, F. Steglich
    • Organizer
      日本物理学会 2016年秋季大会
    • Place of Presentation
      金沢大学
    • Related Report
      2016 Research-status Report
  • [Presentation] 重い電子系化合物CeAl2の高圧下Al-NMR2016

    • Author(s)
      藤原賢二, 小山健太, 梅澤拓也, 本山岳, 三好清貴
    • Organizer
      日本物理学会 2016年秋季大会
    • Place of Presentation
      金沢大学
    • Related Report
      2016 Research-status Report
  • [Presentation] ビスマス系重い電子系化合物の探索2016

    • Author(s)
      瀬崎眞澄, 本山岳, 藤原賢二, 三好清貴, 西郡至誠, 郷地順, 上床美也
    • Organizer
      日本物理学会 2016年秋季大会
    • Place of Presentation
      金沢大学
    • Related Report
      2016 Research-status Report

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Published: 2015-10-21   Modified: 2020-05-15  

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