Field-effect transistors with organic-inorganic perovskite semiconductors
Project/Area Number |
16H04192
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Research Category |
Grant-in-Aid for Scientific Research (B)
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Allocation Type | Single-year Grants |
Section | 一般 |
Research Field |
Organic and hybrid materials
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Research Institution | Kyushu University |
Principal Investigator |
Matsushima Toshinori 九州大学, カーボンニュートラル・エネルギー国際研究所, 准教授 (40521985)
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Research Collaborator |
Fujiwara Takashi
Qin Chuanjiang
Sandanayaka Atula Sangarange Don
Goshi Kenichi
Adachi Chihaya
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Project Period (FY) |
2016-04-01 – 2019-03-31
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Project Status |
Completed (Fiscal Year 2018)
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Budget Amount *help |
¥17,290,000 (Direct Cost: ¥13,300,000、Indirect Cost: ¥3,990,000)
Fiscal Year 2018: ¥2,210,000 (Direct Cost: ¥1,700,000、Indirect Cost: ¥510,000)
Fiscal Year 2017: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
Fiscal Year 2016: ¥13,130,000 (Direct Cost: ¥10,100,000、Indirect Cost: ¥3,030,000)
|
Keywords | 金属ハライドペロブスカイト / 電界効果トランジスタ / キャリア移動度 / 大気安定性 / 単結晶 / 有機無機ペロブスカイト / 半導体 / バイアス安定性 / 電界効果移動度 / アンビポーラ駆動 / トランジスタ / 酸素 / ホール移動度 / 安定性 / 電子移動度 / ヒステリシス / 劣化 / 次元性制御 / 高キャリア移動度 |
Outline of Final Research Achievements |
We could increase hole mobilities to 12 cm2/Vs by optimizing perovskite transistor architectures. We also demonstrated n-channel operation of perovskite transistors, with electron mobilities of 1.5 cm2/Vs. By reducing the influence of contact resistance between source/drain electrodes and perovskite, we successfully obtained hole mobilities of up to 26 cm2/Vs and electron mobilities of up to 4.6 cm2/Vs. We analyzed degradation mechanisms of perovskite transistors in air. By removing the air-induced degradation sources from films, we developed air-stable perovskite transistors although tin-based perovskites are typically unstable in air. We grew large perovskite single crystals and laminated them on substrates. These laminated single crystal transistors had very high hole mobilities of at least 50 cm2/Vs and electron mobilities of about 36 cm2/Vs because of lower grain boundary density and smaller structure disorder in single crystals.
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Academic Significance and Societal Importance of the Research Achievements |
ペロブスカイトトランジスタはスピンコート法などの簡単なプロセスで作製できる。無機骨格を介してキャリアが流れるために高速動作も期待される。しかし、ペロブスカイトの基礎的な動作原理、デバイス特性を低下させる要因、劣化機構などについては分かっていないことが多かった。これらに関する学理を解明し、その結果をフィードバックすることから極めて高性能なペロブスカイトトランジスタを作製できるようになった。本研究成果を用いれば、アンビポーラトランジスタや発光トランジスタなどの次世代デバイスの研究へと展開できる。また、センサー、駆動回路、発光デバイスなどへの応用が期待され、関連産業分野に大きなインパクトがある。
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Report
(4 results)
Research Products
(210 results)
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[Presentation] Efficient and stable hybrid perovskite solar cells2019
Author(s)
Toshinori Matsushima, Chuanjiang Qin, Shinobu Terakawa, Takashi Fujihara, and Chihaya Adachi
Organizer
2019 I2CNER ANNUAL SYMPOSIUM: ENERGY TRANSITIONS AND THE ROLE OF CCS TOWARD A CARBON‐NEUTRAL ENERGY SOCIETY, Kyushu University, Fukuoka, Japan, January 1, 2019
Related Report
Int'l Joint Research
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[Presentation] Organic semiconductor distributed feedback (DFB) laser2019
Author(s)
SANGARANGE DONATULA SANDANAYAKA, Toshinori Matsushima, Fatima Bencheikh, Shinobu Terakawa, William Potscavage, Chuanjiang Qin, Takashi Fujihara, Kenichi Goushi, Jean-Charles Ribierrea, Chihaya Adachi
Organizer
The 66th JSAP Spring Meeting, 2019, Tokyo Institute of Technology, Tokyo, Japan, March 9-12, 2019
Related Report
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[Presentation] p-i-n 逆構造MAPbI3ペロブスカイト太陽電池におけるPEDOT:PSS のエネルギーシフト抑制による開放端電圧の向上2019
Author(s)
藤原隆,菅原峻, 前田真一, 下位祐子, 王胖胖, 小林慎一郎, シンセンコウ, 松島敏則, 伊左治忠之, 河西容督, 八尋正幸, 安達千波矢
Organizer
2019年第66回応用物理学会春季学術講演会, 東京工業大学,2019年3月9-12日
Related Report
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[Presentation] チエノキノイド半導体薄膜におけるラビング温度制御による分子配向度の増大2019
Author(s)
青山 哲也, 田中 利彦, Benoit Heinrich, Fabrice Mathevet, 松島 敏則, 高石 和人, 松本 真哉, 内山 真伸, 安達 千波矢, Jean-Charles Ribierre
Organizer
2019年第66回応用物理学会春季学術講演会, 東京工業大学,2019年3月9-12日
Related Report
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[Presentation] Efficient and stable perovskite-based optoelectronic devices2018
Author(s)
Toshinori Matsushima, Chuanjiang Qin, Takashi Fujihara, and Chihaya Adachi
Organizer
THE 25th INTERNATIONAL WORKSHOP ON ACTIVE-MATRIX FLATPANEL DISPLAYS AND DEVICES (AM-FPD18) -TFT Technologies and FPD Materials- Ryukoku University Avanti Kyoto Hall, Kyoto, Japan, July 3-6, 2018
Related Report
Int'l Joint Research / Invited
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[Presentation] Efficient and stable laser oscillation from organic semiconductor films2018
Author(s)
T. Matsushima, A. S. D. Sandanayaka, F. Bencheikh, K. Yoshida, M. Inoue, T. Fujihara, K. Goushi, J.-C. Ribierre, C. Adachi
Organizer
10th International Symposium on Organic Molecular Electronics (ISOME 2018), Sunmesse Tosu, Tosu, Saga, Japan, May 31-June 2, 2018
Related Report
Int'l Joint Research / Invited
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[Presentation] Mechanical rubbing-induced edge-on to face-on reorientation and molecular alignment in thienoquinoid transistors2018
Author(s)
Tetsuya Aoyama, Toshihiko Tanaka, Benoit Heinrich, Fabrice Mathevet, Toshinori Matsushima, Kazuto Takaishi, Shinya Matsumoto, Masanobu Uchiyama, Chihaya Adachi, Jean-Charles Ribierre
Organizer
9th International Conference On Molecular Electronics (ElecMol9), Paris, France, December 17-20, 2018
Related Report
Int'l Joint Research
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[Presentation] Enhanced Electroluminescence from Organic Light-Emitting Diodes with an Organic-Inorganic Perovskite Host Layer2018
Author(s)
Toshinori Matsushima, Chuanjiang Qin, Kenichi Goushi, Fatima Bencheikh, Takeshi Komino, Matthew Leyden, Atula S. D. Sandanayaka, and Chihaya Adachi
Organizer
EL2018, Meiji University, Tokyo, Japan, September 11-13, 2018
Related Report
Int'l Joint Research
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[Presentation] ラビングによるチエノキノイド分子のEdge-on/Face-on 変換と有機トランジスタ移動度の異方性2018
Author(s)
青山 哲也, 田中 利彦, Benoit Heinrich, Fabrice Mathevet, 松島 敏則, 高石 和人, 松本 真哉, 内山 真伸, 安達 千波矢, Jean-Charles Ribierre
Organizer
2018年第79回応用物理学会秋季学術講演会, 名古屋国際会議場,2018年9月18日-21日
Related Report
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[Presentation] ブロモヘキサセンの合成と薄膜状態での物性評価2018
Author(s)
渡邊源規, 宮崎隆聡, 松島敏則, 松田潤子, 簡敬庭, 芝原雅彦, 安達千波矢, 孫世勝, 周大新 ,石原達己
Organizer
第29回基礎有機化学討論会, 東京工業大学大岡山キャンパス, 2018年9月6-8日
Related Report
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[Presentation] 有機無機ペロブスカイトをホスト材料として用いた有機EL2018
Author(s)
松島敏則, Fatima Bencheikh, Matthew Leyden, Atula S. D. Sandanayaka, Chuanjiang Qin, 合志憲一, 安達千波矢
Organizer
「有機EL討論会」第26回例会, 日本科学未来館, 東京, 日本, 2018年6月21-22日
Related Report
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[Presentation] CW lasing from organic thin-film DFB structure and outlook for electrical lasing, Frontiers of Organic Semiconductor Laser 20182018
Author(s)
A. S. D. Sandanayaka, Toshinori Matsushima, Fatima Bencheikh, Takashi Fujihara, Kenichi Goushi, Jean-Charles Ribierre, Masayuki Mamada, Takuji Hatakeyama, Hajime Nakanotani, and Chihaya Adachi
Organizer
South China University of Technology
Related Report
Int'l Joint Research / Invited
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[Presentation] New materials for fabrication of efficient near infrared OLEDs and organic solid-state lasers2017
Author(s)
Anthony D'Aleo, Dae Hyeon Kim, Atula S. D. Sandanayaka, Dandan Yao, Elena Zaborova, Gabriel Canard, Toshinori Matsushima, Youichi Tsuchiya, Eunyoung Choi, Jeong Weon Wu, Frederic Fages, Jean-Charles Ribierre, Chihaya Adachi
Organizer
SPIE Optics + Photonics 2017
Related Report
Int'l Joint Research / Invited
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[Presentation] Continuous-wave operation of organic semiconductor lasers2017
Author(s)
Atula S. D. Sandanayaka, Toshinori Matsushima, Fatima Bencheikh, Kou Yoshida, Munetomo Inoue, Chuanjiang Qin, Takashi Fujihara, Kenichi Goushi, Jean-Charles Ribierre, Chihaya Adachi
Organizer
International Symposium on Organic and Polymeric Optoelectronics (ISOPO 2017)
Related Report
Int'l Joint Research / Invited
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[Presentation] New Materials for fabrication of Efficienct Near Infrared OLEDs and Organic Solid-state Lasers2017
Author(s)
Anthony D’ Aleo, Dae-Hyeon Kim, Atula S. D. Samdanayaka, Ko Inada, Dandan Yao, Elena Zaborova, Gabriel Canard, Li Zhao, Toshinori Matsushima, Youichi Tsuchiya, Eunyoung Choi, Jeong Weon Wu, FredericFages, Jean-Charles Ribierre, Chihaya Adachi
Organizer
NanoMat2017
Related Report
Int'l Joint Research
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[Presentation] 有機薄膜からのCWレーザー発振2017
Author(s)
A. S. D. Sandanayaka, 松島敏則, F. Bencheikh, 吉田 巧, 井上棟智, 藤原隆, 合志憲一, J.-C. Ribierre, 安達千波矢
Organizer
第64回応用物理学会春季学術講演会
Related Report
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[Presentation] Organic-inorganic perovskite field-effect transistors2016
Author(s)
Toshinori Matsushima, Sunbin Hwang, Atula S. D. Sandanayaka, Chuanjiang Qin, Shinobu Terakawa, Takashi Fujihara, Masayuki Yahiro, and Chihaya Adachi
Organizer
The 23rd International Display Workshops in conjunction with Asia Display 2016
Place of Presentation
Fukuoka, Japan
Year and Date
2016-12-07
Related Report
Int'l Joint Research / Invited
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[Presentation] Organic-inorganic perovskite field-effect transistors2016
Author(s)
Toshinori Matsushima, Sunbin Hwang, Atula S. D. Sandanayaka, Chuanjiang Qin, Shinobu Terakawa, Takashi Fujihara, Masayuki Yahiro, and Chihaya Adachi
Organizer
The 8th Asian Conference on Organic Electronics 2016 (A-COE 2016)
Place of Presentation
Kyoto, Japan
Year and Date
2016-12-05
Related Report
Int'l Joint Research
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[Presentation] Low-threshold Quasi-continuous-wave Organic Semiconductor Laser2016
Author(s)
Atula S. D. Sandanayaka, Toshinori Matsushima, Kou Yoshida, Takashi Fujihara, Kenichi Goushi, Jean-Charles Ribierre, and Chihaya Adachi
Organizer
KJF International Conference on Organic Materials for Electronics and Photonics 2016 (KJF-ICOMEP 2016)
Place of Presentation
Fukuoka, Japan
Year and Date
2016-09-04
Related Report
Int'l Joint Research
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[Presentation] Very High Carrier Mobilities in Organic-inorganic Perovskite Films2016
Author(s)
Toshinori Matsushima, Sunbin Hwang, Atula S. D. Sandanayaka, Chuanjiang Qin, Shinobu Terakawa, Takashi Fujihara, Masayuki Yahiro, and Chihaya Adachi
Organizer
KJF International Conference on Organic Materials for Electronics and Photonics 2016 (KJF-ICOMEP 2016)
Place of Presentation
Fukuoka, Japan
Year and Date
2016-09-04
Related Report
Int'l Joint Research
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[Presentation] Quasi-continuous-wave organic semiconductor lasers using oxygen as triplet scavenger2016
Author(s)
Jean-Charles Ribierre, Atula S.D. Sandanayaka, Li Zhao, Delphine Pitrat, Jean-Christophe Mulatier, Toshinori Matsushima, Chantal Andraud, Ju-Hyung Kim, and Chihaya Adachi
Organizer
SPIE Optics + Photonics 2016
Place of Presentation
San Diego Convention Center, San Diego, California, United States
Year and Date
2016-08-28
Related Report
Int'l Joint Research / Invited
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[Presentation] Quasi Continuous-Wave Lasing in Organic Thin-Film Semiconductors2016
Author(s)
Atula S.D. Sandanayaka, Kou Yoshida, Munetomo Inoue, Chuanjiang Qin, Kenichi Goushi, Jean-Charles Ribierre, Toshinori Matsushima, and Chihaya Adachi
Organizer
SPIE Optics + Photonics
Place of Presentation
San Diego Convention Center, San Diego, California, United States
Year and Date
2016-08-28
Related Report
Int'l Joint Research / Invited
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[Presentation] Morphological control of organic-inorganic perovskite layers by hot isostatic pressing for efficient planar solar cells2016
Author(s)
T. Matsushima, T. Fujihara, C. Qin, S. Terakawa, Y. Esaki, S. Hwang, A. S. D. Sandanayaka, W. J. Potscavage, Jr., and C. Adachi
Organizer
The International Conference on Science and Technology of Synthetic Metals in 2016 (ICSM2016)
Place of Presentation
Guangzhou, China
Year and Date
2016-06-26
Related Report
Int'l Joint Research
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[Presentation] Flat perovskite films for efficient solar cells2016
Author(s)
T. Matsushima, T. Fujihara, C. Qin, S. Terakawa, Y. Esaki, S. Hwang, A. S. D. Sandanayaka, W. J. Potscavage, Jr., and C. Adachi
Organizer
XXth International Krutyn Summer School 2016
Place of Presentation
Krutyn, Masurian Lake District, Poland
Year and Date
2016-06-12
Related Report
Int'l Joint Research
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[Book] 有機ソフトマテリアルレーザーの最新動向2018
Author(s)
Atula S. D. Sandanayaka、松島敏則、Fatima Bencheikh、吉田功、井上棟智、藤原隆、合志憲一、Jean-Charles Ribierre、安達千波矢
Total Pages
4
Publisher
レーザー学会誌、レーザー研究、Volume 46, Number 1, Page 6-9, January 2018
Related Report
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[Book] Efficient and Stable Lasing from Organic Semiconductor Films2018
Author(s)
T. Matsushima, A. S. D. Sandanayaka, F. Bencheikh, K. Yoshida, M. Inoue, T. Fujihara, K. Goushi, J.-C. Ribierre, C. Adachi
Total Pages
6
Publisher
The Papers of Joint Technical Meeting on “Dielectrics and Electrical Insulation” and “Electronic Materials”, IEE Japan, DEI-18-016, EFM-18-016, 43-48, 2018
Related Report
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[Book] Efficient and Stable Lasing from Organic Semiconductor Films2018
Author(s)
T. Matsushima, A. S. D. Sandanayaka, F. Bencheikh, K. Yoshida, M. Inoue, T. Fujihara, K. Goushi, J.-C. Ribierre, C. Adachi
Total Pages
6
Publisher
The Papers of Joint Technical Meeting on “Dielectrics and Electrical Insulation” and “Electronic Materials”, IEE Japan
Related Report
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