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Inteligent treatment and disposal of soils contaminated cesium from accident of nuclear power plant at Fukushima

Research Project

Project/Area Number 24360369
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypePartial Multi-year Fund
Section一般
Research Field Earth system and resources enginnering
Research InstitutionHokkaido University

Principal Investigator

SATO Tsutomu  北海道大学, 工学(系)研究科(研究院), 教授 (10313636)

Co-Investigator(Kenkyū-buntansha) KOGURE Toshihiro  東京大学, 理学研究科, 准教授 (50282728)
NAWA Toyoharu  北海道大学, 大学院工学研究院, 教授 (30292056)
Project Period (FY) 2012-04-01 – 2015-03-31
Project Status Completed (Fiscal Year 2014)
Budget Amount *help
¥18,460,000 (Direct Cost: ¥14,200,000、Indirect Cost: ¥4,260,000)
Fiscal Year 2014: ¥4,420,000 (Direct Cost: ¥3,400,000、Indirect Cost: ¥1,020,000)
Fiscal Year 2013: ¥4,420,000 (Direct Cost: ¥3,400,000、Indirect Cost: ¥1,020,000)
Fiscal Year 2012: ¥9,620,000 (Direct Cost: ¥7,400,000、Indirect Cost: ¥2,220,000)
Keywords地質汚染修復 / セシウム / 土壌汚染 / 環境修復 / 福島 / 粘土鉱物
Outline of Final Research Achievements

In this study, we conducted extraction and identification of particles fixed radioactive cesium from the soils at Fukushima to make proposal of applicable separation method for reduction in volume, and leaching experiments to make proposal safety solidification of cesium adsorbed zeolites. As the results of this study, the particles are categorized in the following three types, 1) coagulation of several mineral particles, 2) mineral-organic matter complex, and 3) weathered mica, and separated from non-contaminated particles by wet screening and using diatomite. These particles will be directly disposed after volume reduction of the contaminated soils because cesium already fixed into structure of the minerals in the particles. However, cesium released from the particles must be collected by adsorbents such as zeolite. We confirmed that the zeolite bearing cesium can be safely disposed after encapsulation by slag cement.

Report

(4 results)
  • 2014 Annual Research Report   Final Research Report ( PDF )
  • 2013 Annual Research Report
  • 2012 Annual Research Report
  • Research Products

    (38 results)

All 2015 2014 2013 2012 Other

All Journal Article (13 results) (of which Peer Reviewed: 13 results,  Open Access: 5 results,  Acknowledgement Compliant: 1 results) Presentation (22 results) (of which Invited: 8 results) Book (3 results)

  • [Journal Article] A passive collection system for whole size fractions in river suspended solids2015

    • Author(s)
      T. Matsunaga, T. Nakanishi, M. Atarashi-Andoh, E. Takeuchi, K. Tsuduki, S. Nishimura, J. Koarashi, S. Otosaka, T. Sato, S. Nagao
    • Journal Title

      Journal of Radioanalytical Nuclear Chemistry

      Volume: 303 Issue: 2 Pages: 1291-1295

    • DOI

      10.1007/s10967-014-3491-5

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Na-montmorillonite dissolution rate determined by varying the2014

    • Author(s)
      C. Oda, C.Walker, D. Chino, S. Ichige, A. Honda, T. Sato, and T. Yoneda
    • Journal Title

      Applied Clay Science

      Volume: 83-94 Pages: 62-71

    • DOI

      10.1016/j.clay.2014.02.021

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Structural and chemical modification of nontronite associated with microbial Fe(III) reduction: Indicators of "illitization"2014

    • Author(s)
      Koo, T, Y. Jang, T. Kogure, J. H. Kim, B. C. Park, D. Sunwoo, and J. Kim
    • Journal Title

      Chemical Geology

      Volume: 377 Pages: 87-95

    • DOI

      10.1016/j.chemgeo.2014.04.005

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Uptake of cesium and strontium ions by artificially altered phlogopite2014

    • Author(s)
      Tamura, K., T. Kogure, Y. Watanabe, C. Nagai, and H. Yamada
    • Journal Title

      Environmental Science and Technology

      Volume: 48 Issue: 10 Pages: 5808-5815

    • DOI

      10.1021/es4052654

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Direct observation of cesium at the interlayer region in phlogopite mica2014

    • Author(s)
      Okumura, T., Tamura, K., Fujii, E., Yamada, H., Kogure, T.
    • Journal Title

      Microscopy

      Volume: 63 Issue: 1 Pages: 65-72

    • DOI

      10.1093/jmicro/dft045

    • Related Report
      2014 Annual Research Report 2013 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Speciation of radioactive soil particles in the Fukushima contaminated area by IP autoradiography and microanalyses2014

    • Author(s)
      Mukai, H., T. Hatta, H. Kitazawa, H. Yamada, T. Yaita, and T. Kogure
    • Journal Title

      Environmental Science and Technology

      Volume: 48 Issue: 22 Pages: 13053-13059

    • DOI

      10.1021/es502849e

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] 無機汚染物質の除去・隔離のための層状化合物2014

    • Author(s)
      佐藤努
    • Journal Title

      Journal of the Society of Inorganic Materials, Japan

      Volume: 368 Pages: 42-48

    • Related Report
      2014 Annual Research Report 2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Mineral Synthesis in Si-Al-Ca Systems and Their Iodide Sorption Capacity under Alkaline Conditions2013

    • Author(s)
      X.J. Liu, A. Asai, T. Sato, E. Opiso, T. Otake, and T. Yoneda
    • Journal Title

      Water Air and Soil Pollution

      Volume: 224 Issue: 3 Pages: 1442-1455

    • DOI

      10.1007/s11270-013-1442-3

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] On the nature of structural disorder in calcium silicate hydrates with a calcium/silicon ratio similar to tobermorite2013

    • Author(s)
      S. Grangeon, C. Claret, C. Lerouge, F. Warmont, T. Sato, S. Anraku, C. Numako, Y. Linard, B. Lanson
    • Journal Title

      Cement and Concrete Research

      Volume: 52 Pages: 31-37

    • DOI

      10.1016/j.cemconres.2013.05.007

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Structure of prismatic halloysite2013

    • Author(s)
      T. Kogure, K. Mori, V.A. Drits and Y. Takai
    • Journal Title

      Am. Mineral.

      Volume: 98 Issue: 5-6 Pages: 1008-1016

    • DOI

      10.2138/am.2013.4385

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Structure of mixed-layer corrensitechlorite revealed by high-resolution transmission electron microcopy (HRTEM)2013

    • Author(s)
      Kogure, T., Drits, V. A. and Inoue, S
    • Journal Title

      Am. Mineral

      Volume: 98 Issue: 7 Pages: 1253-1260

    • DOI

      10.2138/am.2013.4314

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Comparison of the vertical distributions of Fukushima nuclear accident radiocesium in soil before and after the first rainy season, with physicochemical and mineralogical interpretations2013

    • Author(s)
      T. Matsunaga, J. Koarashi a, Mariko Atarashi-Andoh a, Seiya Nagao b, Tsutomu Sato c, Haruyasu Nagai
    • Journal Title

      Science of the Total Environment

      Volume: 447 Pages: 301-314

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] 福島第一原発事故で発生した放射性廃棄物の処理・処分に内在する課題2012

    • Author(s)
      佐藤努
    • Journal Title

      セラミックス

      Volume: 4 7 Pages: 859-863

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Presentation] 福島汚染土壌におけるセシウム吸着箇所の探索2014

    • Author(s)
      向井広樹, 小暮敏博
    • Organizer
      第53回粘土科学討論会
    • Place of Presentation
      福島A・O・Z(アオウゼ)、福島
    • Year and Date
      2014-09-26
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] 福島県花崗岩中黒雲母の風化状態2014

    • Author(s)
      倉又千咲, 菊池亮佑, 甕聡子, 小暮敏博
    • Organizer
      第53回粘土科学討論会
    • Place of Presentation
      福島A・O・Z(アオウゼ)、福島
    • Year and Date
      2014-09-26
    • Related Report
      2014 Annual Research Report
  • [Presentation] アンモニウム型モンモリロナイトの層間イオンの挙動と膨張挙動2014

    • Author(s)
      齋藤彬人, 佐久間博, 小田治恵, 本田明, 佐藤努
    • Organizer
      第53回粘土科学討論会
    • Place of Presentation
      福島市 A ・ O ・ Z (アオウゼ )
    • Year and Date
      2014-09-26
    • Related Report
      2014 Annual Research Report
  • [Presentation] パッシブ除染2014

    • Author(s)
      佐藤努
    • Organizer
      第53回粘土科学討論会
    • Place of Presentation
      福島市 A ・ O ・ Z (アオウゼ )
    • Year and Date
      2014-09-26
    • Related Report
      2014 Annual Research Report
  • [Presentation] 放射性Csを吸着している粘土鉱物は何か ‐電子顕微鏡による探索‐2014

    • Author(s)
      小暮敏博, 向井広樹, 甕聡子
    • Organizer
      第53回粘土科学討論会
    • Place of Presentation
      福島A・O・Z(アオウゼ)、福島
    • Year and Date
      2014-09-25
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] 福島風化黒雲母へのCs吸着実験2014

    • Author(s)
      菊池亮佑, 向井広樹, 小暮敏博, 田村堅志
    • Organizer
      日本鉱物科学会2014年年会
    • Place of Presentation
      熊本大学、熊本
    • Year and Date
      2014-09-18
    • Related Report
      2014 Annual Research Report
  • [Presentation] IPオートラジオグラフィーと電子顕微鏡による土壌中放射性粒子の特定と分析2014

    • Author(s)
      小暮敏博
    • Organizer
      日本土壌肥料学会2014年度東京大会
    • Place of Presentation
      東京農工大学, 東京
    • Year and Date
      2014-09-11
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] 福島土壌の放射能汚染‐放射性核種はどこにいるのか-2014

    • Author(s)
      小暮敏博
    • Organizer
      日本顕微鏡学会第70回記念学術講演会
    • Place of Presentation
      幕張メッセ国際会議場, 千葉
    • Year and Date
      2014-05-11
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] 福島風化雲母へのCs吸着実験-HRTEM及びHAADF-STEMによる層間Csの可視化-2014

    • Author(s)
      菊池亮佑, 奥村大河, 熊本明仁, 小暮敏博
    • Organizer
      日本顕微鏡学会第70回記念学術講演会
    • Place of Presentation
      幕張メッセ国際会議場, 千葉
    • Year and Date
      2014-05-11
    • Related Report
      2014 Annual Research Report
  • [Presentation] 福島飯館村のリターに付着した放射性土壌粒子の鉱物特定2013

    • Author(s)
      小暮敏博、藤井英子、北澤英明、八田珠朗、山田裕久
    • Organizer
      第2回環境放射能除染研究発表会
    • Place of Presentation
      タワーホール船堀(東京都)
    • Related Report
      2013 Annual Research Report
  • [Presentation] The structural and chemical modification of nontronite associated with microbial Fe(III) reduction under various redox conditions: indicators of "Illitization"2013

    • Author(s)
      Koo, T., T. Kogure, J. Kim, J. Kim
    • Organizer
      50th Anniversary Meeting of the Clay Minerals Society
    • Place of Presentation
      University of Illinois(Illinois, USA)
    • Related Report
      2013 Annual Research Report
  • [Presentation] Structural variety of illite investigated by TEM2013

    • Author(s)
      Kogure, T., V. A. Drits
    • Organizer
      50th Anniversary Meeting of the Clay Minerals Society
    • Place of Presentation
      University of Illinois(Illinois, USA)
    • Related Report
      2013 Annual Research Report
  • [Presentation] UPTAKE AND DISPOSAL OF RADIOACTIVE CESIUM BY NATURAL INORGANIC MATERIALS AROUND FUKUSHIMA DAIICHI NUCLEAR POWER PLANT2012

    • Author(s)
      Syafina Binti Mohd Ghazi, Takato Nishita, Hajime Hasegawa, Isamu Matsubara, Tetsuro Yoneda, Tsubasa Otake and Tsutomu Sato
    • Organizer
      The_2<nd> Asian Clay Conference
    • Place of Presentation
      Ewha Womans University, Seoul, Korea
    • Year and Date
      2012-09-08
    • Related Report
      2012 Annual Research Report
  • [Presentation] 福島第一原子力発電所の事故で発生した放射性廃棄物の処理・処分に内在する課題

    • Author(s)
      佐藤努
    • Organizer
      日本地球惑星科学連合2013年大会
    • Place of Presentation
      幕張メッセ(千葉県千葉市)
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] 層状複水酸化物の沈殿課程における廃水中のニッケルの挙動

    • Author(s)
      岡橋 東子、西内 亨、佐藤 努、大竹 翼、米田 哲朗
    • Organizer
      日本地球惑星科学連合2013年大会
    • Place of Presentation
      幕張メッセ(千葉県千葉市)
    • Related Report
      2013 Annual Research Report
  • [Presentation] PROBLEMATICS AND ROLE OF CLAY MINERALOGISTS IN TREATMENT AND DISPOSAL OF THE RADIOACTIVE WASTE PRODUCED BY ACCIDENT AT FUKUSHIMA DAIICHI NPP

    • Author(s)
      T. Sato, H. Yamada, T. Yaita, and T. Hatta
    • Organizer
      International Clay Conference
    • Place of Presentation
      Federal University of Rio de Janeiro (ブラジル・リオデジャネイロ)
    • Related Report
      2013 Annual Research Report
  • [Presentation] Let’s use metastable geomaterials in environmental protection –An intelligent geotechnology learnt from natural processes-

    • Author(s)
      T. Sato and K. Fukushi
    • Organizer
      Goldschmidt Conference 2013
    • Place of Presentation
      Firenze Fiera Congress and Exhibition Center (イタリア・フローレンス)
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] UPTAKE OF RADIOACTIVE CESIUM EMITTED FROM FUKUSHIMA DAIICHI NUCLEAR POWER PLANT BY DIATOMACEOUS EARTH

    • Author(s)
      S. Ghazi1, T. Nishita1, H. Hasegawa1, I. Matsubara, T. Yoneda, T. Otake and T. Sato
    • Organizer
      International Clay Conference
    • Place of Presentation
      Federal University of Rio de Janeiro (ブラジル・リオデジャネイロ)
    • Related Report
      2013 Annual Research Report
  • [Presentation] 福島原発事故で発生した廃棄物の合理的な処理・処分システム構築に向けた基盤研究;(21)セシウムを含むプルシアンブルーの安定性に及ぼす微生物活動の影響

    • Author(s)
      中村隆光,石井 聡,佐藤 努,岡部 聡
    • Organizer
      日本原子力学会2014年春の年会
    • Place of Presentation
      東京都市大学(東京都)
    • Related Report
      2013 Annual Research Report
  • [Presentation] セメント固化処理によるセシウム吸着ゼオライトからのセシウムイオン溶出抑制

    • Author(s)
      石川玲奈,佐藤 努,名和豊春
    • Organizer
      日本原子力学会2014年春の年会
    • Place of Presentation
      東京都市大学(東京都)
    • Related Report
      2013 Annual Research Report
  • [Presentation] Real Structures of Clay Minerals Revealed by HRTEM

    • Author(s)
      Kogure, T.
    • Organizer
      2nd International Conference - CMLM2013
    • Place of Presentation
      Russian Academy of Sciences(St. Petersburg, Russia)
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Finding and analyses of soil particles adsorbing radioactive cesium in Fukushima

    • Author(s)
      Kogure, T.
    • Organizer
      Caesium Workshop: Fukushima recovery - understanding, modelling and managing radiocaesium decontamination
    • Place of Presentation
      CORASSE, Fukushima
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Book] 地球表層物質と結晶学, 日本の結晶学(II)-その輝かしい発展 -2014

    • Author(s)
      小暮敏博
    • Total Pages
      2
    • Publisher
      日本結晶学会
    • Related Report
      2014 Annual Research Report
  • [Book] 放射性物質の吸着・除染および耐放射線技術における材料・施工・測定の新技術2014

    • Author(s)
      山田裕久, 横山信吾, 渡辺雄二郎, 中田弘太郎, 田村堅志, 佐藤努, 八田珠郎
    • Total Pages
      638
    • Publisher
      技術情報協会
    • Related Report
      2014 Annual Research Report
  • [Book] セシウムをどうする 福島原発事故 除染のための基礎知識2012

    • Author(s)
      日本イオン交換学会 編
    • Total Pages
      160
    • Publisher
      日刊工業新聞社
    • Related Report
      2012 Annual Research Report

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Published: 2012-04-24   Modified: 2019-07-29  

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